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Daniel Shaffer

Publications and source records attributed to Daniel Shaffer.

At least 19 recordsLinked to original sources

Kinetic Lifshitz invariants and dynamics of nonreciprocal fluctuations in superconductors

We derive the generalized time-dependent Ginzburg-Landau theory of a disordered noncentrosymmetric superconductor from the Keldysh nonlinear sigma model, using a two-dimensional electron gas with Rashba spin-orbit coupling and an in-plane Zeeman field as a minimal model. On the thermodynamic side we construct the Lifshitz invariants of the free energy, the linear and cubic gradient terms and the momentum-odd part of the quartic vertex, and trace their dependence on disorder. These couplings are governed by a single closed-form kernel controlled by the ratio of the Dyakonov-Perel spin-relaxation rate to temperature, interpolating between the weak-relaxation regime, where the invariants are suppressed, and the relaxation-dominated regime, where the helical modulation of the order parameter saturates at a universal, disorder-independent value. This crossover reconciles conflicting results for the magnetoelectric couplings of dirty Rashba superconductors. Because the theory is formulated on the Keldysh contour, it also determines the dissipative dynamics: the relaxation rate of a fluctuation with pair momentum $\mathbf{q}$, and hence, by the fluctuation-dissipation theorem, the Langevin noise power, acquires a term odd in $\mathbf{q}$ and odd in the magnetic field. The structure of this kinetic Lifshitz invariant is dictated by Onsager reciprocity: friction and noise renormalize in lockstep, so equal-time fluctuations remain Gibbsian while the dynamics are nonreciprocal. As applications we compute the superconducting diode efficiency near $T_c$, where the cubic invariant competes with the quartic vertex and with even higher-gradient terms rendered odd by the helical shift, reversing the sign of the diode coefficient, and the fluctuation-induced magnetochiral anisotropy above $T_c$, where the current-resolved nonreciprocal resistance forms a plateau across the Gaussian regime.

cond-mat.supr-con

Metamagnetism in UTe2: the roles of itinerancy and localization

The metamagnetic transition in UTe$_2$ plays a key role in stabilizing two enigmatic field-induced superconducting phases. One of these phases (SC2) is truncated by the transition, lying directly below it, while the other (SC3) sits predominantly above it and appears to be stabilized because of it. While numerous pulsed field studies have examined this transition, comparatively few steady field experiments have investigated it. Here we report a suite of measurements of metamgnetism in UTe$_2$, at ambient pressure by torque magnetometry and extraction magnetometry techniques, and of the magnetoconductance under pressure. Our steady field measurements resolve a complex sub-structure within the transition, with separate features that possess different temperature evolutions, pointing to distinct contributions from itinerant and localized moments. The itinerant contribution might relate to a possible spin-density wave state. We theoretically model the evolution of Kondo and RKKY interactions and propose that the SC2 state is stabilized under pressure due to the collapse of magnetic anisotropy, leading to an enhancement of longitudinal spin fluctuations along the hard $b$ axis, which are pair-forming in the $p$-wave channel.

cond-mat.str-el

Fluctuation-Induced Magnetoelectric Effect in Noncentrosymmetric Superconductors

We study the effect of superconducting fluctuations on the spin susceptibility and NMR relaxation rate in noncentrosymmetric two-dimensional materials above the superconducting transition temperature, considering arbitrary strength of impurity scattering. Employing a microscopic model with linear Rashba spin-orbit coupling, we show that superconducting fluctuations give rise to a direct contribution to the spin susceptibility through fluctuation-induced Cooper pairs. This fluctuation-driven magnetoelectric effect is possible even for purely $s$-wave singlet pairing, a mechanism that is forbidden in centrosymmetric systems. It competes with the reduction of the susceptibility below the Pauli value arising from the combined effects of the suppression of the density of states and quantum-interference localization processes. In contrast, superconducting fluctuations enhance the NMR relaxation rate above its normal-state Korringa value, with spin-orbit coupling providing an additional amplification of this effect.

