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Jan Sperling

Publications and source records attributed to Jan Sperling.

At least 19 recordsLinked to original sources

Quantum sampling in hybrid light-matter systems with mixed statistics

Boson sampling is one of the most prominent methods to verify quantum advantage, harnessing the computational complexity of the permanent of a network matrix. Similar quantum sampling problems utilize other expressions for the output probabilities, such as the fermion-based analog applying determinants. In this work, we study sampling setups of interacting light-matter systems, combining fermion and boson sampling. The mixed network input consists of fermionic and bosonic excitations. Sampling the output probability of the modes then yields contributions that are neither purely determinant nor permanent but general immanants. Specifically, we prove that these immanant contributions are linearly independent from determinants and permanents, rendering our mixed sampling network an ideal candidate for light-matter quantum application beyond pure fermion and boson sampling. Furthermore, quantum sampling with statistics that are neither bosonic nor fermionic results in expressions which even exceed immanants, further extending the functionality of quantum samplers.

quant-ph

Quantum speedup from nonclassical polarization

We develop a framework for identifying nonclassical speedups in systems with polarization, likewise spin degrees of freedom. By confining the dynamics to the manifold of angular momentum coherent states, which act as the classical reference in this case, we compute the speed limit that bounds the rate of change of the state achievable without generating quantum coherence. A comparison with the unrestricted quantum speed limit enables the quantitative identification of speedups arising from polarization nonclassicality. We apply this framework to the cross-Kerr interaction, demonstrating a persistent speedup scaling as $\mathcal{O}(\sqrt{N})$ with the photon number $N$, with a parity effect in favour of even photon numbers. The results establish polarization nonclassicality as a genuine dynamical resource, linking quantum coherence to quantum-enhanced evolution speeds in nonlinear photonic systems.

quant-ph

Bounding Kirkwood-Dirac negativity of Gaussian processes

The Kirkwood-Dirac quasiprobability provides an operational representation of a quantum state, whose negativity serves as a measure of nonclassicality. Despite its fundamental importance, the extremal values of the Kirkwood-Dirac negativity are still unknown in the general case. We investigate the Kirkwood-Dirac quasiprobability of an arbitrary quantum state under Gaussian processes. In this setting, we derive an upper bound on the negativity for any number of modes and measurements. For a single mode and two measurements, we show that the eigenstates of the quadrature operators saturate this upper bound, while a nontrivial minimum is reached by pure Gaussian states. As a consequence, our results indicate that Gaussian states are sufficient to achieve extreme values of nonclassicality.

quant-ph

Demonstration of unpartible entanglement

We report on the first experimental verification of mode-independent entanglement. Commonly, the entanglement of a state is firmly based on pre-defined parties that are correlated, and the state might be disentangled when the definition of the parties is changed. Exceeding this party-dependent concept, we realize a type of quantum entanglement that persists even if the parties, in our case modes, are transformed. This safeguards the performance of entanglement in real-world applications, such as quantum communication settings involving noise and untrusted parties. For the state generation, we present an experimental scheme based on a fully reconfigurable temporally multiplexed interferometer with measurement-induced nonlinearities, which generates heralded two-photon states in two modes that are entangled for all choices of orthonormal mode basis. For the certification process, we utilize a tailored quantum-state tomography, achieving fidelities that validate the presence of mode-independent entanglement as a resilient and operationally advantageous quantum correlation.

quant-ph

Assessing the classicality of photon echo from excitons in lead halide perovskite nanocrystals

Photon echo (PE) spectroscopy is a powerful technique for probing decoherence mechanisms and charge carrier dynamics in semiconductor systems. Beyond traditional coherence measurements, characterizing the photon statistics of the echo signal is important for assessing its potential in quantum information applications and understanding the underlying quantum mechanical processes. Here, we study the photon statistics of PE signals generated by excitons in ensembles of lead halide perovskite CsPbI$_3$ nanocrystals at cryogenic temperature of 2 K using continuous-variable quantum state optical tomography based on homodyne detection. Pronounced Rabi oscillations of the PE amplitude allow us to evaluate the statistics for various pulse areas in the excitation sequence. The damping of the oscillations with increasing pulse area is attributed to spatial excitation inhomogeneity and excitation-induced dephasing. Despite the large ensemble of optically addressed excitons, the efficiency of generated PE signals is low which is attributed to the complex energy level structure of excitons and non-radiative recombination channels in CsPbI$_3$ nanocrystals. We analyze the statistical characteristics of PE via the second-order correlation function $g^{(2)}(0)$ and the characteristic function for different combinations of the areas of the excitation pulses. Our results show that $g^{(2)}(0) = 1$, and the characteristic function of the PE signal corresponds to classical behavior. The formation of photon echoes as well as $g^{(2)}(0) = 1$ at the echo time is reproduced by a quantized free-space multimode model. Despite the relatively low efficiency, the photon echo exhibits a high degree of coherence and minimal classical noise, consistent with Poissonian statistics.

