arXiv subjects

M. Block

Publications and source records attributed to M. Block.

At least 19 recordsLinked to original sources

arXiv2025

High-Resolution Laser Spectroscopy on the Hyperfine Structure of $^{255}$Fm (Z=100)

We report on high-resolution laser spectroscopy of $^{255}$Fm ($T_{1/2} = 20$h), one of the heaviest nuclides available from reactor breeding. The hyperfine structures in two different atomic ground-state transitions at 398.4~nm and 398.2~nm were probed by in-source laser spectroscopy at the RISIKO mass separator in Mainz, using the PI-LIST high-resolution ion source. Experimental results were combined with hyperfine fields from various atomic ab-initio calculations, in particular using MultiConfigurational Dirac-Hartree-Fock theory, as implemented in GRASP18. In this manner, the nuclear magnetic dipole and electric quadrupole moments were derived to be $\mu = -0.75(5)~ \mu_\textrm{N}$ and $Q_\textrm{S} = +5.84(13)$~eb, respectively. The magnetic moment indicates occupation of the $\nu$~7/2[613] Nilsson orbital, while the large quadrupole moment confirms strong, stable prolate deformation consistent with systematics in the heavy actinides. Comparisons with available expectation values from nuclear theory show good agreement, providing a stringent benchmark for the used theoretical models. These results revise earlier data and establish $^{255}$Fm as a reference isotope for future high-resolution studies.

physics.atom-ph↗

arXiv2021

Some remarks on the discovery of Md-244

In two recent papers by Pore et al. and Khuyagbaatar et al. discovery of the new isotope Md-244 was reported. The decay data, however, are conflicting. While Pore et al. report two isomeric states decaying by alpha emission with E(1)=8.66(2) MeV, T_1/2=0.4+0.4/-0.1s and E(2)=8.31(2) MeV, T_1/2 approx 6 s, Khuyagbaatar et al. report only a single transition with a broad energy distribution of E=(8.73-8.86) MeV and T_1/2=0.30/-0.09 s. The data published by Pore et al. very similar to those published for Md-245 (E=8.64(2), 8.68(2) MeV T_1/2=0.35+0.23/-0.16}$ s ). Therefore, we compare the data presented for Md-244 by Pore et al. with those reported for Md-245 by Ninov et al. and also by Khuyagbaatar et al.. We conclude that the data presented by Pore et al. shall be attributed to Md-245 with small contributions (one event each) from Fm-245 and probably Md-246.

nucl-ex↗

arXiv2020

Optically Enhanced Electric Field Sensing Using Nitrogen-Vacancy Ensembles

Nitrogen-vacancy (NV) centers in diamond have shown promise as inherently localized electric-field sensors, capable of detecting individual charges with nanometer resolution. Working with NV ensembles, we demonstrate that a detailed understanding of the internal electric field environment enables enhanced sensitivity in the detection of external electric fields. We follow this logic along two complementary paths. First, using excitation tuned near the NV's zero-phonon line, we perform optically detected magnetic resonance (ODMR) spectroscopy at cryogenic temperatures in order to precisely measure the NV center's excited-state susceptibility to electric fields. In doing so, we demonstrate that the characteristically observed contrast inversion arises from an interplay between spin-selective optical pumping and the NV centers' local charge distribution. Second, motivated by this understanding, we propose and analyze a novel scheme for optically-enhanced electric-field sensing using NV ensembles; we estimate that our approach should enable order of magnitude improvements in the DC electric-field sensitivity.

quant-ph↗

arXiv2017

Unsupervised Machine Learning on a Hybrid Quantum Computer

Machine learning techniques have led to broad adoption of a statistical model of computing. The statistical distributions natively available on quantum processors are a superset of those available classically. Harnessing this attribute has the potential to accelerate or otherwise improve machine learning relative to purely classical performance. A key challenge toward that goal is learning to hybridize classical computing resources and traditional learning techniques with the emerging capabilities of general purpose quantum processors. Here, we demonstrate such hybridization by training a 19-qubit gate model processor to solve a clustering problem, a foundational challenge in unsupervised learning. We use the quantum approximate optimization algorithm in conjunction with a gradient-free Bayesian optimization to train the quantum machine. This quantum/classical hybrid algorithm shows robustness to realistic noise, and we find evidence that classical optimization can be used to train around both coherent and incoherent imperfections.