cond-mat.supr-con

Superconductivity near two-dimensional Van Hove singularities: a determinant quantum Monte Carlo study

The superconducting transition temperature $T_c$ of the two-dimensional attractive Hubbard model is computed in the vicinity of both ordinary (logarithmic) and higher-order (power-law) Van Hove singularities using determinant quantum Monte Carlo simulations. For interaction strengths $|U| \lesssim W/3$, where $W$ is the electronic bandwidth, $T_c$ is enhanced in the neighborhood of the Van Hove point, albeit more weakly than expected from weak-coupling BCS theory. Enhancing the Van Hove singularity from logarithmic to power-law yields only a minor additional enhancement of $T_c$. For $|U| \gtrsim W/3$, the maximum $T_c$ shifts away from the Van Hove point and instead occurs at a density unrelated to any features in the non-interacting density of states, consistent with a strong-coupling interpretation. We find that the maximal $T_c$ in the model is achieved at intermediate $U$ and at a density away from the Van Hove point.

cond-mat.str-el

Electrically-controllable superconducting memory effect in UTe2

If a computer could be assembled from superconducting components, the energy efficiency would far surpass that of conventional electronics. Historic research efforts towards this goal yielded pivotal breakthroughs in the development and discovery of scanning tunnelling microscopy and high temperature superconductivity. Although recent strides have been taken in advancing superconducting diode and switching technologies, harnessing read/writeable memory functionality in superconducting platforms has remained challenging. Here we show that bulk single crystal specimens of the triplet superconductor candidate uranium ditelluride (UTe$_2$) possess such properties. Upon applying a magnetic field to access an intermediate regime straddling two distinct superconducting phases, we find that direct current pulses can push the material in and out of a metastable state possessing an enhanced critical current $J_c$. This switching is controllable by the strength and duration of the stimuli, with the system `remembering' whether it is in the high or low $J_c$ state for extended periods. We interpret this to be due to competition between two distinct vortex species, which can be perturbatively pushed into a non-equilibrium high-disorder configuration with stronger pinning forces and thus higher $J_c$. Rather than requiring proximate magnetic or semiconducting interfaces, this memory functionality appears to be an intrinsic property of UTe$_2$ rooted in the superconducting order itself. Our findings underscore the rich complexity of quantum vortex matter, and demonstrate the viability of engineering a new class of superconducting memory elements with ultralow-power switching.

cond-mat.supr-con

Theories of Superconducting Diode Effects

Superconducting diode effects (SDE), both in bulk superconductors and in Josephson junctions, have garnered a lot of attention due to potential applications in classical and quantum computing, as well as superconducting sensors. Here we review various mechanisms that have been theoretically proposed for their realization. We first provide a brief historical overview and discuss the basic but subtle phenomenological Ginzburg-Landau theory of SDE, emphasizing the need to the simultaneous breaking of time-reversal and inversion symmetries. We then proceed to more microscopic treatments, focusing especially on implementations in noncentrosymmetric materials described by the Rashba-Zeeman model. Finally, we review proposals based on other condensed matter systems such as altermagnets, valley polarized and topological materials, and systems out of equilibrium.

cond-mat.supr-con

Helical phases and Bogoliubov Fermi surfaces probed by superconducting diode effects

