arXiv subjects

K. Foster

Publications and source records attributed to K. Foster.

8 recordsLinked to original sources

arXiv2026

Resonant photoionization dynamics during optical trapping of lithium atoms

Photoionization induced by trapping and auxiliary laser fields is an inherent feature of many laser-cooling and optical trapping experiments, yet its microscopic dynamics are rarely investigated directly. In this work, we employ a reaction microscope implementing an event-by-event photoionization time retrieval technique to extend momentum-resolved photoelectron spectroscopy to continuous-wave laser--atom interactions. We investigate low-intensity multicolor photoionization of laser-cooled lithium atoms confined in an all-optical trap. Complete three-dimensional electron momentum distributions and kinetic-energy spectra recorded for different laser wavelengths and polarization configurations identify resonant excitation of the $5p$ and $5f$ states and reveal an additional ionization channel following spontaneous decay from the $5f$ to the $4d$ state. A pronounced polarization dependence of the photoionization yield is explained by magnetic-sublevel selection rules and the coherent interference of different virtual excitation pathways. These results demonstrate that reaction microscopy combined with event-by-event time reconstruction provides a powerful approach for investigating microscopic electronic dynamics in laser-cooled atomic systems and offers new insight into photoionization processes occurring during optical trapping.

physics.atom-ph↗

arXiv2023

A pump-probe experiment in cw-mode on ionization of Rydberg atoms

Rydberg atoms are in the focus of intense research due to the peculiar properties which make them interesting candidates for quantum optics and quantum information applications. In this work we study the ionization of Rydberg atoms due to their interaction with a trapping laser field, and a reaction microscope is used to measure photoelectron angular and energy distributions. Reaction microscopes are excellent tools when brandished against atomic photoionization processes involving pulsed lasers; the timing tied to each pulse is crucial in solving the subsequent equations of motion for the atomic fragments in the spectrometer field. However, when used in pump-probe schemes, which rely on continuous wave probe lasers, vital information linked to the time of flight is lost. This study reports on a method in which the standard ReMi technique is extended in time through coincidence measurements. This is then applied to the photoionization of $^6$Li atoms initially prepared in optically pumped $2^{2}S_{1/2}$ and $2^{2}P_{3/2}$ states. Multi-photon excitation from a tunable femtosecond laser is exploited to produce Rydberg atoms inside an infrared optical dipole trap; the structure and dynamics of the subsequent cascade back towards ground is evaluated.

physics.atom-ph↗

arXiv2022

Two-path interference in the resonance-enhanced few-photon ionization of atoms

We investigate the resonance-enhanced few-photon ionization of atomic lithium by linearly polarized light whose frequency is tuned near the 2s-2p transition. Considering the direction of light polarization orthogonal to the quantization axis, the process can be viewed as an atomic "double-slit experiment" where the 2p states with magnetic quantum numbers m_l=+-1 act as the slits. In our experiment, we can virtually close one of the two slits by preparing lithium in one of the two circularly polarized 2p states before subjecting it to the ionizing radiation. This allows us to extract the interference term between the two pathways and obtain complex phase information on the final state. The experimental results show very good agreement with numerical solutions of the time-dependent Schroedinger equation. The validity of the two-slit model is also analyzed theoretically using a time-dependent perturbative approach.

physics.atom-ph↗

arXiv2021

Magnetic Dichroism in Few-Photon Ionization of Polarized Atoms

We consider few-photon ionization of atomic lithium by linearly polarized femtosecond laser pulses, and demonstrate that asymmetries of the electron angular distribution can occur for initially polarized (2p, m=+1) target atoms. The dependence of the photoelectron emission angle relative to the electric field direction is investigated at different laser intensities and wavelengths. The experimental spectra show excellent agreement with numerical solutions of the time-dependent Schroedinger equation. In the perturbative picture, the angular shift is traced back to interferences between partial waves with mean magnetic quantum number $\ne$0. This observation allows us to obtain quantum mechanical information on the electronic final state.

physics.atom-ph↗

arXiv2021

Constraining particle acceleration in Sgr A* with simultaneous GRAVITY, Spitzer, NuSTAR and Chandra observations

