arXiv subjects

Alexander A. High

Publications and source records attributed to Alexander A. High.

22 records · Page 2Linked to original sources

arXiv2017

Atomically thin mirrors made of monolayer semiconductors

Transition metal dichalcogenide monolayers are promising candidates for exploring new electronic and optical phenomena and for realizing atomically thin optoelectronic devices. They host tightly bound electron-hole pairs (excitons) that can be efficiently excited by resonant light fields. Here, we demonstrate that a single monolayer of molybdenum diselenide (MoSe2) can dramatically modify light transmission near the excitonic resonance, acting as an electrically switchable mirror that reflects up to 85% of incident light at cryogenic temperatures. This high reflectance is a direct consequence of the excellent coherence properties of excitons in this atomically thin semiconductor, encapsulated by hexagonal boron nitride. Furthermore, we show that the MoSe2 monolayer exhibits power- and wavelength-dependent nonlinearities that stem from exciton-based lattice heating in the case of continuous-wave excitation and exciton-exciton interactions when fast, pulsed laser excitation is used. These observations open up new possibilities for studying quantum nonlinear optical phenomena and topological photonics, and for miniaturizing optical devices.

cond-mat.mes-hall↗

arXiv2017

Probing dark excitons in atomically thin semiconductors via near-field coupling to surface plasmon polaritons

Transition metal dichalcogenide (TMD) monolayers are direct bandgap semiconductors that feature tightly bound excitons, strong spin-orbit coupling, and spin-valley degrees of freedom. Depending on the spin configuration of the electron-hole pairs, intra-valley excitons of TMD monolayers can be either optically bright or dark. Dark excitons involve nominally spin-forbidden optical transitions with zero in-plane transition dipole moment, making their detection with conventional far-field optical techniques challenging. Here, we introduce a new method for probing the optical properties of two-dimensional (2D) materials via near-field coupling to surface plasmon polaritons (SPPs), which selectively enhances optical transitions with dipole moments normal to the 2D plane. We utilize this method to directly detect dark excitons in monolayer TMDs. When a WSe2 monolayer is placed on top of a single-crystal silver film, its emission into near-field-coupled SPPs displays new spectral features whose energies and dipole orientations are consistent with dark neutral and charged excitons. The SPP-based near-field spectroscopy significantly enhances experimental capabilities for probing and manipulating exciton dynamics of atomically thin materials.

cond-mat.mes-hall↗

arXiv2011

Spontaneous coherence of indirect excitons in a trap

We report on the emergence of spontaneous coherence in a gas of indirect excitons in an electrostatic trap. At low temperatures, the exciton coherence length becomes much larger than the thermal de Broglie wavelength and reaches the size of the exciton cloud in the trap.

cond-mat.quant-gas↗

arXiv2011

Spontaneous Coherence in a Cold Exciton Gas

Excitons, bound pairs of electrons and holes, form a model system to explore the quantum physics of cold bosons in solids. Cold exciton gases can be realized in a system of indirect excitons, which can cool down below the temperature of quantum degeneracy due to their long lifetimes. Here, we report on the measurement of spontaneous coherence in a gas of indirect excitons. We found that extended spontaneous coherence of excitons emerges in the region of the macroscopically ordered exciton state and in the region of vortices of linear polarization. The coherence length in these regions is much larger than in a classical gas, indicating a coherent state with a much narrower than classical exciton distribution in momentum space, characteristic of a condensate. We also observed phase singularities in the coherent exciton gas. Extended spontaneous coherence and phase singularities emerge when the exciton gas is cooled below a few Kelvin.

cond-mat.mes-hall↗