arXiv subjects

Carter Fox

Publications and source records attributed to Carter Fox.

9 recordsLinked to original sources

arXiv2026

Electrically switchable ferron upconversion in a van der Waals ferroelectric

Nonlinear phononics provides a powerful ultrafast route to control lattice excitations, enabling access to hidden quantum orders, phononic computing, and quantum transduction. However, dynamic control of anharmonic phonon interactions remains limited, as these interactions are typically fixed by the equilibrium crystal lattice and lack external tunability. Emergent ferrons in ferroelectrics, which are collective oscillations of the spontaneous electric polarization, may offer a promising platform to overcome this limitation by combining intrinsic phononic nonlinearity with direct electrical control of the ferroelectric order parameter. Here we report electrically controllable nonlinear ferron upconversion in the van der Waals ferroelectric NbOI2. We show that resonant THz excitation of a 3.1 THz ferron drives coherent upconversion to a 7.0 THz optical phonon. Using two-dimensional THz spectroscopy, we directly resolve off-diagonal coupling features and establish the nonlinear upconversion pathway. Supported by first-principles calculations and analytical modeling, we identify the microscopic origin as a cubic anharmonic lattice coupling. Importantly, in situ electric-field switching enables nonvolatile control of both the ferron dynamics and the associated upconversion process. The phase reversal and hysteretic behavior across the coercive fields establish that the ferron-mediated nonlinear phononic interaction is strongly dependent on the underlying ferroelectric order parameter. These results introduce ferron upconversion as a new and universal regime of nonlinear phononics in ferroelectrics and establish an electrically programmable platform for coherent lattice control, paving the way for ferronic information processing and quantum phononic transduction.

cond-mat.mtrl-sci↗

arXiv2026

Visualizing Nanoscopic Acoustic Mode Competition in van der Waals Ferroelectric

Understanding how low-dimensional ferroelectrics respond to ultrafast excitation at nanoscales is essential for controlling energy flow and mechanical functionality in next-generation polar devices, yet the nanoscopic structural response to ultrafast depolarization remains unresolved, obscuring the microscopic pathways of acoustic decoherence and energy dissipation. Here, we spatiotemporally resolve lattice motion in the van der Waals ferroelectric NbOI2 using combined ultrafast electron microscopy and diffraction, revealing three acoustic phonons: two transverse shear modes and one longitudinal breathing mode. The transverse mode that shears the layers perpendicular to the in-plane polar axis dominates over that along the polar axis, reflecting anisotropic polarization-strain coupling. Real-space mapping uncovers spatially correlated heterogeneity in mode amplitudes and lifetimes. Regions dominated by a single shear mode exhibit significantly longer acoustic lifetimes than multimode regions, suggesting acoustic phonon-phonon scattering as a major source of decoherence. Our results provide a microscopic understanding of ultrafast depolarization-driven acoustic dynamics and spatially heterogeneous energy dissipation in van der Waals ferroelectrics.

cond-mat.mtrl-sci↗

arXiv2025

Sliding multiferroicity in hexagonal stacked CrI3

Developing new multiferroics at the two-dimensional (2D) limit with energy-efficient magnetoelectric coupling can inform the interplay physics of novel orders and advance on-chip high-performance computing applications. Here we apply stacking order engineering to create a new type of 2D multiferroics, namely sliding multiferroics, based on polar hexagonal stacked (H-stacked) CrI3. This new stacking order removes structural inversion symmetry and gives rise to room temperature sliding ferroelectricity, as confirmed by Raman spectroscopy, second harmonic generation spectroscopy and electrical transport measurements. Building upon the gate-dependent reflective magnetic circular dichroism, first-principles calculations, and modeling, sliding ferroelectricity is shown to interplay with an emergent interfacial ferromagnetism via interlayer spin-polarized charge transfer. This coupling mechanism results in non-volatile magnetic switching by as low as 0.4V across the H-stacked CrI3. Our demonstration introduces polar stacking order engineering of 2D magnets as a general approach to create non-volatile 2D multiferroics with efficient magnetoelectric coupling, paving the way for low-power electronics and spintronics at the atomically thin limit.

cond-mat.mtrl-sci↗

arXiv2024

Colossal terahertz emission with ultrafast tunability based on van der Waals ferroelectric NbOI$_2$