Noncentrosymmetric superconductors (NCSs) with Rashba spin-orbit coupling (SOC) and in-plane magnetic fields have emerged as natural platforms for realizing both the bulk superconducting diode effect (SDE) and the Josephson diode effect (JDE) - phenomena characterized by unequal critical currents in opposite directions due to the simultaneous breaking of time-reversal and inversion symmetries. Using the quasiclassical Eilenberger formalism, we systematically investigate both the bulk SDE and the JDE in a clean NCS with Rashba SOC and in-plane magnetic fields. For the bulk system, we find that the diode efficiency can nominally approach its maximal value at the critical endpoint of the first-order Lifshitz transition between weak and strong helical phases featuring finite-momentum Cooper pairs, the latter marked by the emergence of Bogolyubov Fermi surfaces (BFSs). In a Josephson junction, we show that finite-momentum pairing in the superconducting leads is the dominant mechanism behind the JDE in short junctions, whereas in long junctions it is primarily governed by the Zeeman field in the normal region. In the long-junction regime, the diode efficiency additionally oscillates between positive and negative values as a function of magnetic field at low fields, providing a route toward a highly tunable Josephson diode. At higher fields, the onset of BFSs in the strong helical phase leads to a sharp suppression of both the JDE and the Josephson current when the current direction is aligned with momenta along the BFS, resulting in strong anisotropy. We propose that this anisotropy in the Josephson current offers an alternative method for detecting BFSs, applicable to systems with or without a JDE.

cond-mat.supr-con

Josephson Diode Effect from Nonequilibrium Current in a Superconducting Interferometer

We investigate the Josephson diode effect in a superconducting interferometer under nonequilibrium conditions. In contrast to its thermodynamic counterpart, which requires the simultaneous breaking of time-reversal and inversion symmetry, we demonstrate that a diode-like asymmetry of the critical current can emerge solely due to a dissipative current in the normal region of an otherwise symmetric Josephson junction. This effect is driven entirely by the nonequilibrium conditions, without the need for additional inversion symmetry breaking. Using the standard quasiclassical Keldysh Green's function formalism, we explicitly calculate the diode coefficient from the supercurrent-phase relation of the interferometer. Remarkably, within certain ranges of control parameters, such as applied voltage, temperature, and the geometric aspect ratio of the device, the diode coefficient can exceed its nominal perfect value.

cond-mat.supr-con

Metamagnetic ripples in the UTe2 high magnetic field phase diagram

The heavy fermion metamagnet uranium ditelluride possesses two distinct magnetic field--induced superconducting states. One of these superconductive phases resides at magnetic fields immediately below a first-order metamagnetic transition to a field--polarized paramagnetic state at a field strength $H_m$, while the other exists predominantly above $H_m$. However, little is known about the microscopic properties of this polarized paramagnetic state. Here we report pulsed magnetic field measurements tracking the evolution of $H_m$ for polar and azimuthal inclinations in the vicinity of the crystallographic $b-a$ plane. We uncover a region of the phase diagram at high fields $>$ 50 T with a ripple-like non-monotonic dependence of $H_m$ on the orientation of field. Within this ripple in the metamagnetic transition surface, $H_m$ exhibits an anomalous temperature dependence. Our results point towards the presence of complex magnetic interactions and possible magnetic sub-phases at high magnetic fields in UTe$_2$, which may have important implications for the manifestation of exotic field-induced superconductivity.

cond-mat.str-el

Superconducting diode efficiency from singlet-triplet mixing in disordered systems

The superconducting diode effect (SDE) -- the nonreciprocity of the critical current in a bulk superconductor -- has garnered significant attention due to its potential applications in superconducting electronics. However, the role of disorder scattering in SDE has rarely been considered, despite its potential qualitative impact, as we demonstrate in this work. We investigate SDE in a disordered Rashba superconductor under an in-plane magnetic field, employing a self-consistent Born approximation to derive the corresponding Ginzburg-Landau theory. Our analysis reveals two surprising effects. First, in the weak Rashba spin-orbit coupling (SOC) regime, disorder can reverse the direction of the diode effect, indicated by a sign change in the superconducting diode efficiency coefficient. Second, in the strong Rashba SOC regime, disorder becomes the driving mechanism of SDE, which vanishes in its absence. In this case, we show that disorder-induced mixing of singlet and triplet superconducting orders underlies the effect.

