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Jonathan Ward

Publications and source records attributed to Jonathan Ward.

At least 19 recordsLinked to original sources
arXiv2025

Spinon mediation of witness spin dynamics in herbertsmithite

The kagome lattice of spin-1/2 copper atoms in herbertsmithite is conjectured to sustain a quantum spin liquid state with spinon quasiparticles. Ideally, the kagome crystal planes are each separated by a plane of spinless zinc atoms. However, in real crystals some spin-1/2 copper atoms substitute randomly onto these inter-kagome zinc sites. Here we reconceptualize such 'impurity' atoms as quantum witness spins whose dynamics is designed to probe the spin liquid state. We then introduce spin noise spectroscopy to measure the frequency and temperature dependence of witness spin dynamics, demonstrating that their phenomenology is consistent with extensive interactions between witness spins mediated by propagation of spinons through a quantum spin liquid. Ultimately, a sharp transition occurs at around 260 mK, below which the properties of both spin noise and magnetic susceptibility suggest that the witness spins form a spin glass phase. Among theoretical models considered, we demonstrate that our observations are only consistent with spinon-mediated interactions between witness spins by either a Z2 or U(1) quantum spin liquid, with the former model more closely matching the data. Our work demonstrates that quantum mechanical witness spins may now conceivably be used as a widely applicable probe of quantum spin liquid physics.

cond-mat.str-el↗
arXiv2024

Discovery of Dynamical Heterogeneity in a Supercooled Magnetic Monopole Fluid

Dynamical heterogeneity, in which transitory local fluctuations occur in the conformation and dynamics of constituent particles, is widely hypothesized to be essential to evolution of supercooled liquids into the structural glass state. Yet its microscopic spatiotemporal phenomenology is challenging to detect directly in molecular glass forming liquids. Because recent theoretical advances predict that corresponding dynamical heterogeneity could occur in supercooled magnetic monopole fluids (Proc. Nat. Acad. Sci. 112, 8549 (2015)), we searched for such phenomena in Dy2Ti2O7. By measuring its microsecond-resolved spontaneous magnetization fluctuations $M(t,T)$ we discovered a sharp bifurcation in monopole noise characteristics below $T \approx 1500$ mK, with the appearance of powerful spontaneous monopole current bursts. This intense dynamics emerges upon entering the supercooled monopole fluid regime, reaches maximum strength near $T \approx 750$ mK and then collapses along with coincident loss of ergodicity approaching $T_g \approx 750$ mK. Moreover, when the four-point dynamical susceptibility $\chi_4(\tau, T)$ is determined directly from temperature dependence of correlations in $M(t,T)$, it evolves as predicted when dynamical heterogeneity is present, revealing its simultaneously and rapidly escalating length and time scales, $\xi(T)$. and $\tau_4(T)$. This overall phenomenology 2 greatly expands our empirical knowledge of supercooled monopole fluids and, more generally, demonstrates direct detection of the time sequence, magnitude, statistics and correlations of dynamical heterogeneity, access to which may greatly accelerate fundamental vitrification studies.

cond-mat.str-el↗
arXiv2024

Spiral Spin Liquid Noise

An emerging concept for identification of different types of spin liquids is through the use of spontaneous spin noise. Here we develop spin noise spectroscopy for spin liquid studies by considering Ca$_{10}$Cr$_7$O$_{28}$, a material hypothesized to be either a quantum or a spiral spin liquid. By enhancing techniques introduced for magnetic monopole noise studies we measure the time and temperature dependence of spontaneous flux $\varPhi(t, T)$ and thus magnetization $M(t, T)$ of Ca$_{10}$Cr$_7$O$_{28}$ samples. The resulting power spectral density of magnetization noise $S_M(\omega,T)$ reveals intense spin fluctuations with $S_M(\omega,T) \propto \omega^{-\alpha(T)}$ and 0.84 < $\alpha (T)$ < 1.04 . Both the variance $\sigma_M^2(T)$ and the correlation function $C_M(t,T)$ of this spin noise undergo crossovers at a temperature $T^* \approx$ 450 mK. While predictions for quantum spin liquids are inconsistent with this phenomenology, those from Monte-Carlo simulations of a 2D spiral spin liquid state in Ca$_{10}$Cr$_7$O$_{28}$ yield overall quantitative correspondence with the measured frequency and temperature dependences of $S_M(\omega,T), C_M(t,T)$ and $\sigma _M^2(T)$, thus indicating that Ca$_{10}$Cr$_7$O$_{28}$ is a spiral spin liquid.

