arXiv subjects

Dimitri Roditchev

Publications and source records attributed to Dimitri Roditchev.

At least 19 recordsLinked to original sources

arXiv2026

Surface reconstruction-driven band folding and spin-orbit enhancement at the $\alpha$-antimonene/Au(111) interface

The electronic properties of the two-dimensional (2D) $\alpha$ phase of antimonene are unique, featuring unpinned Dirac cones that can be moved with strain. Here we investigate the structural and electronic properties of an epitaxial 2D $\alpha$-antimonene, grown on Au(111). Using angle-resolved photoemission spectroscopy and density-functional theory, we reveal a strong hybridization at the Sb/Au interface, which imprints a rectangular reconstruction in the Au states, producing a band folding and hybrid bands exhibiting trigonal pockets. Additionally, hybridization displaces part of the Au wavefunction in regions of large electrostatic potential gradient, thereby enhancing spin-orbit splitting. Our work underscores that the pristine electronic properties of $\alpha$-antimonene may be deeply modified by its substrate, and even overwhelmed by the bands of the latter, and also shows that spin-orbit interaction in a heavy metal (Au) can be substantially enhanced by a lighter element (Sb).

cond-mat.mtrl-sci↗

arXiv2025

Nernst effect and its thickness dependence in superconducting NbN films

Superconducting thin films and layered crystals display a Nernst signal generated by short-lived Cooper pairs above their critical temperature. Several experimental studies have broadly verified the standard theory invoking Gaussian fluctuations of a two-dimensional superconducting order parameter. Here, we present a study of the Nernst effect in granular NbN thin films with a thickness varying from 4 to 30 nm, exceeding the short superconducting coherence length and putting the system in the three-dimensional limit. We find that the Nernst conductivity decreases linearly with reduced temperature ($\alpha_{xy}\propto \frac{T-T_c}{T_c}$), but the amplitude of $\alpha_{xy}$ scales with thickness. While the temperature dependence corresponds to what is expected in a 2D picture, scaling with thickness corresponds to a 3D picture. We argue that this behavior indicates a 2+1D situation, in which the relevant coherence length along the thickness of the film has no temperature dependence. We find no visible discontinuity in the temperature dependence of the Nernst conductivity across T$_c$. Explaining how the response of the superconducting vortices evolves to the one above the critical temperature of short-lived Cooper pairs emerges as a challenge to the theory.

cond-mat.supr-con↗

arXiv2024

Scanning quantum vortex microscopy reveals thickness-dependent pinning nano-network in superconducting Nb-films

The presence of quantum vortices determines the electromagnetic response of superconducting materials and devices. Controlling the vortex motion, their pinning on intrinsic and artificial defects is therefore essential for superconducting electronics. Here we take advantage of the attractive force between a magnetic cantilever of the Magnetic Force Microscope and a single quantum vortex to spatially map the pinning force inside 50-240 nm thick magnetron-sputtered Nb-films, commonly used in advanced superconducting electronics. The revealed pinning nano-network is related to the thickness-dependent granular structure of the films as well as to the characteristic microscopic scales of superconductivity. Our approach is general, and can be directly applied to other type II granular superconducting materials and nanodevices.

cond-mat.supr-con↗

arXiv2023

Anomalous microwave response in the dissipative regime of topological superconducting devices based on Bi2Te2.3Se0.7

Superconducting proximity junctions based on topological insulators are widely believed to harbor Majorana-like bound states. The latter serves as a paradigm non-local topological quantum computation protocols. Nowadays, a search for topological phases in different materials, perspective for a realization of topological qubits, is one of the central efforts in quantum physics. It is motivated, in particular, by recent observation of anomalous ac Josephson effect, which being a signature of Majorana physics. Its manifestations, such as a fractional Josephson frequency and the absence of the first (or several odd in more rare cases), Shapiro steps, were reported for different materials. Here we study Shapiro steps in Nb/Bi2Te2.3Se0.7/Nb junctions, based on ultrasmall single crystals of a 3D topological insulator synthesized by a physical vapor deposition (PVD) technique. We present evidence that our junctions are ballistic. When subjected to microwave radiation, the junctions exhibit Shapiro steps, but the first step is missing. Typically it is assumed that the missing first step (MFS) effect cannot be observed in the presence of quasiparticle poisoning due to suppression of the 4{\pi}-periodic component. Our findings within the context of the RSJ-model of Josephson junction dynamics show that such behaviour of samples corresponds to a specific condition, requiring a minimum of 5% of the 4{\pi}-component for disappearance of the first Shapiro step.

