F. Krishichayan | Search arXiv

arXiv2026

Photonuclear Cross Sections for the $^{197}$Au($\gamma$,pn)$^{195m}$Pt Reaction Near Threshold

Platinum radioisotopes are of growing interest for targeted cancer therapy and diagnostic imaging because their decay delivers highly localized radiation doses in tissue, herewith enabling precise DNA damage through Auger-electron emission. Developing production technologies that provide platinum isotopes with high specific activity is therefore essential, and photonuclear reactions on stable nuclei offer a viable accelerator-based route when supported by reliable cross-section data. We report photonuclear cross-section measurements for the $^{197}$Au($\gamma$,pn)$^{195m}$Pt reaction at incident $\gamma$-ray energies of 27, 29, and 31 MeV using the activation method. The measurements were performed by irradiating a stack of concentric-ring gold targets with a quasi-monoenergetic $\gamma$-ray beam provided by the High Intensity Gamma-ray Source (HI$\gamma$S). The induced $^{195m}$Pt activity was quantified using off-line $\gamma$-ray spectroscopy. These data provide the first experimental constraints on the $^{197}$Au($\gamma$,pn)$^{195m}$Pt cross section in the near-threshold region. The measured excitation function is compared with PHITS and TALYS calculations and indicates that the reaction becomes measurable only near 30 MeV, with substantially higher bremsstrahlung end-point energies required for practically meaningful production.

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arXiv2024

Photo-nuclear cross sections on $^{197}$Au, an update on the gold standard

A method was developed for measuring photonuclear reactions concurrently at several discrete photon beam energies on a stack of different target materials via a single irradiation. Concentric ring targets of the materials (in order from front to back targets: Au, TiO$_2$, Zn, Os, and Au) were irradiated at the High Intensity Gamma-ray Source (HI$\gamma$S). As a proof of principle, we report the result of the cross section measurements from the front Au target. The excitation functions of the $^{197}$Au($\gamma$,n)$^{196}$Au and $^{197}$Au($\gamma$,3n)$^{194}$Au reactions were determined in the incident photon energy range of 13-31 MeV using quasi-monoenergetic photon beams provided at HI$\gamma$S. The cross sections of the combined ground state (2$^{-}$) and short-lived first isomeric state (m1, 5$^{+}$), and of the second isomeric state (m2, 12$^{-}$) in the $^{196}$Au production are obtained separately by subtracting the $\gamma$ rays from the internal conversion of the second isomeric state. The excitation function of the second isomeric state via the photon-induced reaction $^{197}$Au($\gamma$,n)$^{196m2}$Au was measured for the first time. By using the activation method rather than direct neutron counting, the exclusive cross sections for the ($\gamma$,n) and ($\gamma$,3n) reactions were determined. Comparing the yields from the front and back gold targets validates our ability to simulate the effect of photon scattering in the target stack and provides a method for assessing the systematic uncertainty of our technique.

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