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Changle Liu

Publications and source records attributed to Changle Liu.

At least 19 recordsLinked to original sources

Quasi-one-dimensional spin excitations in the iron pnictide NaFe$_{0.53}$Cu$_{0.47}$As

Spectroscopic measurements in model one-dimensional (1D) correlated systems offer insights for understanding their two-dimensional counterparts, which include the cuprate and iron pnictide/chalcogenide superconductors. A major challenge is the identification of such correlated systems with dominantly 1D physics. In this work, inelastic neutron scattering measurements on NaFe$_{0.53}$Cu$_{0.47}$As single crystal directly reveal quasi-1D spin excitations, resulting from atomic order that lead to magnetic Fe and nonmagnetic Cu chains. The dominant exchange interaction is antiferromagnetic along the chain ($SJ_{\rm \parallel}\approx90.1(3)$~meV), whereas the inter-chain couplings are much weaker ($SJ_{\rm \perp}\approx-2.4(1)$~meV and $SJ_{\rm c}\approx0.15(5)$~meV). The quasi-1D spin excitations in NaFe$_{0.53}$Cu$_{0.47}$As stem from both the N\'eel and stripe vectors, with N\'eel excitations sensitive to Fe impurities on the Cu site. The spin excitations in quasi-1D NaFe$_{0.53}$Cu$_{0.47}$As and quasi-2D FeSe exhibit a striking resemblance, suggesting a common origin for their coexistent stripe and N\'eel excitations. Our findings demonstrate magnetic dilution in NaFeAs leads to dimension reduction of its magnetic degree of freedom, presenting a strategy for discovering low-dimensional quantum materials.

cond-mat.str-el

Emergence of Kugel-Khomskii physics in quarter-filled bilayer correlated systems

We present a theoretical study of the low-energy physics of a quarter-hole-filled two-orbital bilayer Hubbard model motivated by transition-metal bilayer systems with strong orbital-selective interlayer hybridization. By explicitly treating the strong interlayer bonding of dz2 orbitals within a molecular orbital basis and projecting out high-energy electronic states, we derive a low-energy effective Kugel-Khomskii Hamiltonian describing the interplay between electron spin and emergent layer pseudospin degrees of freedom. We map out a rich ground state phase diagram featuring diverse spin and charge ordered states. These include conventional ferromagnetic and antiferromagnetic phases with layer staggered charge densities, a layer-coherent phase characterized by spontaneous interlayer quantum coherence, and a novel maximally spin-layer-entangled phase with a hidden composite spin-layer order. We show that this exotic hidden ordered phase arises from the spontaneous breaking of an emergent O(4) symmetry down to a O(3), manifesting a unique excitation spectrum with three entangled gapless Goldstone modes. Our results uncover a geometrically driven mechanism for realizing composite entanglement in strongly correlated bilayer systems and provide a concrete theoretical framework relevant to bilayer nickelate superconductors and other multi-component correlated materials.

cond-mat.str-el

Spectroscopic evidences for the spontaneous symmetry breaking at the $SO(5)$ deconfined critical point of $J$-$Q_3$ model

Recent numerical and theoretical studies on the two-dimensional $J$-$Q_3$ model suggests that the deconfined quantum critical point is actually a $SO(5)$-symmetry-enhanced first-order phase transition that is spontaneously broken to $O(4)$. However, this conclusion has mainly relied on finite-size scaling of the entanglement entropy, lacking direct evidence from physical observables.} Here, we investigate the dynamical spectra of spin and bond operators at the deconfined critical point of the $J$-$Q_3$ model using large-scale quantum Monte Carlo simulations, and contrasting them with the well-established $\mathrm{O(3)}$ Wilson-Fisher criticality in the $J_1$-$J_2$ Heisenberg model. Although both models exhibit two gapless magnon modes in the N\'eel phase, their critical behaviors diverge strikingly. At the $J_1$-$J_2$ critical point, the Higgs mode becomes gapless, yielding three gapless modes that reflect the full restoration of the $\mathrm{O(3)}$ symmetry. {In the $J$-$Q_3$ model, we instead observe four gapless transverse modes at the either side of the transition. This spectral feature, together with the entanglement entropy results, provides direct evidence for the weakly first-order scenario that the deconfined quantum critical point exhibits an emergent $\mathrm{SO(5)}$ symmetry that spontaneously breaks to $\mathrm{O(4)}$.