Terahertz (THz) technology is critical for quantum material physics, biomedical imaging, ultrafast electronics, and next-generation wireless communications. However, standing in the way of widespread applications is the scarcity of efficient ultrafast THz sources with on-demand fast modulation and easy on-chip integration capability. Here we report the discovery of colossal THz emission from a van der Waals (vdW) ferroelectric semiconductor NbOI$_2$. Using THz emission spectroscopy, we observe a THz generation efficiency an order of magnitude higher than that of ZnTe, a standard nonlinear crystal for ultrafast THz generation. We further uncover the underlying generation mechanisms associated with its large ferroelectric polarization by studying the THz emission dependence on excitation wavelength, incident polarization and fluence. Moreover, we demonstrate the ultrafast coherent amplification and annihilation of the THz emission and associated coherent phonon oscillations by employing a double-pump scheme. These findings combined with first-principles calculations, inform new understanding of the THz light-matter interaction in emergent vdW ferroelectrics and pave the way to develop high-performance THz devices on them for quantum materials sensing and ultrafast electronics.

cond-mat.mtrl-sci↗

arXiv2022

Nanoscale covariance magnetometry with diamond quantum sensors

Nitrogen vacancy (NV) centers in diamond are atom-scale defects with long spin coherence times that can be used to sense magnetic fields with high sensitivity and spatial resolution. Typically, the magnetic field projection at a single point is measured by averaging many sequential measurements with a single NV center, or the magnetic field distribution is reconstructed by taking a spatial average over an ensemble of many NV centers. In averaging over many single-NV center experiments, both techniques discard information. Here we propose and implement a new sensing modality, whereby two or more NV centers are measured simultaneously, and we extract temporal and spatial correlations in their signals that would otherwise be inaccessible. We analytically derive the measurable two-point correlator in the presence of environmental noise, quantum projection noise, and readout noise. We show that optimizing the readout noise is critical for measuring correlations, and we experimentally demonstrate measurements of correlated applied noise using spin-to-charge readout of two NV centers. We also implement a spectral reconstruction protocol for disentangling local and nonlocal noise sources, and demonstrate that independent control of two NV centers can be used to measure the temporal structure of correlations. Our covariance magnetometry scheme has numerous applications in studying spatiotemporal structure factors and dynamics, and opens a new frontier in nanoscale sensing.

quant-ph↗

arXiv2021

The Strongest Cluster Lenses: An Analysis of the Relation Between Strong Gravitational Lensing Strength and the Physical Properties of Galaxy Clusters

Strong gravitational lensing provides unique opportunities to investigate the mass distribution at the cores of galaxy clusters and to study high redshift galaxies. Using $94$ strong lensing models of $74$ cluster fields from the \textit{Hubble} Frontier Fields (HFF), Reionization Lensing Cluster Survey (RELICS), and Sloan Giant Arcs Survey (SGAS), modeled with three parametric approaches, we evaluate the lensing strength of each cluster (area with $|\mu|\geq3$ for $z_s=9$). We assess how large scale mass, projected inner core mass, and the inner slope of the projected mass density profile relate to lensing strength. While we do not identify a strong correlation between lensing strength and large scale mass, we reveal that the inner slope ($50$ kpc~$\leq r \leq~200$ kpc) of the projected mass density profile is indicative of lensing strength and can set an upper bound on the possible lensing strength of a cluster. We find that the effective Einstein area correlates with lensing strength, and that a large ($\gtrsim 30^{''}0$) radial extent of lensing evidence is a strong indicator of a powerful lens. These results can help to more efficiently design future observations to maximize lensing strength.

astro-ph.CO↗

arXiv2019

RELICS: A Very Large ($\theta_{E}\sim40"$) Cluster Lens -- RXC J0032.1+1808

Extensive surveys with the \textit{Hubble Space Telescope} (HST) over the past decade, targeting some of the most massive clusters in the sky, have uncovered dozens of galaxy-cluster strong lenses. The massive cluster strong-lens scale is typically $\theta_{E}\sim10\arcsec$ to $\sim30-35\arcsec$, with only a handful of clusters known with Einstein radii $\theta_{E}\sim40\arcsec$ or above (for $z_{source}=2$, nominally). Here we report another very large cluster lens, RXC J0032.1+1808 ($z=0.3956$), the second richest cluster in the redMapper cluster catalog and the 85th most massive cluster in the Planck Sunyaev-Zel'dovich catalog. With our Light-Traces-Mass and fully parametric (dPIEeNFW) approaches, we construct strong lensing models based on 18 multiple images of 5 background galaxies newly identified in the \textit{Hubble} data mainly from the \textit{Reionization Lensing Cluster Survey} (RELICS), in addition to a known sextuply imaged system in this cluster. Furthermore, we compare these models to Lenstool and GLAFIC models that were produced independently as part of the RELICS program. All models reveal a large effective Einstein radius of $\theta_{E}\simeq40\arcsec$ ($z_{source}=2$), owing to the obvious concentration of substructures near the cluster center. Although RXC J0032.1+1808 has a very large critical area and high lensing strength, only three magnified high-redshift candidates are found within the field targeted by RELICS. Nevertheless, we expect many more high-redshift candidates will be seen in wider and deeper observations with \textit{Hubble} or \emph{JWST}. Finally, the comparison between several algorithms demonstrates that the total error budget is largely dominated by systematic uncertainties.

