arXiv subjects

C. Walz

Publications and source records attributed to C. Walz.

7 recordsLinked to original sources

arXiv2026

Ultrafast Dissipative Localization of Electronic Energy in AuPt Superlattices

Controlling the spatial distribution of absorbed optical energy is central to nanoscale photothermal chemistry, plasmonics, and ultrafast materials control. Here, we show that a metallic AuPt superlattice concentrates electronic energy in Pt within a few hundred femtoseconds, regardless of the initial energy distribution between the two constituents. Ultrafast X-ray diffraction follows this energy redistribution through the amplitude of a coherent 570 GHz superlattice phonon driven by the stress imbalance at the AuPt interfaces. Despite the nearly homogeneous absorption at 400 nm, the observed lattice motion is identical to that produced by 800 nm excitation, which is absorbed predominantly in Pt. This dissipation driven localization of energy arises from the large electronic heat capacity of Pt and rapid electronic transport through the superlattice, providing a route to femtosecond control of nanoscale energy distributions.

cond-mat.mtrl-sci↗

arXiv2026

Low-energy collective structure of $^{92,94}$Zr and $^{94}$Mo from ($e,e^{\prime}$) and ($p,p^{\prime}$) scattering I. Experimental results

This is the first of two papers discussing a new signature of quadrupole mixed-symmetry states in the vibrational nuclei $^{92,94}$Zr and $^{94}$Mo based on proton and neutron transition densities derived from the comparison of inelastic electron and proton scattering experiments. Results of the $(e,e^\prime)$ and $(p,p^\prime)$ experiments on these nuclei as well as $(p,p^\prime)$ data for other potential cases $^{96}$Mo and $^{70}$Zn are presented. Spin and parity quantum numbers of excited states are assigned based on angular distributions from the proton scattering data in comparison to calculations employing form factors from the collective model in distorted-wave Born approximation. Possible candidates of one-phonon fully symmetric and mixed-symmetry states as well as members of two-phonon multiplets are identified.

nucl-ex↗

arXiv2026

Low-energy collective structure of $^{92,94}$Zr and $^{94}$Mo from ($e,e^{\prime}$) and ($p,p^{\prime}$) scattering II. Signatures of mixed-symmetry states and origin of collectivity

This is the second of two papers discussing a new experimental signature of mixed-symmetry states (MSS) in the vibrational nuclei $^{92,94}$Zr and $^{94}$Mo based on proton and neutron transition densities. Quasiparticle-phonon model calculations for these nuclei are extensively tested by comparison to ground-state properties, energies and moments of excited states, transition probabilities between them, and the momentum transfer dependence in $(e,e^\prime)$ and $(p,p^\prime)$ reactions. The overall very good agreement permits the extraction of information on the wave functions of the MSS and their fully symmetric (FSS) counterparts. MSS can be identified by a sign change between the leading proton and neutron two-quasiparticle configurations compared to the FSS. Possible candidates for $2^+$, $3^-$, and $4^+$ MSS are identified. The modification of proton and neutron transition densities, which can be derived from a combined analysis of inelastic electron and proton scattering, by the sign change provide a new experimental signature of MSS. The collectivity of ground-state excitations of predominantly one-phonon FSS and MSS is generated to a large extent by the coupling to high-lying states forming giant resonances with the same spin and parity.

nucl-ex↗

arXiv2025

Large strain contribution to the laser-driven magnetization response of magnetostrictive TbFe$_{2}$

We investigate strain-induced contributions to the transient polar magneto-optical Kerr effect response in laser-excited terfenol. The tr-MOKE signals obtained from TbFe$_{2}$ films with and without glass capping exhibit distinct signatures associated with transient strain. We experimentally observe the arrival of strain pulses via the reflectivity change. The tr-MOKE response measured without changing the pump-probe geometry is delayed by several picoseconds. This suggests a genuine magnetization response as opposed to instantaneous changes of optical constants as the origin of the signal. We model the propagation of longitudinal acoustic picosecond strain pulses and incorporate the inverse magnetostriction effect via a magnetoelastic term in the effective field of the Landau-Lifshitz-Gilbert equation with large damping. This reproduces not only the delay of the pulsed response, but also unveils the dominant contribution of quasi-static strain to the magnetization dynamics due to the thermal expansion in the optically probed near-surface region. Our experiments exemplify that purely longitudinal strain along the out-of-plane direction of the thin film enables efficient magnetoelastic coupling via the shear strain components arising in the oblique crystallographic frame of reference.