cond-mat.str-el

Nematicity in iron pnictides: phase competition and emergent symmetry

The phase diagram of iron-based superconductors contains a host of electronic orders, which are intimately connected with their superconductivity. Here we analyze the fluctuations of one type of nematic order in another. Our analysis leads to an emergent U(1) symmetry at a first-order transition between a nematic phase and a $C_4$-symmetric charge-ordered phase. We characterize the continuous symmetry in terms of a certain hidden Lie algebra that links the different orders. This emergent symmetry leads to a Goldstone mode at the transition and causes softening of excitations in the nematic and charge sectors near the transition. The underlying physics bears a resemblance to the anisotropic XZ spin model, with the nematic order and charge $C_4$ order parameters playing the roles of the $x$ and $z$ components of the magnetization vector, respectively. We provide the experimental evidence in support of the proposed effects, and discuss the general implications of our results for the physics of iron-based superconductors and other correlated systems.

cond-mat.str-el

Doped resonating-valence-bond states: Robustness of the spin-ice phases in three-dimensional Rydberg arrays

Rydberg blockade effect provides a convenient platform for simulating locally constrained many-body systems, such as quantum dimer models and quantum loop models, especially their novel phases like topological orders and gapless quantum spin ice (QSI) phases. To discuss the possible phase diagram containing different QSIs in three-dimensional (3D) Rydberg arrays, we have constructed an extended Rokhsar-Kivelson (RK) Hamiltonian with equal weight superposition ground state in different fillings at the RK point. Therefore, the perfect QSIs with fixed local dimer filling and their monomer-doped states can be simulated directly by Monte Carlo sampling. Using single-mode approximation, the excitations of dimers and monomers have also been explored in different fillings. We find that, in the thermodynamical limit, even doping a small amount of monomers can disrupt the topological structure and lead to the existence of off-diagonal long-range order. However, in a finite size (as in cold-atom experiment), the property of QSI will be kept in a certain region like a crossover after doping. The phase diagram containing different QSIs and off-diagonal order phases is proposed.

cond-mat.quant-gas

Theory of rare-earth Kramers magnets on a Shastry-Sutherland lattice: dimer phases in presence of strong spin-orbit coupling

Shastry-Sutherland magnet is a typical frustrated spin system hosting rich phases. While the Heisenberg limit has been extensively studied, the role of spin-orbit coupling is not well explored. Motivated by newly discovered rare-earth Shastry-Sutherland magnets, we construct a generic effective-spin model that describes the interactions between Kramers doublet local moments on a Shastry-Sutherland lattice. Due to the strong spin-orbit coupling, the model takes the form of extended XYZ interactions on both intra- and inter-dimer bonds. We show that, in addition to the conventional "singlet" dimer phase, strong spin-orbit coupling can stabilize peculiar "triplet" dimer phases. These "triplet" dimer phases, though fully gapped, respond immediately to magnetic fields and evolve smoothly into the fully polarized phase. We present that the recently discovered Shastry-Sutherland magnet Yb$_2$Be$_2$GeO$_7$ belongs to the "triplet" dimer phase, and discuss the implication of our results to a broad class of quantum magnets in general.

cond-mat.str-el

Spin excitations of the Shastry-Sutherland model -- altermagnetism and deconfined quantum criticality