cond-mat.supr-con↗

arXiv2023

Josephson vortex-based memory

Josephson junctions are currently used as base elements of superconducting logic systems. Long enough junctions subject to magnetic field host quantum phase 2{\pi}-singularities - Josephson vortices. Here we report the realization of the superconducting memory whose state is encoded by the number of present Josephson vortices. By integrating the junction into a coplanar resonator and by applying a microwave excitation well below the critical current, we were able to control the state of the memory in an energy-efficent and non-destructive manner. The performance of the device is evaluated, and the routes for creating scalable cryogenic memories directly compatible with superconducting microwave technologies are discussed.

cond-mat.supr-con↗

arXiv2023

Dynamic metastable vortex states in interacting vortex lines

The electron transport in current-biased superconducting nano-bridges is determined by the motion of the quantum vortex confined in the internal disorder landscape. Here we consider a simple case of a single or two neighbouring linear defects crossing a nano-bridge. The strong anharmonicity of the vortex motion along the defect leads, upon RF-excitation, to fractional Shapiro steps. In the case of two defects, the vortex motion becomes correlated, characterized by metastable states that can be locked to a resonant RF-drive. The lock-unlock process causes sudden voltage jumps and drops in the voltage-current characteristics observed in experiments. We analyze the parameters promoting these metastable dynamic states and discuss their potential applications in quantum devices.

cond-mat.supr-con↗

arXiv2023

STM observation of the hinge-states of bismuth nanocrystals

The recent application of topological quantum chemistry to rhombohedral bismuth established the non-trivial band structure of this material. This is a 2$^{nd}$order topological insulator characterized by the presence of topology-imposed hinge-states. The spatial distribution of hinge-states and the possible presence of additional symmetry-protected surface-states is expected to depend on the crystal shape and symmetries. To explore this issue, we have grown bismuth nanocrystals in the tens of nanometers on the $(110)$ surface of InAs. By scanning tunneling spectroscopy, we mapped the local density of states on all facets and identified the presence of the hinge-states at the intersection of all facets. Our study confirm the classification of bulk bismuth as a 2$^{nd}$order topological insulator. We propose that the ubiquitous presence of the hinge-states result from their tunnel-coupling across the nanometer-sized facets.

cond-mat.mes-hall↗

arXiv2023

Manipulation of the magnetic state of a porphyrin-based molecule on gold: From Kondo to quantum nanomagnet via the charge fluctuation regime

By moving individual Fe-Porphyrin-based molecules with the tip of Scanning Tunneling Microscope in the vicinity of a Br-atom containing elbow of the herringbone-reconstructed Au(111), we reversibly and continuously control their magnetic state. Several regimes are obtained experimentally and explored theoretically: from the integer spin limit, through intermediate magnetic states with renormalized magnetic anisotropy, until the Kondo-screened regime, corresponding to a progressive increase of charge fluctuations and mixed valency due to an increase in the interaction of the molecular Fe states with the substrate Fermi sea. Our results open a route for the realization, tuning and experimental studies of novel quantum magnetic states in molecule-surface hybrids.

cond-mat.mes-hall↗

arXiv2022

Revealing Josephson vortex dynamics in proximity junctions below critical current

Made of a thin non-superconducting metal (N) sandwiched by two superconductors (S), SNS Josephson junctions enable novel quantum functionalities by mixing up the intrinsic electronic properties of N with the superconducting correlations induced from S by proximity. Electronic properties of these devices are governed by Andreev quasiparticles [1] which are absent in conventional SIS junctions whose insulating barrier (I) between the two S electrodes owns no electronic states. Here we focus on the Josephson vortex (JV) motion inside Nb-Cu-Nb proximity junctions subject to electric currents and magnetic fields. The results of local (Magnetic Force Microscopy) and global (transport) experiments provided simultaneously are compared with our numerical model, revealing the existence of several distinct dynamic regimes of the JV motion. One of them, identified as a fast hysteretic entry/escape below the critical value of Josephson current, is analyzed and suggested for low-dissipative logic and memory elements.

cond-mat.supr-con↗

arXiv2021

Lateral Josephson Junctions as Sensors for Magnetic Microscopy at Nano-Scale

Lateral Josephson junctions (LJJ) made of two superconducting Nb electrodes coupled by Cu-film are applied to quantify the stray magnetic field of Co-coated cantilevers used in Magnetic Force Microscopy (MFM). The interaction of the magnetic cantilever with LJJ is reflected in the electronic response of LJJ as well as in the phase shift of cantilever oscillations, simultaneously measured. The phenomenon is theorized and used to establish the spatial map of the stray field. Based on our findings, we suggest integrating LJJs directly on the tips of cantilevers and using them as nano-sensors of local magnetic fields in Scanning Probe Microscopes. Such probes are less invasive than conventional magnetic MFM cantilevers and simpler to realize than SQUID-on-tip sensors.