cond-mat.str-el↗
arXiv2024

Dichotomous Dynamics of Magnetic Monopole Fluids

A recent advance in the study of emergent magnetic monopoles was the discovery that monopole motion is restricted to dynamical fractal trajectories (J. Hall\'en et al, Science 378, 1218 (2022)) thus explaining the characteristics of magnetic monopole noise spectra (Dusad, R. et al. Nature 571, 234 (2019); Samarakoon, A. M. et al. Proc. Natl. Acad. Sci. 119, e2117453119 (2022)). Here we apply this new theory to explore the dynamics of field-driven monopole currents, finding them comprised of two quite distinct transport processes: initially swift fractal rearrangements of local monopole configurations followed by conventional monopole diffusion. This theory also predicts a characteristic frequency dependence of the dissipative loss-angle for AC-field-driven currents. To explore these novel perspectives on monopole transport, we introduce simultaneous monopole current control and measurement techniques using SQUID-based monopole current sensors. For the canonical material Dy2Ti2O7, we measure ${\Phi}(t)$, the time-dependence of magnetic flux threading the sample when a net monopole current $J(t) = \dot{\Phi}(t)/\mu_0$ is generated by applying an external magnetic field $B_0(t)$. These experiments find a sharp dichotomy of monopole currents, separated by their distinct relaxation time-constants before and after $t \approx 600 {\mu}s$ from monopole current initiation. Application of sinusoidal magnetic fields $B_0(t) = Bcos({\omega}t)$ generates oscillating monopole currents whose loss angle ${\theta}(f)$ exhibits a characteristic transition at frequency $f \approx 1.8$ kHz over the same temperature range. Finally, the magnetic noise power is also dichotomic, diminishing sharply after $t \approx 600 {\mu}s$. This complex phenomenology represents a new form of heterogeneous dynamics generated by the interplay of fractionalization and local spin configurational symmetry.

cond-mat.mes-hall↗
arXiv2022

Self-critiquing models for assisting human evaluators

We fine-tune large language models to write natural language critiques (natural language critical comments) using behavioral cloning. On a topic-based summarization task, critiques written by our models help humans find flaws in summaries that they would have otherwise missed. Our models help find naturally occurring flaws in both model and human written summaries, and intentional flaws in summaries written by humans to be deliberately misleading. We study scaling properties of critiquing with both topic-based summarization and synthetic tasks. Larger models write more helpful critiques, and on most tasks, are better at self-critiquing, despite having harder-to-critique outputs. Larger models can also integrate their own self-critiques as feedback, refining their own summaries into better ones. Finally, we motivate and introduce a framework for comparing critiquing ability to generation and discrimination ability. Our measurements suggest that even large models may still have relevant knowledge they cannot or do not articulate as critiques. These results are a proof of concept for using AI-assisted human feedback to scale the supervision of machine learning systems to tasks that are difficult for humans to evaluate directly. We release our training datasets, as well as samples from our critique assistance experiments.

cs.CL↗
arXiv2021

Blue-band frequency comb and photodarkening in silica whispering gallery microresonators

To date there are extensive studies of optical nonlinearities in whispering gallery resonators (WGRs) in the near and mid-infrared wavelengths. Pushing this research into the visible region is equally valuable. Here, we demonstrate a Kerr frequency comb and Raman lasing at 462 nm in an SiO2 WGR. Notably, due to the high optical intensities achieved, photodarkening is unavoidable and can quickly degrade the optical quality of both the coupling optical nanofiber and the microcavity even at very low pump powers. Nonetheless, stable stimulated Raman scattering (SRS) and hyper-parametric oscillation in normally dispersed WGRs is demonstrated in the presence of photodarkening by taking advantage of in-situ thermal bleaching. These observations highlight the challenges of silica-based, short wavelength nonlinear optics in high quality, small mode volume devices. We propose a method to overcome this apparent limitation and demonstrate blue-band nonlinear optical processes in silica WGRs, thus providing a baseline for optics research in the blue region for any optical devices fabricated from SiO2.