cond-mat.mtrl-sci↗

arXiv2016

Unexpected distribution of $\nu1f_{7/2}$ strength in the calcium isotopes at $N$=30

The calcium isotopes have emerged as an important testing ground for new microscopically derived shell-model interactions, and a great deal of focus has been directed toward this region. We investigate the relative spectroscopic strengths associated with $1f_{7/2}$ neutron hole states in $^{47, 49}$Ca following one-neutron knockout reactions from $^{48,50}$Ca. The observed reduction of strength populating the lowest 7/2$^{-}_{1}$ state in $^{49}$Ca, as compared to $^{47}$Ca, is consistent with the description given by shell-model calculations based on two- and three-nucleon forces in the neutron $pf$ model space, implying a fragmentation of the $l$=3 strength to higher-lying states. The experimental result is inconsistent with both the GXPF1 interaction routinely used in this region of the nuclear chart and with microscopic calculations in an extended model space including the $\nu1g_{9/2}$ orbital.

nucl-ex↗

arXiv2015

Neutron single-particle strength in silicon isotopes: Constraining the driving forces of shell evolution

Shell evolution is studied in the neutron-rich silicon isotopes 36,38,40 Si using neutron single-particle strengths deduced from one-neutron knockout reactions. Configurations involving neutron excita- tions across the N = 20 and N = 28 shell gaps are quantified experimentally in these rare isotopes. Comparisons with shell model calculations show that the tensor force, understood to drive the col- lective behavior in 42 Si with N = 28, is already important in determining the structure of 40 Si with N = 26. New data relating to cross-shell excitations provide the first quantitative support for repulsive contributions to the cross-shell T = 1 interaction arising from three-nucleon forces.

nucl-ex↗

arXiv2013

E2 strengths and transition radii difference of one-phonon 2+ states of 92Zr from electron scattering at low momentum transfer

Background: Mixed-symmetry 2+ states in vibrational nuclei are characterized by a sign change between dominant proton and neutron valence-shell components with respect to the fully symmetric 2+ state. The sign can be measured by a decomposition of proton and neutron transition radii with a combination of inelastic electron and hadron scattering [C. Walz et al., Phys. Rev. Lett. 106, 062501 (2011)]. For the case of 92Zr, a difference could be experimentally established for the neutron components, while about equal proton transition radii were indicated by the data. Method: Differential cross sections for the excitation of one-phonon 2+ and 3- states in 92Zr have been measured with the (e,e') reaction at the S-DALINAC in a momentum transfer range q = 0.3-0.6 fm^(-1). Results: Transition strengths B(E2;2+_1 -> 0+_1) = 6.18(23), B(E2; 2+_2 -> 0+_1) = 3.31(10) and B(E3; 3-_1 -> 0+_1) = 18.4(11) Weisskopf units are determined from a comparison of the experimental cross sections to quasiparticle-phonon model (QPM) calculations. It is shown that a model-independent plane wave Born approximation (PWBA) analysis can fix the ratio of B(E2) transition strengths to the 2+_(1,2) states with a precision of about 1%. The method furthermore allows to extract their proton transition radii difference. With the present data -0.12(51) fm is obtained. Conclusions: Electron scattering at low momentum transfers can provide information on transition radii differences of one-phonon 2+ states even in heavy nuclei. Proton transition radii for the 2+_(1,2) states in 92Zr are found to be identical within uncertainties. The g.s. transition probability for the mixed-symmetry state can be determined with high precision limited only by the available experimental information on the B(E2; 2+_1 -> 0+_1) value.

nucl-ex↗