arXiv subjects

M. Zalewski

Publications and source records attributed to M. Zalewski.

13 recordsLinked to original sources

arXiv2017

Dynamics in poly(propylene glycol) and silica oxide nanoparticles composite glassforming system

Results of broadband dielectric spectroscopy and rheological studies of poly(propylene glycol) + SiO${_2}$ nanocomposites are presented. They show that the dynamics in high-concentrated composite is determined by confinement and adsorption effects, resulting from interactions of confined polymers correspond with the host system at the interface between PPG and solid nanoparticles. The evolution of relaxation times follows the clear Vogel-Fulcher-Tammann pattern, what is proved by the supplementary activation energy temperature index analysis. The strong influence of nanoparticles on the transitional dynamics and the fragility in the ultraviscous domain was noted.

cond-mat.soft↗

arXiv2010

Surface-peaked effective mass in the nuclear energy density functional and its influence on single-particle spectra

Calculations for infinite nuclear matter with realistic nucleon-nucleon interactions suggest that the isoscalar effective mass of a nucleon at the saturation density, m*/m, equals 0.8 +/- 0.1. This result is at variance with empirical data on the level density in finite nuclei, which are consistent with m*/m ~ 1. Ma and Wambach suggested that these two contradicting results may be reconciled within a single theoretical framework by assuming a radial-dependent effective mass, peaked at the nuclear surface. The aim of this exploratory work is to investigate this idea within the density functional theory by using a Skyrme-type local functional enriched with new terms, $τ(\mathbf{\nabla}ρ)^2$ and $τ\frac{dρ}{dr}$, where $τ$ and $ρ$ denote the kinetic and particle densities, respectively. We show that each of these terms can give rise to a surface peak in the effective mass, but of a limited height. We investigate the influence of the radial profile of the effective mass on the spin-orbit splittings and centroids. In particular, we demonstrate that the $τ\frac{dρ}{dr}$ term quenches the 1f5/2-1f7/2 splitting in 40Ca, which is strongly overestimated within conventional Skyrme parametrizations.

nucl-th↗

arXiv2009

Global nuclear structure effects of tensor interaction

A direct fit of the isoscalar spin-orbit (SO) and both isoscalar and isovector tensor coupling constants to the f5/2-f7/2 SO splittings in 40Ca, 56Ni, and 48Ca nuclei requires a drastic reduction of the isoscalar SO strength and strong attractive tensor coupling constants. The aim of this work is to address further consequences of these strong attractive tensor and weak SO fields on binding energies, nuclear deformability, and high-spin states. In particular, we show that contribution to the nuclear binding energy due to the tensor field shows generic magic structure with tensorial magic numbers at N(Z)=14, 32, 56, or 90 corresponding to the maximum spin-asymmetries in 1d5/2, 1f7/2-2p3/2, 1g9/2-2d5/2 and 1h11/2-2f7/2 single-particle configurations and that these numbers are smeared out by pairing correlations and deformation effects. We also examine the consequences of strong attractive tensor fields and weak SO interaction on nuclear stability at the drip lines, in particular close to the tensorial doubly magic nuclei and discuss the possibility of an entirely new tensor-force driven deformation effect.

nucl-th↗

arXiv2009

The nuclear energy density functionals with modified radial dependence of the isoscalar effective mass

Calculations for infinite nuclear matter with realistic nucleon-nucleon interactions suggest that the isoscalar effective mass (IEM) of a nucleon at the saturation density equals $m^*/m\sim 0.8\pm 0.1$, at variance with empirical data on the nuclear level density in finite nuclei which are consistent with $m^*/m\approx 1$. This contradicting results might be reconciled by enriching the radial dependence of IEM. In this work four new terms are introduced into the Skyrme-force inspired local energy-density functional: $\tau(\nabla\rho)^2$, $\tau\frac{d\rho}{dr}$, $\tau^2$ and $\tau\Delta\rho$. The aim is to investigate how they influence the radial dependence of IEM and, in turn, the single-particle spectra.

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arXiv2009

HFODD (v2.40h) User's Guide

We describe the input data and installation procedures of the code HFODD (v2.40h). The present write-up contains complete and comprehensive information that has originally been given in six independent publications. It is enhanced by the subject index and indexes of variables, input-data keywords, subroutines, and files that are used in this user guide.

nucl-th↗

arXiv2009

Solution of the Skyrme-Hartree-Fock-Bogolyubov equations in the Cartesian deformed harmonic-oscillator basis. (VI) HFODD (v2.38j): a new version of the program

We describe the new version (v2.38j) of the code HFODD which solves the nuclear Skyrme-Hartree-Fock or Skyrme-Hartree-Fock-Bogolyubov problem by using the Cartesian deformed harmonic-oscillator basis. In the new version, we have implemented: (i) projection on good angular momentum (for the Hartree-Fock states), (ii) calculation of the GCM kernels, (iii) calculation of matrix elements of the Yukawa interaction, (iv) the BCS solutions for state-dependent pairing gaps, (v) the HFB solutions for broken simplex symmetry, (vi) calculation of Bohr deformation parameters, (vii) constraints on the Schiff moments and scalar multipole moments, (viii) the D2h transformations and rotations of wave functions, (ix) quasiparticle blocking for the HFB solutions in odd and odd-odd nuclei, (x) the Broyden method to accelerate the convergence, (xi) the Lipkin-Nogami method to treat pairing correlations, (xii) the exact Coulomb exchange term, (xiii) several utility options, and we have corrected two insignificant errors.