physics.optics↗
arXiv2020

Transaction Pricing for Maximizing Throughput in a Sharded Blockchain Ledger

In this paper, we present a pricing mechanism that aligns incentives of agents who exchange resources on a decentralized ledger with the goal of maximizing transaction throughput. Subdividing a blockchain ledger into shards promises to greatly increase transaction throughput with minimal loss of security. However, the organization and type of the transactions also affects the ledger's efficiency, which is increased by wallet agents transacting in a single shard whenever possible while collectively distributing their transactions uniformly across the available shards. Since there is no central authority to enforce these properties, the only means of achieving them is to design the system such that it is in agents' interest to act in a way that benefits overall throughput. We show that our proposed pricing policy does exactly this by inducing a potential game for the agents, where the potential function relates directly to ledger throughput. Simulations demonstrate that this policy leads to near-optimal throughput under a variety of conditions.

eess.SY↗
arXiv2020

Democratising blockchain: A minimal agency consensus model

We propose a novel consensus protocol based on a hybrid approach, that combines a directed acyclic graph (DAG) and a classical chain of blocks. This architecture allows us to enforce collective block construction, minimising the monopolistic power of the round-leader. In this way, we decrease the possibility for collusion among senders and miners, as well as miners themselves, allowing the use of more incentive compatible and fair pricing strategies. We investigate these possibilities alongside the ability to use the DAG structure to minimise the risk of transaction censoring. We conclude by providing preliminary benchmarks of our protocol and by exploring further research directions.

cs.CR↗
arXiv2017

Logarithmic singularities and quantum oscillations in magnetically doped topological insulators

We report magnetotransport measurements on magnetically doped (Bi,Sb)$_2$Te$_3$ films grown by molecular beam epitaxy. In Hallbar devices, logarithmic dependence on temperature and bias voltage are obseved in both the longitudinal and anomalous Hall resistance. The interplay of disorder and electron-electron interactions is found to explain quantitatively the observed logarithmic singularities and is a dominant scattering mechanism in these samples. Submicron scale devices exhibit intriguing quantum oscillations at high magnetic fields with dependence on bias voltage. The observed quantum oscillations can be attributed to bulk and surface transport.

cond-mat.str-el↗
arXiv2017

Pump induced lasing suppression in Yb:Er-doped microlasers

A pump source is one of the essential prerequisites in order to achieve lasing, and, in most cases, a stronger pump leads to higher laser power at the output. However, this behavior may be suppressed if two pump beams are used. In this work, it is shown that lasing around the 1600 nm band can be suppressed completely if two pumps, at wavelengths of 980 nm and 1550 nm, are applied simultaneously to a Yb:Er-doped microlaser, whereas it can be revived by switching one of them off. This phenomenon can be explained by assuming that the existence of one pump (980 nm) changes the role of the other pump (1550 nm); more specifically, the 1550 nm pump starts to consume the population inversion instead of increasing it when the 980 nm pump power exceeds a certain value. As a result, the two pump fields lead to a closed-loop transition within the gain medium (i.e., erbium ions). This study unveils an interplay similar with coherence effects between different pump pathways, which provides a reference for designing the laser pump and may have applications in lasing control.

physics.optics↗
arXiv2016

Tunable erbium-doped microbubble laser fabricated by sol-gel coating

In this work, we show that the application of a sol-gel coating renders a microbubble whispering gallery resonator into an active device. During the fabrication of the resonator, a thin layer of erbium-doped sol-gel is applied to a tapered microcapillary, then a microbubble with a wall thickness of 1.3 $\mu$m is formed with the rare earth diffused into its walls. The doped microbubble is pumped at 980 nm and lasing in the emission band of the Er$^{3+}$ ions with a wavelength of 1535 nm is observed. The laser wavelength can be tuned by aerostatic pressure tuning of the whispering gallery modes of the microbubble. Up to 240 pm tuning is observed with 2 bar of applied pressure. It is shown that the doped microbubble could be used as a compact, tunable laser source. The lasing microbubble can also be used to improve sensing capabilities in optofluidic sensing applications.

physics.optics↗
arXiv2016

Four-wave mixing parametric oscillation and frequency comb generation at visible wavelengths in a silica microbubble resonator

Frequency comb generation in microresonators at visible wavelengths has found applications in a variety of areas such as metrology, sensing, and imaging. To achieve Kerr combs based on four-wave mixing in a microresonator, dispersion must be in the anomalous regime. In this work, we demonstrate dispersion engineering in a microbubble resonator (MBR) fabricated by a two-CO$_2$ laser beam technique. By decreasing the wall thickness of the MBR down to 1.4 $\mu$m, the zero dispersion wavelength shifts to values shorter than 764 nm, making phase matching possible around 765 nm. With the optical \textit{Q}-factor of the MBR modes being greater than $10^7$, four-wave mixing is observed at 765 nm for a pump power of 3 mW. By increasing the pump power, parametric oscillation is achieved, and a frequency comb with 14 comb lines is generated at visible wavelengths.

