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I. Paulescu

Publications and source records attributed to I. Paulescu.

2 recordsLinked to original sources

Field-induced incipient spin-density phase stabilized inside the nematic phase of FeSe$_{1-x}$S$_x$

Spin-density wave (SDW) order and superconductivity frequently compete and coexist in unconventional superconductors, where spin fluctuations often mediate superconducting pairing. In iron-chalcogenide superconductors, FeSe$_{1-x}$S$_x$, SDW order has only been detected under applied pressure, while both spin and nematic fluctuations are involved in determining their rich superconducting phase diagrams. Here, we report evidence for an incipient SDW phase, within the nematic state of FeSe$_{1-x}$S$_x$, revealed in magnetic fields up to 68~T. Once superconductivity is quenched, we observe sharp upturns in longitudinal resistivity accompanied by anomalies in tunnel diode oscillator frequency response and torque anisotropy, consistent with a field-induced electronic order. Dominant low-frequency quantum oscillations reveal a small reconstructed Fermi surface, consistent with a field-induced SDW order. Direct experimental comparisons with a pressure-tuned nematic, analogue, FeSe$_{0.96}$S$_{0.04}$, demonstrate that SDW phases are stabilized within the nematic phase of FeSe$_{1-x}$S$_x$ via both chemical substitution and applied pressure. These findings reveal that by weakening nematicity, the SDW orders are stabilised, which promotes the dominant superconducting pairing mechanism in iron chalcogenides.

cond-mat.supr-con↗

Drastic field-induced resistivity upturns as signatures of unconventional magnetism in superconducting iron chalcogenides

Electronic scattering is a powerful tool to identify underlying changes in electronic behavior and incipient electronic and magnetic orders. The nematic and magnetic phases are strongly intertwined under applied pressure in FeSe, however, the additional isoelectronic substitution of sulphur offers an elegant way to separate them. Here we report the detailed evolution of the electronic and superconducting behaviour of FeSe$_{0.96}$S$_{0.04}$ under applied pressure via longitudinal magnetoresistance studies up to 15T. At intermediate pressures, inside the nematic phase, the resistivity displays an upturn in zero magnetic field, which is significantly enhanced in the magnetic field, suggesting the stabilization of a spin-density wave phase, which competes with superconductivity. At higher pressures, beyond the nematic phase boundaries, the resistivity no longer displays any clear anomalies in the zero magnetic field, but an external magnetic field induces significant upturns in resistivity reflecting a field-induced order, where superconductivity and magnetic anomalies are enhanced in tandem. This study highlights the essential role of high magnetic fields in stabilizing different electronic phases and revealing a complex interplay between magnetism and superconductivity tuned by applied pressure in FeSe$_{1-x}$S$_{x}$.

cond-mat.supr-con↗