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Effects of lattice disorder in the UCu_(5-x)Pd_(x) system

E. D. Bauer·C. H. Booth·G. H. Kwei·R. Chau·M. B. Maple
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Abstract

The UCu(5-x)Pd(x) system exhibits non-Fermi liquid (NFL) in the thermodynamic and transport properties at low temperatures for Pd concentrations 0.9 <~ x <~ 1.5. The local structure around the U, Cu, and Pd atoms has been measured for 0 <= x <= 1.5 using the X-ray Absorption Fine Structure (XAFS) technique in order to quantify the effects of lattice disorder on the NFL properties. A model which allows a percentage of the Pd atoms to occupy nominal Cu (16e) sites, s, was used to fit the Pd and Cu K edge and U L(III) edge data. Pd/Cu site interchange was found to occur in all samples (x != 0), reaching a minimum value of s ~0.17 at x = 0.7 and increasing monotonically to s ~ 0.4 at x=1.5. These data also determine the static disorder the nearest neighbor U--Cu pairs. The results indicate that the measured U--Cu static disorder is not sufficient to explain the NFL behavior of the magnetic susceptibility within the single-ion Kondo disorder model and casts doubt on the applicability of this model to UCu(5-x)Pd(x).

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E. D. Bauer, C. H. Booth, G. H. Kwei, R. Chau, M. B. Maple. 2002-05-07. Effects of lattice disorder in the UCu_(5-x)Pd_(x) system. https://doi.org/10.1103/physrevb.65.245114

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