astro-ph.CO↗

arXiv2019

RELICS: Reionization Lensing Cluster Survey

Large surveys of galaxy clusters with the Hubble and Spitzer Space Telescopes, including CLASH and the Frontier Fields, have demonstrated the power of strong gravitational lensing to efficiently deliver large samples of high-redshift galaxies. We extend this strategy through a wider, shallower survey named RELICS, the Reionization Lensing Cluster Survey. This survey, described here, was designed primarily to deliver the best and brightest high-redshift candidates from the first billion years after the Big Bang. RELICS observed 41 massive galaxy clusters with Hubble and Spitzer at 0.4-1.7um and 3.0-5.0um, respectively. We selected 21 clusters based on Planck PSZ2 mass estimates and the other 20 based on observed or inferred lensing strength. Our 188-orbit Hubble Treasury Program obtained the first high-resolution near-infrared images of these clusters to efficiently search for lensed high-redshift galaxies. We observed 46 WFC3/IR pointings (~200 arcmin^2) with two orbits divided among four filters (F105W, F125W, F140W, and F160W) and ACS imaging as needed to achieve single-orbit depth in each of three filters (F435W, F606W, and F814W). As previously reported by Salmon et al., we discovered 322 z ~ 6 - 10 candidates, including the brightest known at z ~ 6, and the most distant spatially-resolved lensed arc known at z ~ 10. Spitzer IRAC imaging (945 hours awarded, plus 100 archival) has crucially enabled us to distinguish z ~ 10 candidates from z ~ 2 interlopers. For each cluster, two HST observing epochs were staggered by about a month, enabling us to discover 11 supernovae, including 3 lensed supernovae, which we followed up with 20 orbits from our program. We delivered reduced HST images and catalogs of all clusters to the public via MAST and reduced Spitzer images via IRSA. We have also begun delivering lens models of all clusters, to be completed before the JWST GO call for proposals.

astro-ph.GA↗

arXiv2018

RELICS: Strong Lensing Analysis of MACS J0417.5-1154 and Predictions for Observing the Magnified High-Redshift Universe with JWST

Strong gravitational lensing by clusters of galaxies probes the mass distribution at the core of each cluster and magnifies the universe behind it. MACS J0417.5-1154 at z=0.443 is one of the most massive clusters known based on weak lensing, X-ray, and Sunyaev-Zel'dovich analyses. Here we compute a strong lens model of MACS J0417 based on Hubble Space Telescope imaging observations collected, in part, by the Reionization Lensing Cluster Survey (RELICS), and recently reported spectroscopic redshifts from the MUSE instrument on the Very Large Telescope (VLT). We measure an Einstein radius of ThetaE=36'' at z = 9 and a mass projected within 200 kpc of M(200 kpc) = 1.78+0.01-0.03x10**14Msol. Using this model, we measure a ratio between the mass attributed to cluster-member galaxy halos and the main cluster halo of order 1:100. We assess the probability to detect magnified high-redshift galaxies in the field of this cluster, both for comparison with RELICS HST results and as a prediction for the James Webb Space Telescope (JWST) Guaranteed Time Observations upcoming for this cluster. Our lensing analysis indicates that this cluster has similar lensing strength to other clusters in the RELICS program. Our lensing analysis predicts a detection of at least a few z~6-8 galaxies behind this cluster, at odds with a recent analysis that yielded no such candidates in this field. Reliable strong lensing models are crucial for accurately predicting the intrinsic properties of lensed galaxies. As part of the RELICS program, our strong lensing model produced with the Lenstool parametric method is publicly available through the Mikulski Archive for Space Telescopes (MAST).

astro-ph.GA↗