We report the time-resolved spectral analysis of a bright near-infrared and moderate X-ray flare of Sgr A*. We obtained light curves in the $M$-, $K$-, and $H$-bands in the mid- and near-infrared and in the $2-8~\mathrm{keV}$ and $2-70~\mathrm{keV}$ bands in the X-ray. The observed spectral slope in the near-infrared band is $\nu L_\nu\propto \nu^{0.5\pm0.2}$; the spectral slope observed in the X-ray band is $\nu L_\nu \propto \nu^{-0.7\pm0.5}$. We tested synchrotron and synchrotron self-Compton (SSC) scenarios. The observed near-infrared brightness and X-ray faintness, together with the observed spectral slopes, pose challenges for all models explored. We rule out a scenario in which the near-infrared emission is synchrotron emission and the X-ray emission is SSC. A one-zone model in which both the near-infrared and X-ray luminosity are produced by SSC and a model in which the luminosity stems from a cooled synchrotron spectrum can explain the flare. In order to describe the mean SED, both models require specific values of the maximum Lorentz factor $\gamma_{max}$, which however differ by roughly two orders of magnitude: the SSC model suggests that electrons are accelerated to $\gamma_{max}\sim 500$, while cooled synchrotron model requires acceleration up to $\gamma_{max}\sim5\times 10^{4}$. The SSC scenario requires electron densities of $10^{10}~\mathrm{cm^{-3}}$ much larger than typical ambient densities in the accretion flow, and thus require in an extraordinary accretion event. In contrast, assuming a source size of $1R_s$, the cooled synchrotron scenario can be realized with densities and magnetic fields comparable with the ambient accretion flow. For both models, the temporal evolution is regulated through the maximum acceleration factor $\gamma_{max}$, implying that sustained particle acceleration is required to explain at least a part of the temporal evolution of the flare.

astro-ph.HE↗

arXiv2021

Circular Dichroism in Atomic Resonance-Enhanced Few-Photon Ionization

We investigate few-photon ionization of lithium atoms prepared in the polarized 2$p$($m_\ell=\!+1$) state when subjected to femtosecond light pulses with left- or right-handed circular polarization at wavelengths between 665 nm and 920 nm. We consider whether ionization proceeds more favorably for the electric field co- or counter-rotating with the initial electronic current density. Strong asymmetries are found and quantitatively analyzed in terms of "circular dichroism" ($CD$). While the intensity dependence of the measured $CD$ values is rather weak throughout the investigated regime, a very strong sensitivity on the center wavelength of the incoming radiation is observed. While the co-rotating situation overall prevails, the counter-rotating geometry is strongly favored around 800 nm due to the 2$p$-3$s$ resonant transition, which can only be driven by counter-rotating fields. The observed features provide insights into the helicity dependence of light-atom interactions, and on the possible control of electron emission in atomic few-photon ionization by polarization-selective resonance enhancement.

physics.atom-ph↗

arXiv2020

Using circular dichroism to control energy transfer in multi-photon ionization

Chirality causes symmetry breaks in a large variety of natural phenomena ranging from particle physics to biochemistry. We investigate one of the simplest conceivable chiral systems, a laser-excited, oriented, effective one-electron Li target. Prepared in a polarized p state with |m|=1 in an optical trap, the atoms are exposed to co- and counter-rotating circularly polarized femtosecond laser pulses. For a field frequency near the excitation energy of the oriented initial state, a strong circular dichroism is observed and the photoelectron energies are significantly affected by the helicity-dependent Autler-Townes splitting. Besides its fundamental relevance, this system is suited to create spin-polarized electron pulses with a reversible switch on a femtosecond timescale at an energy resolution of a few meV.

physics.atom-ph↗

arXiv2019

Photo-ionization of polarized lithium atoms out of an all-optical atom trap: A complete experiment

An all-optical, near-resonant laser atom trap is used to prepare an electronically excited and polarized gas target at mK-temperature for complete photo-ionization studies. As a proof-of-principal experiment, lithium atoms in the 2$^2$P$_{3/2}$($m_l$=+1) state are ionized by a 266 nm laser source, and emitted electrons and Li$^+$ ions are momentum analyzed in a COLTRIMS spectrometer. The excellent resolution achieved in the present experiment allows not only to extract the relative phase and amplitude of all partial waves contributing to the final state, it also enables to characterize the experiment regarding target and spectrometer properties. Photo-electron angular distributions are measured for five different laser polarizations and described in a one-electron approximation with excellent agreement.

physics.atom-ph↗