arXiv subjects

Mathieu Bertrand

Publications and source records attributed to Mathieu Bertrand.

At least 19 recordsLinked to original sources

arXiv2025

Free-Running Ring Quantum Cascade Laser with 50 kHz Linewidth

We report on the noise characterization of a free-running ring quantum cascade laser resonator emitting a single frequency mode around 7.7 $\mu$m. Using a gas cell filled with N$_2$O as a frequency-to-voltage discriminator, we measured the frequency noise power spectral density of the laser from which we extracted its linewidth. The results show a full width at half maximum close to 50 kHz at 1 s integration time, which represents at least a sixfold improvement compared to state-of-the-art quantum cascade lasers operating in a spectral region above 7 $\mu$m. We also demonstrate that such lasers can be efficiently used for frequency modulation spectroscopy, which opens up new possibilities for high resolution metrology and spectroscopic applications in the mid-infrared.

physics.optics↗

arXiv2025

Towards a Global Scale Quantum Information Network: A Study Applied to Satellite-Enabled Distributed Quantum Computing

Recent developments have reported on the feasibility of interconnecting small quantum registers in a quantum information network of a few meter-scale for distributed quantum computing purposes. This multiple small-scale quantum processors communicating and cooperating to execute computational tasks is considered as a promising solution to the scalability problem of reaching more than thousands of noise-free qubits. Here, we propose and assess a satellite-enabled distributed quantum computing system at the French national scale, based on existing infrastructures in Paris and Nice. We consider a system composed of both a ground and a space segment, allowing for the distribution of end-to-end entanglement between Alice in Paris and Bob in Nice, each owning a few-qubit processor composed of trapped ions. In the context of quantum computing, this entanglement resource can be used for the teleportation of a qubit state or for gate teleportation. We numerically assess the entanglement distribution rate and fidelity generated by this space-based quantum information network, and discuss concrete use cases and service performance levels in the framework of distributed quantum computing.

quant-ph↗

arXiv2025

Time-resolved spectroscopy of noise-driven collective states of light

We study a collective liquid state of light in a fast-gain laser. Controlled temporal noise on the cavity modulation creates a fluctuating linear potential along the synthetic frequency lattice of the cavity modes. We identify three regimes of lattice occupation as noise increases: an extended distribution, a Gaussian envelope, and exponential localization. Time-resolved spectroscopy on single realizations of noise reveals distinct dynamics in the latter two: transport persists in the Gaussian regime, modulated by the fluctuating potential, but is fully suppressed at all times in the localized regime. Averaging over many noise realizations shows that noise reduces the transport speed and confirms ergodicity of the system.

physics.optics↗

arXiv2025

The Role of the Satellite in Quantum Information Networks

Quantum Information Networks (QIN) attract increasing interest, as they will enable interconnection of multiple quantum devices in a distributed organization thus enhancing intrinsic computing, sensing, and security capabilities. The core mechanism of a QIN is quantum state swapping, based on teleportation, which consumes quantum entanglement, and which can be seen in this context as a new kind of network resource. The satellite is expected to play a central role for supporting global connectivity in such novel networks in which ground fiber links have stringent restrictions in length due to the absorption losses in optical fibers. There is indeed fundamental limits in the maximal fiber links distance which may not be exceeded for any unitary links. In this paper we clarify our motivations to develop such networks with satellites, and we discuss their associated use cases based on entanglement distribution, and we present the future potential users. We also assess quantitatively the ranges for which the satellite becomes mandatory in quantum information networks.

quant-ph↗

arXiv2025

On-chip pulse generation at 8 {\mu}m wavelength

The mid-infrared spectral region holds growing importance for applications such as gas sensing and spectroscopy. Although compact ultrashort pulse laser sources are essential to enable these applications, their realization in this spectral range remains an open challenge. We demonstrate an integrated approach to generate pulses in the mid-infrared based on chirped Bragg gratings engineered to compensate for the group delay dispersion of quantum cascade laser frequency comb sources. SiGe graded-index photonic circuits are used for operation around 8 {\mu}m wavelength. With this approach, pulses as short as 1.39 picoseconds were obtained, marking a key step towards fully integrated ultrashort pulse sources in the mid-infrared.