cond-mat.mes-hall

Resource-efficient universal photonic processor based on time-multiplexed hybrid architectures

For the ever-growing field of quantum information processing, large-scale, efficient multi-port interferometers serving as photonic processors are required. In this context, the suitability of quantum walks as the interferometric base for universal computation has been theoretically proven. In this work, we bridge the gap between theoretical proposals and state-of-the-art experimental capabilities by providing the recipe for the implementation of a universal photonic processor in discrete-time quantum walks. Specifically, we present the protocol how to translate arbitrary linear transformations into the coin and step operator of a quantum walk and map these to the experimental parameters of the established time-multiplexed platform. We show that our interface is highly scalable and resource-efficient due to the hybrid encoding consisting of multiple degrees of freedom. Finally, we prove that our system is highly resilient against experimental imperfections and show that it compares favorably against existing architectures.

quant-ph

The entangling power of non-entangling channels

There are processes that cannot generate entanglement but may, nevertheless, amplify entanglement already present in a system. Here, we show that a non-entangling operation can increase the Schmidt number of a quantum state only if it can generate entanglement with some non-zero probability. This is in stark contrast to the case where the parties of a quantum network are only able to control their joint state by local operations and classical communication (LOCC). There, being able to apply operations probabilistically (stochastic LOCC) does not increase the Schmidt number. Our findings show that certain non-entangling operations become entangling when selecting on specific measurement outcomes. This naturally leads us to the class of stochastically non-entangling maps, being those that cannot generate entanglement even probabilistically. Intrigued by this finding, we devise a Schmidt number for quantum channels that quantifies whether a channel can generate entanglement probabilistically. Moreover, we show that a channel is non-entangling if and only if its dual map is witness-preserving -- it takes entanglement witnesses to witnesses. Based on this finding, we derive Bell-like inequalities whose violation signals that a process generates entanglement.

quant-ph

3D Anderson localization of light in disordered systems of dielectric particles

We investigate light transport in three-dimensional disordered media composed of irregular dielectric particles using large scale full-wave simulations. For subwavelength particles with size parameter $kr \approx 1$ and high refractive index contrast, we observe a transition from diffusion to a regime characterized by non-exponential decay of time-resolved transmission as disorder increases. The corresponding time-dependent diffusion coefficient decreases with time and approaches a $t^{-1}$ scaling at long times. This dynamical slowdown is accompanied by the emergence of spectrally isolated transmission resonances with Thouless conductance below unity, indicating the dominance of long-lived modes with weak spectral overlap. The late time near-field maps reveal evolving, non-propagating clusters of intensity hotspots. Together, the transport, spectral, and near-field signatures provide consistent numerical evidence for Anderson localization of light in three-dimensional disordered dielectric media.

physics.optics

Benchmarking Gaussian and non-Gaussian input states with a hybrid sampling platform

The original boson sampling paradigm-consisting of multiple single-photon input states, a large interferometer, and multi-channel click detection-was originally proposed as a photonic route to quantum computational advantage. Its non-Gaussian resources, essential for outperforming any classical system, are provided by single-photon inputs and click detection. Yet the drive toward larger experiments has led to the replacement of experimentally demanding single-photon sources with Gaussian states, thereby diminishing the available non-Gaussianity-a critical quantum resource. As the community broadens its focus from the initial sampling task to possible real-world applications, it becomes crucial to quantify the performance cost associated with reducing non-Gaussian resources and to benchmark sampling platforms that employ different input states. To address this need, we introduce the Paderborn Quantum Sampler (PaQS), a hybrid platform capable of performing sampling experiments with eight Gaussian or non-Gaussian input states in a 12-mode interferometer within a single experimental run. This architecture enables direct, side-by-side benchmarking of distinct sampling regimes under otherwise identical conditions. By employing a semi-device-independent framework, offering certification that does not rely on prior knowledge of the interferometer or the input states, we verify that the observed data cannot be reproduced by any classical model-a prerequisite for demonstrating quantum advantage. Applying this framework, we observe clear performance gains arising from non-Gaussian input states.