quant-ph↗

arXiv2017

Parametrically Activated Entangling Gates Using Transmon Qubits

We describe and implement a family of entangling gates activated by radio-frequency flux modulation applied to a tunable transmon that is statically coupled to a neighboring transmon. The effect of this modulation is the resonant exchange of photons directly between levels of the two-transmon system, obviating the need for mediating qubits or resonator modes and allowing for the full utilization of all qubits in a scalable architecture. The resonance condition is selective in both the frequency and amplitude of modulation and thus alleviates frequency crowding. We demonstrate the use of three such resonances to produce entangling gates that enable universal quantum computation: one iSWAP gate and two distinct controlled Z gates. We report interleaved randomized benchmarking results indicating gate error rates of 6% for the iSWAP (duration 135ns) and 9% for the controlled Z gates (durations 175 ns and 270 ns), limited largely by qubit coherence.

quant-ph↗

arXiv2017

Demonstration of Universal Parametric Entangling Gates on a Multi-Qubit Lattice

We show that parametric coupling techniques can be used to generate selective entangling interactions for multi-qubit processors. By inducing coherent population exchange between adjacent qubits under frequency modulation, we implement a universal gateset for a linear array of four superconducting qubits. An average process fidelity of $\mathcal{F}=93\%$ is estimated for three two-qubit gates via quantum process tomography. We establish the suitability of these techniques for computation by preparing a four-qubit maximally entangled state and comparing the estimated state fidelity against the expected performance of the individual entangling gates. In addition, we prepare an eight-qubit register in all possible bitstring permutations and monitor the fidelity of a two-qubit gate across one pair of these qubits. Across all such permutations, an average fidelity of $\mathcal{F}=91.6\pm2.6\%$ is observed. These results thus offer a path to a scalable architecture with high selectivity and low crosstalk.

quant-ph↗

arXiv2017

High-precision mass measurements for the isobaric multiplet mass equation at A = 52

Masses of $^{52}$Co, $^{52}$Co$^m$, $^{52}$Fe, $^{52}$Fe$^m$, and $^{52}$Mn have been measured with the JYFLTRAP double Penning trap mass spectrometer. Of these, $^{52}$Co and $^{52}$Co$^m$ have been experimentally determined for the first time and found to be more bound than predicted by extrapolations. The isobaric multiplet mass equation for the $T=2$ quintet at $A=52$ has been studied employing the new mass values. No significant breakdown (beyond the $3\sigma$ level) of the quadratic form of the IMME was observed ($\chi^2/n=2.4$). The cubic coefficient was 6.0(32) keV ($\chi^2/n=1.1$). The excitation energies for the isomer and the $T=2$ isobaric analogue state in $^{52}$Co have been determined to be 374(13) keV and 2922(13) keV, respectively. The $Q$ value for the proton decay from the $19/2^-$ isomer in $^{53}$Co has been determined with an unprecedented precision, $Q_{p} = 1558.8(17)$ keV. The proton separation energies of $^{52}$Co and $^{53}$Ni relevant for the astrophysical rapid proton capture process have been experimentally determined for the first time. \end{abstract}

nucl-ex↗

arXiv2016

Direct determination of the atomic mass difference of Re187 and Os187 for neutrino physics and cosmochronology

For the first time a direct determination of the atomic mass difference of 187Re and 187Os has been performed with the Penning-trap mass spectrometer SHIPTRAP applying the novel phase-imaging ion-cyclotron-resonance technique. The obtained value of 2492(30stat)(15sys) eV is in excellent agreement with the Q values determined indirectly with microcalorimetry and thus resolves a long-standing discrepancy with older proportional counter measurements. This is essential for the determination of the neutrino mass from the beta-decay of 187Re as planned in future microcalorimetric measurements. In addition, an accurate mass difference of 187Re and 187Os is also important for the assessment of 187Re for cosmochronology.

nucl-ex↗

arXiv2016

Direct Measurement of the Mass Difference of Ho163 and Dy163 Solves the Q-Value Puzzle for the Neutrino Mass Determination

The atomic mass difference of 163Ho and 163Dy has been directly measured with the Penning trap mass spectrometer SHIPTRAP applying the novel phase imaging ion cyclotron resonance technique. Our measurement has solved the long standing problem of large discrepancies in the Q value of the electron capture in 163Ho determined by different techniques. Our measured mass difference shifts the current Q value of 2555(16) eV evaluated in the Atomic Mass Evaluation 2012 [G. Audi et al., Chin. Phys. C 36, 1157 (2012)] by more than 7 sigma to 2833(30stat)(15sys) eV/c2. With the new mass difference it will be possible, e.g., to reach in the first phase of the ECHo experiment a statistical sensitivity to the neutrino mass below 10 eV, which will reduce its present upper limit by more than an order of magnitude.