cond-mat.supr-con↗

arXiv2020

How to induce superconductivity in epitaxial graphene $via$ remote proximity effect through an intercalated gold layer

Graphene holds promises for exploring exotic superconductivity with Dirac-like fermions. Making graphene a superconductor at large scales is however a long-lasting challenge. A possible solution relies on epitaxially-grown graphene, using a superconducting substrate. Such substrates are scarce, and usually destroy the Dirac character of the electronic band structure. Using electron diffraction (reflection high-energy, and low-energy), scanning tunneling microscopy and spectroscopy, atomic force microscopy, angle-resolved photoemission spectroscopy, Raman spectroscopy, and density functional theory calculations, we introduce a strategy to induce superconductivity in epitaxial graphene $via$ a remote proximity effect, from the rhenium substrate through an intercalated gold layer. Weak graphene-Au interaction, contrasting with the strong undesired graphene-Re interaction, is demonstrated by a reduced graphene corrugation, an increased distance between graphene and the underlying metal, a linear electronic dispersion and a characteristic vibrational signature, both latter features revealing also a slight $p$ doping of graphene. We also reveal that the main shortcoming of the intercalation approach to proximity superconductivity is the creation of a high density of point defects in graphene (10$^{14}$~cm$^{-2}$). Finally, we demonstrate remote proximity superconductivity in graphene/Au/Re(0001), at low temperature.

cond-mat.supr-con↗

arXiv2018

Isolated pairs of Majorana zero modes in a disordered superconducting lead monolayer

Majorana zero modes are fractional quantum excitations appearing in pairs, each pair being a building block for quantum computation . Some possible signatures of these excitations have been reported as zero bias peaks at endpoints of one-dimensional semiconducting wires and magnetic chains. However, 1D systems are by nature fragile to a small amount of disorder that induces low-energy excitations, hence obtaining Majorana zero modes well isolated in a hard gap requires extremely clean systems. Two-dimensional systems offer an alternative route to get robust Majorana zero modes. Indeed, it was shown recently that Pb/Co/Si(111) could be used as a platform for generating 2D topological superconductivity with a strong immunity to local disorder. While 2D systems exhibit dispersive chiral edge states, they can also host Majorana zero modes located on local topological defects. According to predictions, if an odd number of zero modes are located in a topological domain an additional zero mode should appear all around the domain's edge. Here we use scanning tunneling spectroscopy to characterize a disordered superconducting monolayer of Pb coupled to underlying Co-Si magnetic islands meant to induce a topological transition. We show that pairs of zero modes are stabilized: one zero mode positioned at a point in the middle of the magnetic domain and its zero mode partner extended all around the domain. The zero mode pair is remarkably robust, it is isolated within a hard superconducting energy gap and it appears totally immune to the strong disorder present in the Pb monolayer. Our theoretical scenario supports the protected Majorana nature of this zero mode pair, highlighting the role of magnetic or spin-orbit coupling textures. This robust pair of Majorana zero modes offers a new platform for theoretical and experimental study of quantum computing.

cond-mat.supr-con↗

arXiv2018

Quantum confinement effects in Pb Nanocrystals grown on InAs

In the recent work of Ref.\cite{Vlaic2017-bs}, it has been shown that Pb nanocrystals grown on the electron accumulation layer at the (110) surface of InAs are in the regime of Coulomb blockade. This enabled the first scanning tunneling spectroscopy study of the superconducting parity effect across the Anderson limit. The nature of the tunnel barrier between the nanocrystals and the substrate has been attributed to a quantum constriction of the electronic wave-function at the interface due to the large Fermi wavelength of the electron accumulation layer in InAs. In this manuscript, we detail and review the arguments leading to this conclusion. Furthermore, we show that, thanks to this highly clean tunnel barrier, this system is remarkably suited for the study of discrete electronic levels induced by quantum confinement effects in the Pb nanocrystals. We identified three distinct regimes of quantum confinement. For the largest nanocrystals, quantum confinement effects appear through the formation of quantum well states regularly organized in energy and in space. For the smallest nanocrystals, only atomic-like electronic levels separated by a large energy scale are observed. Finally, in the intermediate size regime, discrete electronic levels associated to electronic wave-functions with a random spatial structure are observed, as expected from Random Matrix Theory.

cond-mat.supr-con↗

arXiv2018

Yu-Shiba-Rusinov bound states versus topological edge states in Pb/Si(111)

