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I. Das

Publications and source records attributed to I. Das.

39 records · Page 3Linked to original sources

Thermal relaxation in charge ordered Pr$_{0.63}$ Ca$_{0.37}$ MnO$_3$ in presence of a magnetic field

We report observation of substantial thermal relaxation in single crystal of charge ordered system Pr$_{0.63}$Ca$_{0.37}$MnO$_3$ in an applied magnetic field of H = 8T. The relaxation is observed when the temperature is scanned in presence of a magnetic field in the temperature interval $T_{MH}<T<T_{CO}$ where $T_{CO}$ is the charge ordering temperature and $T_{MH}$ is charge melting temperature in a field. In this temperature range the system has coexisting charged ordered insulator (COI) and ferromagnetic metallic (FMM) phases. No such relaxation is observed in the COI state in H = 0T or in the FMM phase at $T < T_{MH}$ in presence of a magnetic field. We conclude that the thermal relaxation is due to two coexisting phases with nearly same free energies but separated by a potential barrier. This barrier makes the transformation from one phase to the other time-dependent in the scale of the specific heat experiment and gives rise to the thermal relaxation.

cond-mat.str-el↗

Specific heat study of single crystalline Pr$_{0.63}$ Ca$_{0.37}$ MnO$_{3}$ in presence of a magnetic field

We present the results of a study of specific heat on a single crystal of Pr$_{0.63}$Ca$_{0.37}$MnO$_3$ performed over a temperature range 3K-300K in presence of 0 and 8T magnetic fields. An estimate of the entropy and latent heat in a magnetic field at the first order charge ordering (CO) transition is presented. The total entropy change at the CO transition which is $\approx$ 1.8 J/mol K at 0T, decreases to $\sim$ 1.5 J/mol K in presence of 8T magnetic field. Our measurements enable us to estimate the latent heat $L_{CO}$ $\approx$ 235 J/mol involved in the CO transition. Since the entropy of the ferromagnetic metallic (FMM) state is comparable to that of the charge-ordered insulating (COI) state, a subtle change in entropy stabilises either of these two states. Our low temperature specific heat measurements reveal that the linear term is absent in 0T and surprisingly not seen even in the metallic FMM state.

cond-mat.str-el↗

Magneto-Transport properties in the thin films of Charge ordered thin films

Thin films of Pr0.7Ca 0.3MnO3, Nd-0.5Ca0.5MnO3 and Nd0.5Sr0.5MnO3 have been fabricated. by pulse laser deposition. Magnetic and electrical transport properties of these films were compared with their bulk solids. All the films grow in (101) direction on LaAlO3(100). Electrical transport measurements carried out with and without magnetic field has shown dr/dT<0 in these thin films. Application of magnetic field has shown dilution of the insulating behavior. The magnetization studies of Nd-0.5Sr0.5MnO3 exhibited ferromagnetic behavior at 260K and showed antiferomagnetic feature below 130K. This is close to the bulk magnetic behavior of Nd-0.5Sr0.5MnO3. Pr0.7Ca0.3MnO3 showed ferromagnetic transition below 130K and becomes antiferromagnetic at 90K. Nd-0.5Ca0.5MnO3 showed paramagnetic behavior down to low temperatures. Deviation in the properties of the thin films from the bulk solids is attributed to the growth of the films in more symmetric structure.

cond-mat.mtrl-sci↗