physics.ins-det↗

arXiv2015

Extending the applicability of an open-ring trap to perform experiments with a single laser-cooled ion

An open-ring ion trap, also referred to as transparent trap was initially built up to perform $\beta$-$\nu$ correlation experiments with radioactive ions. This trap geometry is also well suited to perform experiments with laser-cooled ions, serving for the development of a new type of Penning trap, in the framework of the project TRAPSENSOR at the University of Granada. The goal of this project is to use a single $^{40}$Ca$^+$ ion as detector for single-ion mass spectrometry. Within this project and without any modification to the initial electrode configuration, it was possible to perform Doppler cooling on $^{40}$Ca$^+$ ions, starting from large clouds and reaching single ion sensitivity. This new feature of the trap might be important also for other experiments with ions produced at Radioactive Ion Beam (RIB) facilities. In this publication, the trap and the laser system will be described, together with their performance with respect to laser cooling applied to large ion clouds down to a single ion.

physics.ins-det↗

arXiv2015

Recoil-alpha-fission and recoil-alpha-alpha-fission events observed in the reaction Ca-48 + Am-243

Products of the fusion-evaporation reaction Ca-48 + Am-243 were studied with the TASISpec set-up at the gas-filled separator TASCA at the GSI Helmholtzzentrum f\"ur Schwerionenforschung. Amongst the detected thirty correlated alpha-decay chains associated with the production of element Z=115, two recoil-alpha-fission and five recoil-alpha-alpha-fission events were observed. The latter are similar to four such events reported from experiments performed at the Dubna gas-filled separator. Contrary to their interpretation, we propose an alternative view, namely to assign eight of these eleven decay chains of recoil-alpha(-alpha)-fission type to start from the 3n-evaporation channel 115-288. The other three decay chains remain viable candidates for the 2n-evaporation channel 115-289.

nucl-ex↗

arXiv2014

Direct mapping of nuclear shell effects in the heaviest elements

Quantum-mechanical shell effects are expected to strongly enhance nuclear binding on an "island of stability" of superheavy elements. The predicted center at proton number $Z=114,120$, or $126$ and neutron number $N=184$ has been substantiated by the recent synthesis of new elements up to $Z=118$. However the location of the center and the extension of the island of stability remain vague. High-precision mass spectrometry allows the direct measurement of nuclear binding energies and thus the determination of the strength of shell effects. Here, we present such measurements for nobelium and lawrencium isotopes, which also pin down the deformed shell gap at $N=152$.

nucl-ex↗

arXiv2012

Q value and half-life of double-electron capture in Os-184

Os-184 has been excluded as a promising candidate for the search of neutrinoless double-electron capture. High-precision mass measurements with the Penning-trap mass spectrometer TRIGA-TRAP resulted in a marginal resonant enhancement with = -8.89(58) keV excess energy to the 1322.152(22) keV 0+ excited state in W-184. State-of-the-art energy density functional calculations are applied for the evaluation of the nuclear matrix elements to the excited states predicting a strong suppression due to the large deformation of mother and daughter states. The half-life of the transition in Os-184 exceeds T_{1/2} > 1.3 10^{29} years for an effective neutrino mass of 1 eV.

nucl-ex↗

arXiv2012

Direct mass measurements of cadmium and palladium isotopes and their double-beta transition Q-values

The Q-value of the double-electron capture in Cd-108 has been determined to be (272.04 +/- 0.55) keV in a direct measurement with the double-Penning trap mass spectrometer TRIGA-TRAP. Based on this result a resonant enhancement of the decay rate of Cd-108 is excluded. We have confirmed the double-beta transition Q-values of Cd-106 and Pd-110 recently measured with the Penning-trap mass spectrometers SHIPTRAP and ISOLTRAP, respectively. Furthermore, the atomic masses of the involved nuclides Cd-106, Cd-108, Cd-110, Pd-106, Pd-108 and Pd-110 have been directly linked to the atomic mass standard.

