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Andrew Attar

Publications and source records attributed to Andrew Attar.

6 recordsLinked to original sources

Development of a Photonically Generated Frequency Reference for Space VLBI

Space-based Very Long Baseline Interferometry (VLBI) can improve both the angular and temporal resolution of images over terrestrial VLBI techniques. Future space VLBI (sVLBI) missions are targeting higher observation frequencies than modern, terrestrial VLBI, and therefore these missions will require higher stability frequency references than standard hydrogen masers. While existing frequency references for space-based applications have concentrated on long-term stability, in this effort, we present a frequency reference with high short-term stability intended for sVLBI missions. This reference leverages developments in cavity-stabilized lasers from the Laser Interferometer Space Antenna (LISA) mission and commercial efforts towards a robust, space-qualifiable optical frequency comb. We describe the implementation and experimental results of this system with a path to spaceflight, which demonstrates an Allan deviation of $3.26 \times 10^{-14}$ at 1 second, $6.00 \times 10^{-15}$ at 10 seconds, and $6.73 \times 10^{-15}$ at 30 seconds for the 100 MHz frequency reference signal, and show that this performance meets the needs of future sVLBI missions.

astro-ph.IM↗

Environmental qualification and performance of a CubeSat-scale dual optical frequency comb payload for space applications

We report the environmental qualification and performance of CombSat, a dual optical frequency comb payload designed for deployment on a 12U CubeSat in low Earth orbit. The payload integrates two self-referenced, 200 MHz hybrid fiber-waveguide frequency combs, a narrow-linewidth optical reference, a heterodyne beat detection unit, and FPGA-based control electronics in a total mass of 8.3 kg and volume of 5.7 L, and nominal power consumption of 21W. We describe the mechanical, thermal, and radiation-tolerant design features of the system and present the results of random vibration, storage temperature cycling, and thermal-vacuum testing conducted in accordance with NASA's General Environmental Verification Standard. We show that key comb performance metrics including oscillator and amplifier output power, frep, fCEO, and fopt signal-to-noise ratios, and integrated phase noise, remain within specification after environmental exposure, and we discuss observed failure modes and design modifications that improved robustness. These results demonstrate that compact, low power, fully stabilized, autonomous dual-comb systems can be engineered and qualified for spaceflight on CubeSat platforms, providing a path forward for future low-cost comb-based space applications.

physics.optics↗

Ultra-low noise laser and optical frequency comb-based timing system for the Black Hole Explorer (BHEX) mission

In this effort, we demonstrate the performance of a highly stable time reference for the proposed Black Hole Explorer (BHEX) mission, a space-based extension to the Event Horizon Telescope (EHT) Very Long Baseline Interferometry (VLBI) project. This precision timing system is based on the use of a space-qualified, ultra-low noise laser developed as part of the Laser Interferometer Space Antenna (LISA) mission as the timing reference, and an optical frequency comb to transfer the stability of this laser to the microwave regime for instrumentation use. We describe the implementation of this system and experimental setup to characterize the stability performance. We present the results of this experiment that demonstrate the performance of this system meets requirements for the BHEX mission.

astro-ph.IM↗

X-ray Free Electron Laser Studies of Electron and Phonon Dynamics of Graphene Adsorbed on Copper

We report optical pumping and X-ray absorption spectroscopy experiments at the PAL free electron laser that directly probe the electron dynamics of a graphene monolayer adsorbed on copper in the femtosecond regime. By analyzing the results with ab-initio theory we infer that the excitation of graphene is dominated by indirect excitation from hot electron-hole pairs created in the copper by the optical laser pulse. However, once the excitation is created in graphene, its decay follows a similar path as in many previous studies of graphene adsorbed on semiconductors, i e. rapid excitation of SCOPS (Strongly Coupled Optical Phonons) and eventual thermalization. It is likely that the lifetime of the hot electron-hole pairs in copper governs the lifetime of the electronic excitation of the graphene.

cond-mat.mes-hall↗

Rehybridization dynamics into the pericyclic minimum of an electrcyclic reaction imaged in real-time

Electrocyclic reactions are characterized by the concerted formation and cleavage of both σ and π bonds through a cyclic structure. This structure is known as a pericyclic transition state for thermal reactions and a pericyclic minimum in the excited state for photochemical reactions. However, the structure of the pericyclic geometry has yet to be observed experimentally. We use a combination of ultrafast electron diffraction and excited state wavepacket simulations to image structural dynamics through the pericyclic minimum of a photochemical electrocyclic ring-opening reaction in the molecule α-terpinene. The structural motion into the pericyclic minimum is dominated by rehybridization of two carbon atoms, which is required for the transformation from two to three conjugated π bonds. The σ bond dissociation largely happens after internal conversion from the pericyclic minimum to the electronic ground state. These findings may be transferrable to electrocyclic reactions in general.

physics.chem-ph↗

Direct visualization of ultrafast lattice ordering triggered by an electron-hole plasma in 2D perovskites

Direct visualization of ultrafast coupling between charge carriers and lattice degrees of freedom in photo-excited semiconductors has remained a long-standing challenge and is critical for understanding the light-induced physical behavior of materials under extreme non-equilibrium conditions. Here, by monitoring the evolution of the wave-vector resolved ultrafast electron diffraction intensity following above-bandgap photo-excitation, we obtain a direct visual of the structural dynamics in monocrystalline 2D perovskites. Analysis reveals a surprising, light-induced ultrafast lattice ordering resulting from a strong interaction between hot-carriers and the perovskite lattice, which induces an in-plane octahedra rotation, towards a more symmetric phase. Correlated ultrafast spectroscopy performed at the same carrier density as ultrafast electron diffraction reveals that the creation of a hot and dense electron-hole plasma triggers lattice ordering at short timescales by modulating the crystal cohesive energy. Finally, we show that the interaction between the carrier gas and the lattice can be altered by tailoring the rigidity of the 2D perovskite by choosing the appropriate organic spacer layer.

cond-mat.mtrl-sci↗