Frustrated quantum magnets can host a variety of exotic spin excitations, including fractionalized spin excitations coupled to emergent gauge fields at deconfined quantum critical points (DQCPs) and chiral magnons in altermagnets. Here, we investigate the spin excitation spectra of the highly frustrated $S=1/2$ antiferromagnetic (AFM) Shastry-Sutherland model, focusing on the evolution of low-energy collective modes from the N\'{e}el AFM phase to the plaquette valence bond solid (PVBS). We demonstrate that the AFM state exhibits altermagnetic behavior, characterized by a non-relativistic splitting between two chiral magnon bands. Furthermore, we identify two additional low-energy excitations: a Higgs mode in the longitudinal excitation channel and an $S=0$ excitation with vanishing spectral weight. As the system approaches the AFM-to-PVBS transition, both these modes soften along with the lowest-energy triplet and singlet modes in the PVBS state. The closing gap of the Higgs mode, combined with the nearly degenerate velocities of $S=1$ and $S=0$ excitations, provides spectral evidence that the AFM-to-PVBS transition is proximate to a DQCP with emergent $O(4)$ symmetry. Our results help clarify the spectral signature of a broad class of symmetry enhanced quantum phase transitions including deconfined quantum criticality.

cond-mat.str-el

Theory of magnetism for rare-earth magnets on the Shastry-Sutherland lattice with non-Kramers ions

Motivated by the rapid experimental progress on the rare-earth Shastry-Sutherland lattice magnets, we propose a generic effective spin model that describes interacting non-Kramers local moments on the Shastry-Sutherland lattice. We point out that the local moments consist of both magnetic dipole and quadrupole components and the effective model turns out to be an extended XYZ model with an intrinsic field that accounts for the crystal field splitting. We then study the ground-state phase diagram of the model and find that pure quadrupole orders, which are invisible to conventional experimental probes, can be stabilized over a broad regime. In particular, we show that a hidden ``1/3 magnetization plateau'' with quadrupole orders generally exists and discuss its experimental signatures. Finally, we discuss the relevance of our results to the rare-earth Shastry-Sutherland lattice magnets Pr$_{2}$Ga$_{2}$BeO$_{7}$ and Pr$_{2}$Be$_{2}$GeO$_{7}$.

cond-mat.str-el

Subsystem symmetries, critical Bose surface, and immobile excitations in an extended compass model

We propose an extended compass model that hosts subsystem symmetries and has potential experimental relevance with 3d transition metal compounds. The subsystem symmetries strongly constrain the mobility of spin excitations and lead to profound consequences. At the quantum critical point we find the presence of "critical Bose surface" along the entire $k_x$ and $k_y$ axis. Across which we find a nodal-line spin liquid that undergoes nematic instability at low temperatures. In the ferro-quadrupole phase, we find that one excitation is immobile individually analogous to "fractons".

cond-mat.str-el

Electron correlations and superconductivity in La$_3$Ni$_2$O$_7$ under pressure tuning

Motivated by the recent discovery of superconductivity in La$_3$Ni$_2$O$_7$ under pressure, we discuss the basic ingredients of a model that captures its microscopic physics under pressure tuning. We anchor our description in terms of the spectroscopic evidence of strong correlations in this system. In a bilayer Hubbard model including the Ni $3d$ $x^2-y^2$ and $z^2$ orbitals, we show the ground state of the model crosses over from a low-spin $S=1/2$ state to a high-spin $S=3/2$ state. In the high-spin state, the two $x^2-y^2$ and the bonding $z^2$ orbitals are all close to half-filling, which promotes a strong orbital selectivity in a broad crossover regime of the phase diagram pertinent to the system. Based on these results, we construct an effective multiorbital $t$-$J$ model to describe the superconductivity of the system, and find the leading pairing channel to be an intraorbital spin singlet with a competition between the extended $s$-wave and $d_{x^2-y^2}$ symmetries. Our results highlight the role of strong multiorbital correlation effects in driving the superconductivity of La$_3$Ni$_2$O$_7$.