nucl-ex↗

arXiv2011

Probing the nuclide 180W for neutrinoless double-electron capture exploration

The mass difference of the nuclides 180W and 180Hf has been measured with the Penning-trap mass spectrometer SHIPTRAP to investigate 180W as a possible candidate for the search for neutrinoless doubleelectron capture. The Q-value was measured to 143.20(27)keV. This value in combination with the calculations of the atomic electron wave functions and other parameters results in a half-life of the 0+ \rightarrow 0+ ground-state to ground-state double-electron capture transition of approximately 5\cdot10E27 years/ ^2.

nucl-ex↗

arXiv2011

Mass measurements of very neutron-deficient Mo and Tc isotopes and their impact on rp process nucleosynthesis

The masses of ten proton-rich nuclides, including the N=Z+1 nuclides 85-Mo and 87-Tc, were measured with the Penning trap mass spectrometer SHIPTRAP. Compared to the Atomic Mass Evaluation 2003 a systematic shift of the mass surface by up to 1.6 MeV is observed causing significant abundance changes of the ashes of astrophysical X-ray bursts. Surprisingly low alpha-separation energies for neutron-deficient Mo and Tc are found, making the formation of a ZrNb cycle in the rp process possible. Such a cycle would impose an upper temperature limit for the synthesis of elements beyond Nb in the rp process.

nucl-ex↗

arXiv2010

Dust formation in the ejecta of the Type II-P supernova 2004dj

Core-collapse supernovae (CC SNe), especially Type II-Plateau ones, are thought to be important contributors to cosmic dust production. SN 2004dj, one of the closest and brightest SN since 1987A, offered a good opportunity to examine dust formation processes. To find signs of newly formed dust, we analyze all available mid-infrared (MIR) archival data from the Spitzer Space Telescope. We re-reduce and analyze data from IRAC, MIPS and IRS instruments obtained between +98 and +1381 days after explosion, generating light curves and spectra for each epoch. Observed spectral energy distributions are fitted with both analytic and numerical models, using the radiative-transfer code MOCASSIN for the latter ones. We also use imaging polarimetric data obtained at +425 days by the Hubble Space Telescope. We present convincing evidence of dust formation in the ejecta of SN 2004dj from MIR light curves and spectra. Significant MIR excess flux is detected in all bands between 3.6 and 24 um. In the optical, a ~0.8% polarization is also detected at a 2-sigma level, which exceeds the interstellar polarization in that direction. Our analysis shows that the freshly-formed dust around SN 2004dj can be modeled assuming a nearly spherical shell containing amorphous carbon grains, cooling from ~700 K to ~400 K between +267 and +1246 days. Persistent excess flux has been found above 10 um, which is explained by a cold (~115 K) dust component. If this cold dust is of circumstellar origin, it is likely to be condensed in a cool, dense shell between the forward and reverse shocks. Pre-existing circumstellar dust is less likely, but cannot be ruled out. An upper limit of ~8x10^{-4} M_sun was derived for the dust mass, which is similar to previously published values for other dust-producing SNe.

astro-ph.SR↗

arXiv2010

An Aromatic Inventory of the Local Volume

Using infrared photometry from the Spitzer Space Telescope, we perform the first inventory of aromatic feature emission (AFE, but also commonly referred to as PAH emission) for a statistically complete sample of star-forming galaxies in the local volume. The photometric methodology involved is calibrated and demonstrated to recover the aromatic fraction of the IRAC 8 micron flux with a standard deviation of 6% for a training set of 40 SINGS galaxies (ranging from stellar to dust dominated) with both suitable mid-infrared Spitzer IRS spectra and equivalent photometry. A potential factor of two improvement could be realized with suitable 5.5 and 10 micron photometry, such as what may be provided in the future by JWST. The resulting technique is then applied to mid-infrared photometry for the 258 galaxies from the Local Volume Legacy (LVL) survey, a large sample dominated in number by low-luminosity dwarf galaxies for which obtaining comparable mid-infrared spectroscopy is not feasible. We find the total LVL luminosity due to five strong aromatic features in the 8 micron complex to be 2.47E10 solar luminosities with a mean volume density of 8.8E6 solar luminosities per cubic Megaparsec. Twenty-four of the LVL galaxies, corresponding to a luminosity cut at M = -18.22 in the B band, account for 90% of the aromatic luminosity. Using oxygen abundances compiled from the literature for 129 of the 258 LVL galaxies, we find a correlation between metallicity and the aromatic to total infrared emission ratio but not the aromatic to total 8 micron dust emission ratio. A possible explanation is that metallicity plays a role in the abundance of aromatic molecules relative to the total dust content, but other factors such as star formation and/or the local radiation field affect the excitation of those molecules.

astro-ph.CO↗