physics.optics↗

arXiv2025

Integrated thin film lithium niobate mid-infrared modulator

The mid-infrared spectral range holds great promise for applications such as molecular spectroscopy and telecommunications. Many key molecules exhibit strong absorption features in this range, and free-space optical communication benefits from reduced atmospheric attenuation and low transmission losses in specific wavelength bands spanning from 3 to 14 $\mu m$. Recent progress in MIR photonics has been fuelled by the rapid development of efficient light sources and detectors. However, further advancement is hindered by the lack of low-loss, high-performance integrated photonic platforms and modulators. Lithium niobate on sapphire is a promising candidate, operating across a broad spectral range from 0.4 $\mu m$ to 4.5 $\mu m$. We demonstrate a broadband, high-speed lithium niobate on sapphire Mach-Zehnder electro-optic modulator operating from 3.95 to 4.3 $\mu m$. The device achieves a 3 dB bandwidth exceeding 20 GHz, an extinction ratio of 34 dB, and a half-wave voltage of 22 V$\cdot$cm, delivering optical output power at the half-milliwatt level. These properties are leveraged to demonstrate data transmission at 10 Gbit/s. The modulator is also used to generate a frequency comb with a width of 80 GHz. Furthermore, we demonstrate full $\pi$-phase modulation in the MIR, representing a key milestone for integrated MIR photonics. These results establish a pathway toward high-speed, energy-efficient MIR photonic systems for applications in telecommunications, sensing, and quantum technologies.

physics.optics↗

arXiv2024

Non-resonant Optical Injection Locking in Quantum Cascade Laser Frequency Combs

Optical injection locking of the repetition frequency of a quantum cascade laser frequency comb is demonstrated using an intensity modulated near-infrared light at 1.55 $\mu$m illuminating the front facet of the laser. Compared to the traditional electrical modulation approach, the introduced technique presents benefits from several perspectives such as the availability of mature and high bandwidth equipment in the near-infrared, circumvent the need of dedicated electronic components for the quantum cascade laser, and allows a direct link between the near and mid-infrared for amplitude to frequency modulation. We show that this stabilization scheme, used with moderate near-infrared power of a few milliwatts, allows for a strong reduction of the frequency noise. We also perform a full characterization of the mechanism and evidence that the locking range follows Adler's law. A comparison of our results with those in recent literature indicates that the optical approach leads to better performance compared to the traditional method, which we expect to benefit mid-infrared spectroscopy and metrological applications.

physics.optics↗

arXiv2024

A Quantum Walk Comb Source at Telecommunication Wavelengths

We demonstrate a quantum walk comb in synthetic frequency space formed by externally modulating a semiconductor optical amplifier operating in the telecommunication wavelength range in a unidirectional ring cavity. The ultrafast gain saturation dynamics of the gain medium and its operation at high current injections is responsible for the stabilization of the comb in a broad frequency modulated state. Our device produces a nearly flat broadband comb with a tunable repetition frequency reaching a bandwidth of 1.8THz at the fundamental repetition rate of 1GHz while remaining fully locked to the RF drive. Comb operation at harmonics of the repetition rate up to 14.1GHz is also demonstrated. This approach paves the way for next-generation optical frequency comb devices with potential applications in precision ranging and high-speed communications.

physics.optics↗

arXiv2024

Shot-noise-limited emission from interband and quantum cascade lasers

The intensity noise of a laser source represents one of the key factors limiting the ultimate sensitivity in laser-based systems for sensing and telecommunication. For advanced applications based on interferometry, the availability of a shot-noise-limited local oscillator is even more important for the effective feasibility of high-precision measurements. This is particularly crucial in quantum optics applications based on homodyne detection schemes to measure non-classical light states, such as squeezed states. This work deeply investigates and analyzes the intensity noise features of the most widely used mid-infrared semiconductor heterostructured lasers: quantum cascade and interband cascade lasers. For this purpose, a comprehensive comparison of three different continuous-wave lasers operating at room temperature around 4.5 {\mu}m wavelength is presented. First, a thorough electro-optical characterization is given, highlighting the differences and the shared common characteristics of the tested devices. Then, a detailed intensity noise analysis is reported, identifying their different noise operations with a particular reference to shot-noise-limited operations. Finally, some perspectives towards advanced applications are discussed.