cond-mat.supr-con

Superconducting Diode Effect in Multiphase Superconductors

We identify a new mechanism for the intrinsic superconducting diode effect (SDE) in multiphase superconductors. Using a Ginzburg-Landau and a microscopic two-band model, we find phase transitions into a mixed phase with finite-momentum Cooper pairs and SDE with high (including maximal) diode efficiencies, despite the individual phases exhibiting no SDE and equal inversion parity. We thus show that parity mixing $-$ invoked in previous proposals $-$ is not a crucial ingredient for SDE. The new mechanism may be relevant in a multitude of known multiphase superconductors like UTe$_2$.

cond-mat.supr-con

Supercurrent Diode Effect in Helical Superconductors

In this work, we explore the generalities of the supercurrent diode effect. As an illustrative example, we examine a model of a two-dimensional superconductor with Rashba-type spin-orbit coupling under an in-plane magnetic field and in the clean limit, which realizes a helical phase. First, we utilize Ginzburg-Landau phenomenology to derive a general formula for the diode efficiency. This is achieved by incorporating higher gradient terms in the Lifshitz invariants, which are responsible for the nonreciprocal superflow. Subsequently, we validate these results through microscopic diagrammatic computation and further estimate correction terms arising from interband pairing correlations. We provide a detailed comparison to prior investigations of this problem conducted within the framework of the quasiclassical approximation based on the Eilenberger equation.

cond-mat.supr-con

Time-Reversal Invariant Topological Moir\'e Flatband: A Platform for the Fractional Quantum Spin Hall Effect

Motivated by recent observation of the quantum spin Hall effect in monolayer germanene and twisted bilayer transition-metal-dichalcogenides (TMDs), we study the topological phases of moir\'e twisted bilayers with time-reversal symmetry and spin $s_z$ conservation. By using a continuum model description which can be applied to both germanene and TMD bilayers, we show that at small twist angles, the emergent moir\'e flatbands can be topologically nontrivial due to inversion symmetry breaking. Each of these flatbands for each spin projection admits a lowest-Landau-level description in the chiral limit and at magic twist angle. This allows for the construction of a many-body Laughlin state with time-reversal symmetry which can be stabilized by a short-range pseudopotential, and therefore serves as an ideal platform for realizing the so-far elusive fractional quantum spin Hall effect with emergent spin-1/2 U(1) symmetry.

cond-mat.mes-hall

Entanglement and Topology in Su-Schrieffer-Heeger Cavity Quantum Electrodynamics

Cavity materials are a frontier to investigate the role of light-matter interactions on the properties of electronic phases of matter. In this work, we raise a fundamental question: can non-local interactions mediated by cavity photons destabilize a topological electronic phase? We investigate this question by characterizing entanglement, energy spectrum and correlation functions of the topological Su-Schrieffer-Heeger (SSH) chain interacting with an optical cavity mode. Employing density-matrix renormalization group (DMRG) and exact diagonalization (ED), we demonstrate the stability of the edge state and establish an area law scaling for the ground state entanglement entropy, despite long-range correlations induced by light-matter interactions. These features are linked to gauge invariance and the scaling of virtual photon excitations entangled with matter, effectively computed in a low-dimensional Krylov subspace of the full Hilbert space. This work provides a framework for characterizing novel equilibrium phenomena in topological cavity materials.

cond-mat.str-el

Quantum Fractality on the Surface of Topological Insulators

Three-dimensional topological insulators support gapless Dirac fermion surface states whose rich topological properties result from the interplay of symmetries and dimensionality. Their topological properties have been extensively studied in systems of integer spatial dimension but the prospect of these surface electrons arranging into structures of non-integer dimension like fractals remains unexplored. In this work, we investigate a new class of states arising from the coupling of surface Dirac fermions to a time-reversal symmetric fractal potential, which breaks translation symmetry while retaining self-similarity. Employing large-scale exact diagonalization, scaling analysis of the inverse participation ratio, and the box-counting method, we establish the onset of self-similar Dirac fermions with fractal dimension for a symmetry-preserving surface potential with the geometry of a Sierpinski carpet fractal with fractal dimension $D \approx 1.89$. Dirac fractal surface states open a fruitful avenue to explore exotic regimes of transport and quantum information storage in topological systems with fractal dimensionality.