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arXiv2008

Shell-structure fingerprints of tensor interaction

We address consequences of strong tensor and weak spin-orbit terms in the local energy density functional, resulting from fits to the $f_{5/2} - f_{7/2}$ splittings in $^{40}$Ca, $^{48}$Ca, and $^{56}$Ni. In this study, we focus on nuclear binding energies. In particular, we show that the tensor contribution to the binding energies exhibits interesting topological features closely resembling that of the shell-correction. We demonstrate that in the extreme single-particle scenario at spherical shape, the tensor contribution shows tensorial magic numbers equal to $N(Z)$=14, 32, 56, and 90, and that this structure is smeared out due to configuration mixing caused by pairing correlations and migration of proton/neutron sub-shells with neutron/proton shell filling. Based on a specific Skyrme-type functional SLy4$_T$, we show that the proton tensorial magic numbers shift with increasing neutron excess to $Z$=14, 28, and 50.

nucl-th↗

arXiv2008

Global nuclear structure aspects of tensor interaction

A direct fit of the isoscalar spin-orbit and both isoscalar and isovector tensor coupling constants to the f5/2-f7/2 SO splittings in 40Ca, 56Ni, and 48Ca requires: (i) a significant reduction of the standard isoscalar spin-orbit strength and (ii) strong attractive tensor coupling constants. The aim of this paper is to address the consequences of these strong attractive tensor and weak spin-orbit fields on total binding energies, two-neutron separation energies and nuclear deformability.

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arXiv2008

Contradicting effective mass scalings within the Skyrme energy density functional method

The problem of the effective mass scaling in the single particle spectra calculated within the Skyrme energy density functional (EDF) method is studied. It is demonstrated that for specific pairs of orbitals the commonly anticipated isoscalar effective mass (m*) scaling of the single-particle level splittings is almost canceled by an implicit m*-scaling due to other parameters in the Skyrme EDF. This holds in particular for an indirect m*-scaling of the two-body spin-orbit strength making the theory essentially unpredictable with respect to single particle energies. It is argued that this unphysical property of the Skyrme EDF is a mere consequence of the strategies and datasets used to fit these functionals. The inclusion of certain single-particle spin-orbit splittings to fit the two-body spin-orbit and the tensor interaction strengths reinstates the conventional m*-scaling and improves the performance of the Skyrme EDF.

nucl-th↗

arXiv2008

Spin-orbit and tensor mean-field effects on spin-orbit splitting including self-consistent core polarizations

A new strategy of fitting the coupling constants of the nuclear energy density functional is proposed, which shifts attention from ground-state bulk to single-particle properties. The latter are analyzed in terms of the bare single-particle energies and mass, shape, and spin core-polarization effects. Fit of the isoscalar spin-orbit and both isoscalar and isovector tensor coupling constants directly to the f5/2-f7/2 spin-orbit splittings in 40Ca, 56Ni, and 48Ca is proposed as a practical realization of this new programme. It is shown that this fit requires drastic changes in the isoscalar spin-orbit strength and the tensor coupling constants as compared to the commonly accepted values but it considerably and systematically improves basic single-particle properties including spin-orbit splittings and magic-gap energies. Impact of these changes on nuclear binding energies is also discussed.

nucl-th↗

arXiv2007

Terminating states as a unique laboratory for testing nuclear energy density functional

Systematic calculations of favored signature maximum-spin I_max and unfavored signature I_max - 1 terminating states for [f 7/2 ^ n] and [d 3/2 ^ (-1) f 7/2 ^ (n+1)] configurations (n denotes number of valence particles) in A ~ 44 mass region are presented. Following the result of Zdunczuk et al., Phys. Rev. C71 (2005) 024305 the calculations are performed using Skyrme energy density functional with empirical Landau parameters and slightly reduced spin-orbit strength. The aim is to identify and phenomenologically restore rotational symmetry broken by the Skyrme-Hartree-Fock solutions. In particular, it is shown that correlation energy due to symmetry restoration is absolutely crucial in order to reproduce energy splitting E(I_max) - E(I_max -1) in [f 7/2 ^ n] configurations but is relatively less important for [d 3/2 ^ (-1) f 7/2 ^ (n+1)] configurations.

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arXiv2007

Shell Model and Mean-Field Description of Band Termination

We study nuclear high-spin states undergoing the transition to the fully stretched configuration with maximum angular momentum I_max within the space of valence nucleons. To this end, we perform a systematic theoretical analysis of non-fully-stretched I_max-2 and I_max-1 f_{7/2}^n seniority isomers and d_{3/2}^{-1} f_{7/2}^{n+1} intruder states in the A~44 nuclei from the lower-fp shell. We employ two theoretical approaches: (i) the density functional theory based on the cranked self-consistent Skyrme-Hartree-Fock method, and (ii) the nuclear shell model in the full sdfp configuration space allowing for 1p-1h cross-shell excitations. We emphasize the importance of restoration of broken angular momentum symmetry inherently obscuring the mean-field treatment of high-spin states. Overall good agreement with experimental data is obtained.

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arXiv2005

High-spin intruder states in the fp shell nuclei and isoscalar proton-neutron correlations

We perform a systematic shell-model and mean-field study of fully-aligned, high-spin f_{7/2}^{n} seniority isomers and d_{3/2}^{-1} f_{7/2}^{n+1} intruder states in the A~44 nuclei from the lower-fp shell. The shell-model calculations are performed in the full sdfp configuration space allowing 1p-1h cross-shell excitations. The self-consistent mean-field calculations are based on the Hartree-Fock approach with the Skyrme energy density functional that reproduces empirical Landau parameters. While there is a nice agreement between experimental and theoretical relative energies of fully-aligned states in N>Z nuclei, this is no longer the case for the N=Z systems. The remaining deviation from the data is attributed to the isoscalar proton-neutron correlations. It is also demonstrated that the Coulomb corrections at high spins noticeably depend on the choice of the energy density functional.

nucl-th↗