quant-ph

Multipartite entanglement dynamics in quantum walks

Quantum walks constitute a rich area of quantum information science, where multipartite entanglement plays a central role in the dynamics and scalability of quantum advantage over classical simulators. In this work, we study the multipartite entanglement of quantum walks in optical settings. We present methods for computing a geometric measure of entanglement for arbitrary partitions of a single-walker quantum walk and for analyzing the entanglement in multi-walker scenarios. These techniques are used for numerical studies on the entanglement dynamics of quantum walks in large systems and under various initial conditions. For a given bipartition, based on the coin degrees of freedom, we derive exact expressions describing the complete entanglement dynamics for arbitrary localized initial conditions. We use these expressions for analytic statements about the asymptotic behavior of the system. Furthermore, we demonstrate the emergence of entanglement typicality in statistical ensembles of random optical networks.

quant-ph

Quantifying entanglement in quantum thermodynamics via separability constraints

The role of quantum entanglement in thermodynamical systems remains elusive. Does entanglement result in thermodynamic advantages or does it impose fundamental limitations? Here, we unambiguously quantify the amount of heat and work in a quantum system that is due to the presence of entanglement. This is achieved by constraining the system's non-equilibrium dynamics to separable states, thereby isolating the impact entanglement has on thermodynamic effects. Unlike thermodynamic entanglement measures, which signify a loose connection between entanglement and thermodynamic properties, imposing a constraint constitutes an active intervention into a system -- answering how much of a system's thermodynamics is caused by (not correlated with) its quantumness. We benchmark our theory by applying the constrained dynamics to several multipartite systems, including quantum batteries and quantum refrigerators.

quant-ph

Learning to detect optical nonclassicality

Nonclassicality, defined in the quantum optical sense, serves as a resource for photon-based quantum technologies. Therefore, certifying the nonclassicality of a quantum state is crucial for gauging its potential for quantum advantage. However, traditional nonclassicality witnesses that assume perfect knowledge of the witness observables often fail in realistic scenarios with limited statistics and finite-resolution photon detectors. Furthermore, these witnesses do not exploit the fact that certain states are unlikely to be observed in a given experiment. Here, we train a variational model to distinguish classical from nonclassical states using finitely many measurement samples of multimode quantum states that are probed with different photon-number-resolving detection schemes. The learned decision rule is then an indicator of nonclassicality, tailored to a given set of physically relevant states. Our approach is both data-driven and interpretable in the sense that the learned analytical decision rule can be extracted. Training the model on experimental data measured with (i) a superconducting nanowire single-photon detector and (ii) a time-bin multiplexing detection scheme demonstrates the versatility of the approach, paving the way for efficient nonclassicality detection.

quant-ph

Observable nonclassicality witnesses for multiplexed detection systems

We address the problem of constructing witnesses for nonclassical light that are applicable in state-of-the-art photon-counting devices. The key ingredient for the criteria we derive are generalized and directly measurable counting statistics and matrices of counting moments. Beyond common criteria, we find classes of witnesses that are based on half-integer powers of click moments and counts. Remarkably, this leads to an exponential increase of the number of nonclassicality criteria one can construct and apply. With this finding, special attention is payed to probing even and odd parity states, requiring such distinct witnesses. Our method is applicable to spatial and time-bin multiplexing in optical systems, where each spatial and temporal mode can be measured with both on-off detectors and detectors with partial internal quasi-photon-number resolution. Generalizations to multimode scenarios are provided, allowing for the direct measurement of nonclassical correlations and coincidence counts between an arbitrary number of modes.