physics.optics↗

arXiv2024

Quench dynamics of Wannier-Stark states in an active synthetic photonic lattice

Photonic emulators have facilitated the investigation of numerous solid-state phenomena and have contributed to the development of optical devices inspired by quantum mechanics. Although current photonic emulators are constrained to bosonic behavior with local interactions, the utilization of active synthetic lattices holds promise for surpassing these limitations. In this study, we propose employing the modulated ring fast-gain laser as a foundation for emulating quench dynamics within a synthetic lattice that conforms to equal density filling of its reciprocal space. To illustrate the effectiveness of this emulation platform, we subject a dispersed Wannier-Stark ladder to quenching and directly observe oscillations, enabled by the fast-gain, along with their coherent stabilization to a single Wannier stark state. These coherent dynamics stem directly from our lasers liquid state of light, a characteristic resulting from fast-gain and explained by the rapid decay of fluctuations occurring on the system's shortest timescale. Additionally, by adequately biasing the lattice through detuning the modulation from the cavity resonance, this process supports oscillatory dynamics within the synthetic space.

physics.optics↗

arXiv2023

Quantum Cascade Lasers as Broadband Sources via Strong RF Modulation

In this work, we demonstrate that in a regime of strong modulation, by generating pulses of the length of the order of a few cavity lifetimes (hundreds of ps), a broadband quantum cascade laser can be driven to lase on a bandwidth (250cm-1) limited by the gain. In addition, the amplitude noise of the radiation was shown to be limited by the detector. A laser linewidth study has been performed under different operating conditions finding values spanning from 20MHz to 800MHz, indicating a trade-off between emission bandwidth, amplitude stability and coherence.

physics.optics↗

arXiv2023

Coherence analysis of tightly locked mid-infrared quantum cascade laser frequency combs

Frequency combs are powerful tools for many applications and high performances are achieved by stabilizing these lasers. For operation in the mid-infrared, quantum cascade lasers (QCL) are ideal candidates as they present numerous advantages. However, stabilized QCL-combs lack of a detailed characterization of their noise properties due to the sensitivity limits of current analyzing techniques. To overcome these challenges, we developed what we believe to be the first tightly locked dual QCL-comb system. Its use is twofold. First, phase noise analysis of the dual-comb signal shows residual phase noise below 600 mrad for all comb lines, and we characterize the comb coherence as well as the performances of the repetition frequency locking mechanism. Second, we demonstrate coherent averaging with a $7 \times 10^5$ Hz$^{1/2}$ figure-of-merit system, which is compatible with high precision spectroscopy.

physics.optics↗

arXiv2023

Quantum Walk Comb in a Fast Gain Laser

Synthetic lattices in photonics enable the exploration of light states in new dimensions, transcending phenomena common only to physical space. We propose and demonstrate a Quantum Walk Laser in synthetic frequency space formed by externally modulating a ring-shaped semiconductor laser with ultrafast recovery times. In this device, the initially ballistic quantum walk does not dissipate into low supermode states of the synthetic lattice; instead, thanks to the fast-gain nonlinearity of our quantum cascade laser active material, the state stabilizes in a broad frequency comb, unlocking the full potential of the lattice. This device produces a low-noise, nearly-flat broadband comb (reaching 100 cm$^{-1}$ bandwidth), well predicted by our models. The proposed Quantum Walk Laser offers a promising platform to generate broadband, tunable and stable frequency combs.

physics.optics↗

arXiv2023

Quantum Cascade Surface Emitting Lasers

A low-cost single frequency laser emitting in the mid-infrared spectral region and dissipating minimal electrical power is a key ingredient for the next generation of portable gas sensors for high-volume applications involving chemical sensing of important greenhouse and pollutant gases. We propose here a Quantum Cascade Surface Emitting Laser (QCSEL), which we implement as a short linear cavity with high reflectivity coated end-mirrors to suppress any edge emission and use a buried semiconductor diffraction grating to extract the light from the surface. By wafer-level testing we investigate the cavity length scaling, extract mirror reflectivities larger than 0.9, and achieve a pulsed threshold power dissipation of 237 mW for an emission wavelength near 7.5 $\mu$m. Finally, we demonstrate single mode emission with a side-mode suppression ratio larger than 33 dB of a 248 $\mu$m short cavity mounted with the epitaxial layer up and operated in continuous wave at 20 $^\circ$C.

physics.optics↗

arXiv2023

Coherent Control of Mid-Infrared Frequency Comb by Optical Injection of Near-Infrared Light