There is presently a tremendous activity around the field of topological superconductivity and Majorana fermions. Among the many questions raised, it has become increasingly important to establish the topological or non-topological origin of features associated with Majorana fermions such as zero-bias peaks. Here, we compare in-gap features associated either with isolated magnetic impurities or with magnetic clusters strongly coupled to the atomically thin superconductor Pb/Si(111). We study this system by means of scanning tunneling microscopy and spectroscopy (STM/STS). We take advantage of the fact that the Pb/Si(111) monolayer can exist either in a crystal-ordered phase or in an incommensurate disordered phase to compare the observed spectroscopic features in both phases. This allows us to demonstrate that the strongly resolved in-gap states we found around the magnetic clusters in the disordered phase of Pb have a clear topological origin.

cond-mat.supr-con↗

arXiv2017

Superconducting parity effect across the Anderson limit

How small superconductors can be? For isolated nanoparticles subject to quantum size effects, P.W. Anderson conjectured in 1959 that superconductivity could only exist when the electronic level spacing $\delta$ is smaller than the superconducting gap energy $\Delta$. Here, we report a scanning tunneling spectroscopy study of superconducting lead (Pb) nanocrystals grown on the (110) surface of InAs. We find that for nanocrystals of lateral size smaller than the Fermi wavelength of the 2D electron gas at the surface of InAs, the electronic transmission of the interface is weak; this leads to Coulomb blockade and enables the extraction of the electron addition energy of the nanocrystals. For large nanocrystals, the addition energy displays superconducting parity effect, a direct consequence of Cooper pairing. Studying this parity effect as function of nanocrystal volume, we find the suppression of Cooper pairing when the mean electronic level spacing overcomes the superconducting gap energy, thus demonstrating unambiguously the validity of the Anderson criterion.

cond-mat.supr-con↗

arXiv2016

Two-dimensional topological superconductivity in Pb/Co/Si(111)

Just like insulators can host topological Dirac states at their edges, superconductors can also exhibit topological phases characterized by Majorana edge states. Remarkable zero-energy states have been recently observed at the two ends of proximity induced superconducting wires, and were interpreted as localized Majorana end states in one-dimensional (1D) topological superconductor. By contrast, propagating Majorana states should exist at the 1D edges of two-dimensional (2D) topological superconductors. Here we report the direct observation of dispersive in-gap states surrounding topological superconducting domains made of a single atomic layer of Pb covering magnetic islands of Co/Si(111). We interpret the observed continuous dispersion across the superconducting gap in terms of a spatial topological transition accompanied by a chiral edge mode and residual gaped helical edge states. Our experimental approach enables the engineering and control of a large variety of novel quantum phases. This opens new horizons in the field of quantum materials and quantum electronics where the magnetization of the domains could be used as a control parameter for the manipulation of topological states.

cond-mat.supr-con↗

arXiv2015

Long range coherent magnetic bound states in superconductors

The quantum coherent coupling of completely different degrees of freedom is a challenging path towards creating new functionalities for quantum electronics. Usually the antagonistic coupling between spins of magnetic impurities and superconductivity leads to the destruction of the superconducting order. Here we show that a localized classical spin of an iron atom immersed in a superconducting condensate can give rise to new kind of long range coherent magnetic quantum state. In addition to the well-known Shiba bound state present on top of an impurity we reveal the existence of a star shaped pattern which extends as far as 12 nm from the impurity location. This large spatial dispersion turns out to be related, in a non-trivial way, to the superconducting coherence length. Inside star branches we observed short scale interference fringes with a particle-hole asymmetry. Our theoretical approach captures these features and relates them to the electronic band structure and the Fermi wave length of the superconductor. The discovery of a directional long range effect implies that distant magnetic atoms could coherently interact leading to new topological superconducting phases with fascinating properties.

cond-mat.supr-con↗

arXiv2013

Resistive switching induced by electronic avalanche breakdown in GaTa$_4$Se$_{8-x}$Te$_x$ narrow gap Mott Insulators

Mott transitions induced by strong electric fields are receiving a growing interest. Recent theoretical proposals have focused on the Zener dielectric breakdown in Mott insulators, however experimental studies are still too scarce to conclude about the mechanism. Here we report a study of the dielectric breakdown in the narrow gap Mott insulators GaTa$_4$Se$_{8-x}$Te$_x$. We find that the I-V characteristics and the magnitude of the threshold electric field (E$_{th}$) do not correspond to a Zener breakdown, but rather to an avalanche breakdown. E$_{th}$ increases as a power law of the Mott Hubbard gap (E$_g$), in surprising agreement with the universal law E$_{th}$ $\propto$E$_g$$^{2.5}$ reported for avalanche breakdown in semiconductors. However, the delay time for the avalanche that we observe in Mott insulators is over three orders of magnitude longer than in conventional semiconductors. Our results suggest that the electric field induces local insulator-to-metal Mott transitions that create conductive domains which grow to form filamentary paths across the sample.

cond-mat.str-el↗