quant-ph

Universal entanglement-inspired correlations

Quantum correlations, crucial for the advantage and advancement of quantum science and technology, arise from the impossibility of expressing a quantum state as a tensor product over a given set of parties. In this work, a generalized notion of correlations via arbitrary products is formulated. Remarkably, as a universal property, the connection between such general products and tensor products is established, allowing one to relate generic non-product states to the common notion of entangled states. We construct the set of free operations for general types of products by extending the local-operation-and-classical-communication paradigm, familiar from standard entanglement theory, thereby establishing a resource theory of correlations for general products. A generalization is provided beyond two factors that can be universally related to multipartite entanglement. Applications that highlight the usefulness of the approach are discussed, such as the factorization of fermionic states, the non-local factorization of multi-photon states into single-photon states, and the interesting possibility of understanding prime numbers as a form of single-party entanglement.

quant-ph

Numerical approaches to entangling dynamics from variational principles

In this work, we address the numerical identification of entanglement in dynamical scenarios. To this end, we consider different programs based on the restriction of the evolution to the set of separable (i.e., non-entangled) states, together with the discretization of the space of variables for numerical computations. As a first approach, we apply linear splitting methods to the restricted, continuous equations of motion derived from variational principles. We utilize an exchange interaction Hamiltonian to confirm that the numerical and analytical solutions coincide in the limit of small time steps. The application to different Hamiltonians shows the wide applicability of the method to detect dynamical entanglement. To avoid the derivation of analytical solutions for complex dynamics, we consider variational, numerical integration schemes, introducing a variational discretization for Lagrangians linear in velocities. Here, we examine and compare two approaches: one in which the system is discretized before the restriction is applied, and another in which the restriction precedes the discretization. We find that the "first-discretize-then-restrict" method becomes numerically unstable, already for the example of an exchange-interaction Hamiltonian, which can be an important consideration for the numerical analysis of constrained quantum dynamics. Thereby, broadly applicable numerical tools, including their limitations, for studying entanglement over time are established for assessing the entangling power of processes that are used in quantum information theory.

quant-ph

Local-oscillator-agnostic squeezing detection

We address the problem of measuring nonclassicality in continuous-variable bosonic systems without having access to a known reference signal. To this end, we construct broader classes of criteria for nonclassicality which allow us to investigate quantum phenomena regardless of the quantumness of selected subsystems. Such witnesses are based on the notion of partial normal ordering. This approach is applied to balanced homodyne detection using arbitrary, potentially nonclassical local oscillator states, yet only revealing the probed signal's quantumness. Our framework is compared to standard techniques, and the robustness and advanced sensitivity of our approach is shown. Therefore, a widely applicable framework, well-suited for applications in quantum metrology and quantum information, is derived to assess the quantum features of a photonic system when a well-defined coherent laser as a reference state is not available in the physical domain under study.

quant-ph

Universal Topology of Exceptional Points in Nonlinear Non-Hermitian Systems

Exceptional points (EPs) are non-Hermitian degeneracies where eigenvalues and eigenvectors coalesce, giving rise to unusual physical effects across scientific disciplines. The concept of EPs has recently been extended to nonlinear physical systems. We theoretically demonstrate a universal topology in the nonlinear parameter space for a large class of physical systems that support 2nd order EPs in the linear regime. Knowledge of this topology (called elliptic umbilic singularity in bifurcation theory) deepens our understanding of 2nd order linear EPs, which here emerge as coalescence of 4 nonlinear eigenvectors. This helps guide future experimental discovery of nonlinear EPs and their classification, establish rigorous bounds of sensitivity enhancement of EPs in nonlinear systems, and helps envision and optimize technological applications of nonlinear EPs. Our theoretical approach is general and can be extended to nonlinear perturbations of 3rd and higher-order EPs.

physics.optics

Separability Lindblad equation for dynamical open-system entanglement

Providing entanglement for the design of quantum technologies in the presence of noise constitutes today's main challenge in quantum information science. A framework is required that assesses the build-up of entanglement in realistic settings. In this work, we put forth a new class of nonlinear quantum master equations in Lindblad form that unambiguously identify dynamical entanglement in open quantum systems via deviations from a separable evolution. This separability Lindblad equation restricts quantum trajectories to classically correlated states only. Unlike many conventional approaches, here the entangling capabilities of a process are not characterized by input-output relations, but separability is imposed at each instant of time. We solve these equations for crucial examples, thereby quantifying the dynamical impact of entanglement in non-equilibrium scenarios. Our results allow to benchmark the engineering of entangled states through dissipation. The separability Lindblad equation provides a unique path to characterizing quantum correlations caused by arbitrary system-bath interactions, specifically tailored for the noisy intermediate-scale quantum era.

quant-ph