We demonstrate the use of a low power near-infrared laser illuminating the front facet of a quantum cascade laser (QCL) as an optical actuator for the coherent control of a mid-infrared frequency comb. We show that by appropriate current control of the QCL comb and intensity modulation of the near-infrared laser, a tight phase lock of a comb line to a distributed feedback laser is possible with 2 MHz of locking bandwidth and 200 mrad of residual phase noise. A characterization of the whole scheme is provided showing the limits of the electrical actuation which we bypassed using the optical actuation. Both comb degrees of freedom can be locked by performing electrical injection locking of the repetition rate in parallel. However, we show that the QCL acts as a fast near-infrared light detector such that injection locking can also be achieved through modulation of the near-infrared light. These results on the coherent control of a quantum cascade laser frequency comb are particularly interesting for coherent averaging in dual-comb spectroscopy and for mid-infrared frequency comb applications requiring high spectral purity.

physics.optics↗

arXiv2022

Sensitive dependence of the linewidth enhancement factor on electronic quantum effects in quantum cascade lasers

The linewidth enhancement factor (LEF) describes the coupling between amplitude and phase fluctuations in a semiconductor laser, and has recently been shown to be a crucial component for frequency comb formation in addition to linewidth broadening. It necessarily arises from causality, as famously formulated by the Kramers-Kronig relation, in media with non-trivial dependence of the susceptibility on intensity variations. While thermal contributions are typically slow, and thus can often be excluded by suitably designing the dynamics of an experiment, the many quantum contributions are harder to separate. In order to understand and, ultimately, design the LEF to suitable values for frequency comb formation, soliton generation, or narrow laser linewidth, it is therefore important to systematically model all these effects. In this comprehensive work, we introduce a general scheme for computing the LEF, which we employ with a non-equilibrium Green's function model. This direct method, based on simulating the system response under varying optical intensity, and extracting the dependence of the susceptibility to intensity fluctuations, can include all relevant electronic effects and predicts the LEF of an operating quantum cascade laser to be in the range of 0.1 - 1, depending on laser bias and frequency. We also confirm that many-body effects, off-resonant transitions, dispersive (Bloch) gain, counter-rotating terms, intensity-dependent transition energy, and precise subband distributions all significantly contribute and are important for accurate simulations of the LEF.

physics.optics↗

arXiv2022

Intensity correlations in quantum cascade laser harmonic frequency combs

A novel study on harmonic frequency combs emitted by Quantum Cascade Lasers (QCLs) is here presented, demonstrating the presence of intensity correlations between twin modes characterising the emission spectra. These originate from a Four-Wave Mixing (FWM) process driven by the active medium's third-order non-linearity. The study of such correlations is essential for the engineering of a new generation of semiconductor devices with the potential of becoming integrated emitters of light with quantum properties, such as squeezing and entanglement. Starting from experimental results, the limits of state-of-the-art technology are discussed as well as the possible methodologies that could lead to the detection of non-classical phenomena, or alternatively improve the design of QCLs, in the compelling perspective of generating quantum correlations in mid-infrared light.

physics.optics↗

arXiv2022

Frequency chirped Fourier-Transform spectroscopy

Fast (sub-second) spectroscopy with high spectral resolution is of vital importance for revealing quantum chemistry kinetics of complex chemical and biological reactions. Fourier transform (FT) spectrometers can achieve high spectral resolution and operate at hundreds of ms time scales in rapid-scan mode. However, the linear translation of a scanning mirror imposes stringent time-resolution limitations to these systems, which makes simultaneous high spectral and temporal resolution impossible. Here, we demonstrate an FT spectrometer whose operational principle is based on continuous rotational, rather than linear, motion of the scanning mirror, decoupling the spectral resolution from the temporal one. This enables 0.5 cm${}^{-1}$ resolution on sub-ms time scales. Furthermore, we show that such rotational FT spectrometers can perform dual-comb spectroscopy with a single comb source, since the Doppler-shifted version of the comb serves as the second comb. In this way, we combine the advantages of dual-comb and FT spectroscopy using a single quantum cascade laser frequency comb as a light source. Our technique does not require any diffractive or dispersive optical elements and hence preserve the Jacquinot's-, Fellgett's-, and Connes'-advantages of FT spectrometers. The system supports a large optical bandwidth from visible to THz frequencies. The combination of a rotational delay line with collimated coherent or non-coherent light sources pave the way for FT spectrometers in applications where high speed, large optical bandwidth, and high spectral resolution are desired.

physics.optics↗