arXiv subjects

Matthew Toole

Publications and source records attributed to Matthew Toole.

5 recordsLinked to original sources

arXiv2026

Directional Manipulation of a Staggered Charge Density Wave and Kondo Resonance in UTe2

UTe2 is a rare example of a correlated quantum material in which unconventional density wave orders, Kondo physics, spin-triplet pairing, and reentrant superconductivity coexist within the same electronic system. Its superconducting state develops out of a strongly correlated normal phase. The identification and control of competing or intertwined normal-state orders are thus central to elucidating the electronic landscape from which its superconductivity arises. Here, using scanning tunnelling microscopy (STM) in a vector magnetic field, we uncover a previously unreported staggered charge-density-wave (CDW) in high-quality UTe2 crystals and demonstrate its strong directional response to an external magnetic field: the staggered CDW is completely quenched by a modest 1.7 T field aligned with the quasi-one-dimensional uranium chain direction (a-axis), while remaining robust against fields along other crystallographic directions. This pronounced anisotropy is consistent with an orbital-driven mechanism that leads to a field-tuned quantum phase transition. Strikingly and counterintuitively, the same field orientation and strength concomitantly alter the hybridization gap and suppress the 5f Kondo resonance. Modelling indicates that this correlated evolution arises from a switch of the dominant hybridization channel from Te 5p- U 5f to U 6d- U 5f coupling, suggesting an intimate interplay between CDW and the Kondo effect. Our work establishes an effective tuning knob for the intertwined orders in UTe2 and provides evidence for orbital-selective Kondo hybridization, shedding light on its correlated normal state.

cond-mat.str-el↗

arXiv2025

Visualizing Pair-breaking Scattering Interference in Bulk FeSe

Spatially periodic modulations of the superconducting gap have been recently reported in diverse materials and are often attributed to pair density wave order. An alternative mechanism, termed pair-breaking scattering interference (PBSI), was proposed to produce gap modulations without finite-momentum pairing. Here we investigate signatures of PBSI in bulk FeSe using scanning tunneling microscopy with superconductive tips, enabling enhanced energy resolution and Josephson tunneling. Subsurface magnetic scatterers with Yu-Shiba-Rusinov states are identified in FeSe, around which we observe particle-hole symmetric gap modulations accompanied by spatial modulation of the Josephson current. Those modulations have wavevectors consistent with intra-pocket PBSI. We further demonstrate that phase-referenced quasiparticle interference imaging offers an independent and direct probe of PBSI beyond gap mapping. These results establish PBSI as a viable origin of gap modulations in superconductors lacking preexisting charge/spin density wave orders, and motivate further investigation of the intriguing gap modulation phenomenology.

cond-mat.supr-con↗

arXiv2025

Atomic-scale Frustrated Josephson Coupling and Multi-condensate Visualization in FeSe

In a Josephson junction involving multi-band superconductors, competition between inter-band and inter-junction Josephson coupling gives rise to frustration and spatial disjunction of superfluid densities among superconducting condensates. Such frustrated coupling manifests as quantum interference of Josephson currents from different tunneling channels and becomes tunable if channel transparency can be varied. To explore these unconventional effects in the prototypical $s^\pm$-wave superconductor FeSe, we use atomic resolution scanned Josephson tunneling microscopy SJTM for condensate resolved imaging and junction tuning -- capabilities unattainable in macroscopic Josephson devices with fixed characteristics. We quantitatively demonstrate frustrated Josephson tunneling by examining two tunneling inequalities. The relative transparency of two parallel tunneling pathways is found tunable, revealing a tendency towards a 0-pi transition with decreasing SJTM junction resistance. Simultaneous visualization of both superconducting condensates reveals anti correlated superfluid modulations, highlighting the role of inter-band scattering. Our study establishes SJTM as a powerful tool enabling new research frontiers of multi condensate superconductivity.

cond-mat.supr-con↗

arXiv2025

Quasiparticle Interference Kernel Extraction with Variational Autoencoders via Latent Alignment

Quasiparticle interference (QPI) imaging is a powerful tool for probing electronic structures in quantum materials, but extracting the single-scatterer QPI pattern (i.e., the kernel) from a multi-scatterer image remains a fundamentally ill-posed inverse problem, because many different kernels can combine to produce almost the same observed image, and noise or overlaps further obscure the true signal. Existing solutions to this extraction problem rely on manually zooming into small local regions with isolated single-scatterers. This is infeasible for real cases where scattering conditions are too complex. In this work, we propose the first AI-based framework for QPI kernel extraction, which models the space of physically valid kernels and uses this knowledge to guide the inverse mapping. We introduce a two-step learning strategy that decouples kernel representation learning from observation-to-kernel inference. In the first step, we train a variational autoencoder to learn a compact latent space of scattering kernels. In the second step, we align the latent representation of QPI observations with those of the pre-learned kernels using a dedicated encoder. This design enables the model to infer kernels robustly under complex, entangled scattering conditions. We construct a diverse and physically realistic QPI dataset comprising 100 unique kernels and evaluate our method against a direct one-step baseline. Experimental results demonstrate that our approach achieves significantly higher extraction accuracy, improved generalization to unseen kernels. To further validate its effectiveness, we also apply the method to real QPI data from Ag and FeSe samples, where it reliably extracts meaningful kernels under complex scattering conditions.

cs.LG↗

arXiv2025

Observation of Persistent Zero Modes and Superconducting Vortex Doublets in UTe$_2$

Superconducting vortices can reveal electron pairing details and nucleate topologically protected states. Yet, vortices of bulk spin-triplet superconductors have never been visualized. Recently, UTe$_2$ has emerged as a nominative spin-triplet superconductor, but its superconducting order parameter is elusive, and whether time-reversal symmetry is broken remains unsettled. Here, we visualize superconducting vortices on the (011) surface of ultra-clean UTe$_2$ single crystals ($T_c=2.1 K$) using scanning tunneling microscopy (STM). We introduce $\frac{d^2 I}{dV^2}$ imaging as an effective method for vortex visualization in superconductors with substantial residual zero-energy density of states (DOS), as in UTe$_2$. Anisotropic single-flux-quantum vortices, with coherence lengths of $\sim$ 12 nm (4 nm) parallel (perpendicular) to the a-axis, form a triangular vortex lattice (VL) under small out-of-plane magnetic fields. The vortex size decreases at higher fields, suggesting multi-band superconductivity. The robustness of vortex structures and VL against magnetic field polarity and cooling history strongly supports time-reversal invariant superconductivity. Spatially non-splitting and spectroscopically narrow zero-bias peaks (ZBPs) of differential conductance at vortex cores (VCs) persist up $8T$, well beyond the Pauli limit ($3.9T$), consistent with Majorana zero modes (MZMs) in a topological vortex line protected by a combination of mirror, time-reversal, and particle-hole symmetries. Close examination of vortex structures reveals a mirror-asymmetric doublet $--$ one with a singular core and another with an enhanced energy gap. Such unconventional vortices in a non-chiral $p$-wave superconductor could originate from the induction of a subdominant order parameter close to the VCs.

cond-mat.supr-con↗