cond-mat.supr-con

Emergent criticality in fully frustrated quantum magnets

Phase transitions in condensed matter are often linked to exotic emergent properties. We study the fully frustrated bilayer Heisenberg antiferromagnet to demonstrate that an applied magnetic field creates a novel emergent criticality. The quantum phase diagram contains four states, the DS (singlets on every interlayer dimer bond), DTAF (all triplets with antiferromagnetic order), TC (a singlet-triplet checkerboard) and FM (saturated ferromagnet). The thermal phase diagram is dominated by a wall of discontinuities extending from the zero-field DTAF-DS transition to a quantum critical endpoint where the field drives the DTAF and TC into the FM. This first-order wall is terminated at finite temperatures by a line of critical points, where the Berezinskii-Kosterlitz-Thouless (BKT) transition of the DTAF and the thermal Ising transition of the TC also terminate. We demonstrate by quantum Monte Carlo simulations that the BKT transition does not change the Ising nature of the DTAF-DS critical line. By contrast, the combination of symmetries merging on the multicritical DTAF-TC line leads to a 4-state Potts universality not contained in the microscopic Hamiltonian, which we associate with the Ashkin-Teller model. Our results represent a systematic step in understanding emergent phenomena in quantum magnetic materials including the ``Shastry-Sutherland compound'' SrCu$_2$(BO$_3$)$_2$.

cond-mat.str-el

Quantum Simulation of Two-Dimensional $\mathrm{U(1)}$ Gauge Theory in Rydberg and Rydberg-Dressed Atom Arrays

Simulating $\mathrm{U(1)}$ quantum gauge theories with spatial dimension greater than one is of great physical significance yet has not been achieved experimentally. Here we propose a simple realization of $\mathrm{U(1)}$ gauge theory on triangular lattice Rydberg atom arrays. Within experimentally accessible range, we find that the effective model well simulates various aspects of the $\mathrm{U(1)}$ gauge theory, such as emergence of topological sectors, incommensurability, and the deconfined Rokhsar-Kivelson point. Our proposal is easy to implement experimentally and exhibits pronounced quantum dynamics compared with previous proposals realizing $\mathrm{U(1)}$ and $\mathbb Z_2$ gauge theories.

quant-ph

Emergent Rokhsar-Kivelson point in realistic quantum Ising models

We show that the Rokhsar-Kivelson (RK) point in quantum dimer models (QDM) can emerge in realistic quantum Ising spin systems. Specifically, we investigate the $J_1$-$J_2$-$J_3$ transverse field Ising model on the triangular lattice with large-scale quantum Monte Carlo simulations. We find that the multicritical point in the phase diagram corresponds to the RK point of the QDM on the honeycomb lattice. We further measure the spectral functions and identify three branches of quadratic dispersions. In the phase diagram, we also find a sequence of incommensurate states, which meet the microscopic ingredients for the 'Cantor deconfinement' scenario. Our study provides a promising direction to realise the RK deconfinement in experimental platforms such as magnetic materials or programmable Rydberg arrays.

cond-mat.str-el

Field-Tuned Quantum Effects in a Triangular-Lattice Ising Magnet

We report thermodynamic and neutron scattering measurements of the triangular-lattice quantum Ising magnet TmMgGaO 4 in longitudinal magnetic fields. Our experiments reveal a quasi-plateau state induced by quantum fluctuations. This state exhibits an unconventional non-monotonic field and temperature dependence of the magnetic order and excitation gap. In the high field regime where the quantum fluctuations are largely suppressed, we observed a disordered state with coherent magnon-like excitations despite the suppression of the spin excitation intensity. Through detailed semi-classical calculations, we are able to understand these behaviors quantitatively from the subtle competition between quantum fluctuations and frustrated Ising interactions.

cond-mat.str-el

Magnetic field effects on the quantum spin liquid behaviors of NaYbS$_2$

Spin-orbit coupling is an important ingredient to regulate the many-body physics, especially for many spin liquid candidate materials such as rare-earth magnets and Kitaev materials. The rare-earth chalcogenides NaYbCh$_2$ (Ch = O, S, Se) is a congenital frustrating system to exhibit the intrinsic landmark of spin liquid by eliminating both the site disorders between Na$^{+}$ and Yb$^{3+}$ ions with the big ionic size difference and the Dzyaloshinskii-Moriya interaction with the perfect triangular lattice of the Yb$^{3+}$ ions. The temperature versus magnetic-field phase diagram is established by the magnetization, specific heat, and neutron-scattering measurements. Notably, the neutron diffraction spectra and the magnetization curve might provide microscopic evidence for a series of spin configuration for in-plane fields, which include the disordered spin liquid state, 120$^{o}$ antiferromagnet, and one-half magnetization state. Furthermore, the ground state is suggested to be a gapless spin liquid from inelastic neutron scattering, and the magnetic field adjusts the spin orbit coupling. Therefore, the strong spin-orbit coupling in the frustrated quantum magnet substantially enriches low-energy spin physics. This rare-earth family could offer a good platform for exploring the quantum spin liquid ground state and quantum magnetic transitions.

