arXiv subjects

Deepak Dhariwal

Publications and source records attributed to Deepak Dhariwal.

3 recordsLinked to original sources

arXiv2026

Modeling Dynamic Magnetic Response of Spinel Soft Ferrites with the Steepest-Entropy-Ascent Quantum Thermodynamics Formalism

Selecting soft ferrites for alternating-field applications requires balancing magnetic response, dissipation, nonlinearity, and heating. We use a field-driven steepest-entropy-ascent quantum thermodynamic (SEAQT) model to compare the electron, phonon, and magnon responses of Fe$_3$O$_4$, MnFe$2$O$4$, and (Mn${0.5}$Zn${0.5}$)Fe$_2$O$_4$ within a common first-principles framework. The model treats spatially uniform longitudinal relaxation and neglects domain-wall motion, transverse rotation, resonance, eddy-current effects, and heat removal. We use $τ_e=0.05$ ps and $τ_p=3$ ps for all three materials, with effective longitudinal magnon relaxation times of 500, 200, and 85 ps, respectively; these literature-motivated values are model inputs, not fits to measured losses. Within this framework, the Mn--Zn ferrite gives the largest peak longitudinal magnetization change, retains its response best at high frequency, and shows the largest work per cycle and peak-to-peak magnon temperature change, whereas MnFe$_2$O$_4$ gives the largest normalized $χ''$ peak. Thus, no single ferrite ranks highest across all metrics: the preferred material depends on the property, frequency, field amplitude, and cation configuration of interest. The model therefore provides a spectrum- and kinetics-resolved screening tool for engineering comparison of ferrites rather than a prediction of total core loss.

cond-mat.mtrl-sci↗

arXiv2026

Field-Driven Coupled Magnon--Phonon--Electron Relaxation in Magnetite Using Steepest-Entropy-Ascent Quantum Thermodynamic Formalism

A field-driven steepest-entropy-ascent quantum thermodynamic (SEAQT) formulation is developed for longitudinal nonequilibrium relaxation in magnetite (Fe$_3$O$_4$) with coupled electron, phonon, and magnon populations. Material-specific excitation spectra define the thermodynamic state space, while one relaxation parameter for each population sets its kinetic scale. A longitudinal magnetic field shifts the dressed magnon eigenenergies while the occupation basis remains fixed; irreversible redistribution conserves instantaneous energy and electron number while allowing the magnon population to vary. The formulation yields nonequilibrium subsystem temperatures, entropy production, magnetic-work identities, and a coupled small-signal susceptibility incorporating energy-conservation feedback among all three populations; the one-pole Debye response appears only as a limiting case. Numerical results under sinusoidal driving show a transition from nearly quasistatic behavior to frequency-dependent lag, finite-amplitude departure from the linear-response ellipse, and increasing higher-harmonic content. Relaxational work per cycle increases strongly with field amplitude and frequency, while the complex susceptibility is broader and shifted relative to a Debye reference. Entropy production remains positive, and the electron, phonon, and magnon temperatures show distinct excursions followed by secular heating when positive magnetic work is retained without heat rejection. The calculated work represents longitudinal magnon quasiparticle relaxation in a homogeneous single-domain model, not the total core loss of a finite ferrite specimen.

cond-mat.mtrl-sci↗

arXiv2026

Energy Eigenstates of Electrons, Magnons and Phonons in Fe$_3$O$_4$ (magnetite), MnFe$_2$O$_4$ (jacobsite), and mixed Mn-Zn ferrites

We report first-principles calculations of the electronic structure, magnon excitations, and phonons in magnetite (Fe$_3$O$_4$), jacobsite (MnFe$_2$O$_4$), and mixed manganese-zinc ferrites (Mn$_{x}$,Zn$_{1-x}$)Fe$_2$O$_4$ for representative compositions ($0\le x \le 1$) and A/B-site cation arrangements. Electronic structures are computed using density functional theory (DFT) augmented by rotationally invariant DFT+U+J, with on-site Hubbard and Hund's parameters, $U$ and $J$, respectively, determined self-consistently by spin-polarized linear-response perturbations of the chosen correlated subspaces (including, where applied, the ligand $2p$ subspace). A classical Heisenberg spin Hamiltonian is parameterized by mapping DFT+U+J total energies for multiple collinear spin configurations onto nearest-neighbor exchange couplings, which are then used to obtain magnon dispersions and magnon densities of states within linear spin-wave theory. Phonon spectra and densities of states are obtained from finite-displacement force constants and dynamical matrices computed on the same DFT+U+J-relaxed structures. Overall, the workflow provides a consistent, composition- and configuration-aware route to electronic, vibrational, and magnetic excitation spectra across the Mn/Zn ferrite space.

cond-mat.mtrl-sci↗