physics.optics↗
arXiv2015

Degenerate four-wave-mixing in a silica hollow bottle-like microresonator

A hollow bottle-like microresonator (BLMR) with ultra-high quality factor is fabricated from a microcapillary with nearly parabolic profile. At 1.55 $\mu m$ pumping, degenerate four-wave mixing can be observed for a BLMR of diameter 102 $\mu$m. The parabolic profile of the BLMR guarantees a nearly zero waveguide dispersion, which is theoretically discussed in detail. From the simulation, at 1.55 $\mu$m wavelength in such a BLMR, the fundamental bottle mode is in the anomalous dispersion regime, whilst the ordinary whispering gallery mode (WGM) confined at the center of the BLMR is in the normal dispersion regime. Experimentally, no degenerate FWM is observed for the WGM selected by positioning the coupling tapered fiber in the same BLMR. Furthermore, dispersion tuning is briefly discussed. As the work predicted, the BLMR shows promise for the implementation of sparsely distributed, widely spanned frequency combs at the telecommunication wavelength.

physics.optics↗
arXiv2015

Raman lasing in a hollow, bottle-like microresonator

We report on the fabrication of an ultrahigh quality factor, bottle-like microresonator from a microcapillary, and the realization of Raman lasing therein at pump wavelengths of $1.55~\mathrm{\mu m}$ and $780~\mathrm{nm}$. The dependence of the Raman laser threshold on mode volume is investigated. The mode volume of the fundamental bottle mode is calculated and compared with that of a microsphere. Third-order cascaded Raman lasing was observed when pumped at $780~\mathrm{nm}$. In principle, Raman lasing in a hollow bottle-like microresonator can be used in sensing applications. As an example, we briefly discuss the possibility of a high dynamic range, high resolution aerostatic pressure sensor.

physics.optics↗
arXiv2015

Coupled-mode induced transparency in aerostatically-tuned microbubble whispering gallery resonators

Coupled-mode induced transparency is realized in a single microbubble whispering gallery mode resonator. Using aerostatic tuning, we find that the pressure induced shifting rates are different for different radial order modes. A finite element simulation considering both the strain and stress effects shows a GHz/bar difference and this is confirmed by experiments. A transparency spectrum is obtained when a first order mode shifts across a higher order mode through precise pressure tuning. The resulting lineshapes are fitted with the theory. This work lays a foundation for future applications in microbubble sensing.

physics.optics↗
arXiv2014

Quasi-droplet Microbubbles for High Resolution Sensing Applications

Optical properties and sensing capabilities of fused silica microbubbles were studied numerically using a finite element method. Mode characteristics, such as quality factor (Q) and effective refractive index, were determined for different bubble diameters and shell thicknesses. For sensing applications with whispering gallery modes (WGMs), thinner shells yield improved sensitivity. However, the Q-factor decreases with reduced thickness and this limits the final resolution. Three types of sensing applications with microbubbles, based on their optimized geometrical parameters, were studied. Herein the so-called quasi-droplet regime is defined and discussed. It is shown that best resolution can be achieved when microbubbles act as quasi-droplets, even for water-filled cavities at the telecommunications C-band.

physics.optics↗
arXiv2013

Aperiodic dynamics in a deterministic model of attitude formation in social groups

Homophily and social influence are the fundamental mechanisms that drive the evolution of attitudes, beliefs and behaviour within social groups. Homophily relates the similarity between pairs of individuals' attitudinal states to their frequency of interaction, and hence structural tie strength, while social influence causes the convergence of individuals' states during interaction. Building on these basic elements, we propose a new mathematical modelling framework to describe the evolution of attitudes within a group of interacting agents. Specifically, our model describes sub-conscious attitudes that have an activator-inhibitor relationship. We consider a homogeneous population using a deterministic, continuous-time dynamical system. Surprisingly, the combined effects of homophily and social influence do not necessarily lead to group consensus or global monoculture. We observe that sub-group formation and polarisation-like effects may be transient, the long-time dynamics being quasi-periodic with sensitive dependence to initial conditions. This is due to the interplay between the evolving interaction network and Turing instability associated with the attitudinal state dynamics.

physics.soc-ph↗