cond-mat.str-el

Topological phase transition between distinctWeyl semimetal states in MoTe2

We present experimental evidence of an intriguing phase transition between distinct topological states in the type-II Weyl semimetal MoTe2. We observe anomalies in the Raman phonon frequencies and linewidths as well as electronic quasielastic peaks around 70 K, which, together with structural, thermodynamic measurements, and electron-phonon coupling calculations, demonstrate a temperature-induced transition between two topological phases previously identified by contrasting spectroscopic measurements. An analysis of experimental data suggests electron-phonon coupling as the main driving mechanism for the change of key topological characters in the electronic structure of MoTe2.We also find the phase transition to be sensitive to sample conditions distinguished by synthesis methods. These discoveries of temperature and material condition-dependent topological phase evolutions and transitions in MoTe2 advance the fundamental understanding of the underlying physics and enable an effective approach to tuning Weyl semimetal states for technological applications.

cond-mat.mtrl-sci

Experimental identification of electric dipoles induced by magnetic monopoles in Tb2Ti2O7

The fundamental principles of electrodynamics allow an electron carrying both electric monopole (charge) and magnetic dipole (spin) but prohibit its magnetic counterpart. Recently it was predicted that the magnetic "monopoles" carrying emergent magnetic charges in spin ice systems can induce electric dipoles. The inspiring prediction offers a novel way to study magnetic monopole excitations and magnetoelectric coupling. However, no clear example has been identified up to now. Here, we report the experimental evidence for electric dipoles induced by magnetic monopoles in spin frustrated Tb2Ti2O7. The magnetic field applied to pyrochlore Tb2Ti2O7 along [111] direction, brings out a "3-in-1-out" magnetic monopole configuration, and then induces a subtle structural phase transition at Hc~2.3 T. The transition is evidenced by the non-linear phonon splitting under magnetic fields and the anomalous crystal-field excitations of Tb3+ ions. The observations consistently point to the displacement of the oxygen O" anions along [111] axis which gives rise to the formation of electric dipoles. The finding demonstrates that the scenario of magnetic monopole having both magnetic charge and electric dipole is realized in Tb2Ti2O7 and sheds light into the coupling between electricity and magnetism of magnetic monopoles in spin frustrated systems.

cond-mat.str-el

Anisotropic magnetic excitations of a frustrated bilinear-biquadratic spin model -- Implications for spin waves of detwinned iron pnictides

Elucidating the nature of spin excitations is important to understanding the mechanism of superconductivity in the iron pnictides. Motivated by recent inelastic neutron scattering measurements in the nearly 100% detwinned BaFe$_{2}$As$_{2}$, we study the spin dynamics of an $S=1$ frustrated bilinear-biquadratic Heisenberg model in the antiferromagnetic phase with wavevector $(\pi,0)$. The biquadratic interactions are treated in a dynamical way using a flavor-wave theory in an $SU(3)$ representation. Besides the magnon (dipolar) excitations, the biquadratic interactions give rise to quadrupolar excitations at high energies. We find that the quadrupolar wave significantly influences, in an energy dependent way, the anisotropy between the spin excitation spectra along the $(\pi,0)$ and $(0,\pi)$ directions in the wave vector space. Our theoretical results capture the essential behavior of the spin dynamics measured in the antiferromagnetic phase of the detwinned BaFe$_2$As$_2$. More generally, our results underscore the importance of electron correlation effects for the microscopic physics of the iron pnictides.

cond-mat.supr-con