cond-mat.mes-hall

Emergence of Chern Supermetal and Pair-Density Wave through Higher-Order Van Hove Singularities in the Haldane-Hubbard Model

While advances in electronic band theory have brought to light new topological systems, understanding the interplay of band topology and electronic interactions remains a frontier question. In this work, we predict new interacting electronic orders emerging near higher-order Van Hove singularities present in the Chern bands of the Haldane model. We classify the nature of such singularities and employ unbiased renormalization group methods that unveil a complex landscape of electronic orders, which include ferromagnetism, density-waves and superconductivity. Importantly, we show that repulsive interactions can stabilize long-sought pair-density wave state and an exotic Chern supermetal, which is a new class of non-Fermi liquid with anomalous quantum Hall response. This framework opens a new path to explore unconventional electronic phases in two-dimensional chiral bands through the interplay of band topology and higher-order Van Hove singularities.

cond-mat.str-el

Triplet Pair-Density Wave Superconductivity on the $\pi$-flux Square Lattice

Pair-density waves (PDW) are superconducting states that spontaneously break translation symmetry in systems with time-reversal symmetry (TRS). Evidence for PDW has been seen in several recent experiments, as well as in the pseudogap regime in cuprates. Theoretical understanding of PDW has been largely restricted to phenomenological and numerical studies, while microscopic theories typically require strong-coupling or fine-tuning. In this work, we provide a novel symmetry-based mechanism under which PDW emerges as a weak coupling instability of a 2D TRS metal. Combining mean-field and renormalization group analyses, we identify a weak-coupling instability towards a triplet PDW realized in the $\pi$-flux square lattice model with on-site repulsion and moderate nearest-neighbor attraction when the Fermi level crosses Van Hove singularities at 1/4 and 3/4 fillings. This PDW is protected by the magnetic translation symmetries characteristic of Hofstadter systems, of which the $\pi$-flux lattice is a special time-reversal symmetric case.

cond-mat.supr-con

Weak-Coupling Theory of Pair Density-Wave Instabilities in Transition Metal Dichalcogenides

The possibility of realizing pair density wave (PDW) phases, in which Cooper pairs have a finite momentum, presents an interesting challenge that has been studied in a wide variety of systems. In conventional superconductors, this is only possible when external fields lift the spin degeneracy of the Fermi surface, leading to pair formation at an incommensurate momentum. Here, we study a second possibility, potentially relevant to transition metal dichalcogenides, in which the Fermi surface consists of a pair of pockets centered at the $\pm K$ points of the Brillouin zone as well as a central pocket at the $\Gamma$ point. In the limit where these three pockets are identical, the pairing susceptibility has a logarithmic divergence at the non-zero wave-vectors $\pm \mathbf{K}$, allowing for a weak-coupling analysis of the PDW instability. We find that repulsive electronic interactions combine to yield effective attractive interactions in the singlet and triplet PDW channels, as long as the $\Gamma$ pocket is present. Because these PDW channels decouple from the uniform superconducting channel, they can become the leading unconventional pairing instability of the system. Upon solving the linearized gap equations, we find that the PDW instability is robust against small trigonal warping of the $\pm K$ pockets and small detuning between the $\Gamma$ and $\pm K$ pockets, which affect the PDW transition in a similar way as the Zeeman magnetic field affects the uniform superconducting transition. We also derive the Ginzburg-Landau free energy for the PDW gaps with momenta $\pm \mathbf{K}$, analyzing the conditions for and consequences of the emergence of FF-type and LO-type PDW ground states. Our classification of the induced orders in each ground state reveals unusual phases, including an odd-frequency charge-$2e$ superconductor in the LO-type PDW.

cond-mat.supr-con