Search arXiv⌕ Search

arXiv subjects

Mounica Mahankali

Publications and source records attributed to Mounica Mahankali.

8 recordsLinked to original sources

Chiral Weyl-Kondo semimetallic state through enhanced correlation in CeGaGe

Strongly correlated chiral materials have been proposed to host a chiral Weyl-Kondo semimetal (cWKSM) state, in which Kondo hybridization pins chirality-induced Kramers-Weyl point crossings, together with additional symmetry-enforced band crossings, near the Fermi level. Realizing this state requires a material that combines crystal chirality, non-symmorphic symmetry, and Kondo correlations, and currently there are no known materials that combine all these requirements. Here we report evidence for a cWKSM state in CeGaGe, a member of the RXY (R = rare earth; X = Al, Si; Y = Ga, Ge) family. Magnetization measurements confirm long-range antiferromagnetic order below T$_N$ = 4.7 K with a complex, canted magnetic structure. Unique to CeGaGe among the known RXY systems is a structural transition from an achiral tetragonal I4$_{1}$md structure (at high temperatures) to the chiral tetragonal P4$_{3}$ structure (at low temperatures). The structural transition in CeGaGe allows us to highlight the role of chirality in stabilizing the Kramers cWKSM state. Hall resistivity measurements with $H || c$ reveal an anomalous Hall conductivity (AHC) that is constant below the Kondo temperature $T_K \approx 7$ K and drops sharply above it. This crossover tracks the onset of Kondo coherence rather than the magnetic ordering, which occurs at T$_N$ = 4.7 K. Together with first-principles calculations for the $P4_3$ structure, this identifies the AHC as an intrinsic, Berry-curvature-driven contribution generated by Kondo hybridization, rather than a consequence of extrinsic scattering or dynamic scalar spin chirality. These results establish CeGaGe as a rare experimental platform in which crystal chirality, strong electronic correlations, and non-trivial band topology coexist, providing the first material realization of a Kondo-driven cWKSM state.

cond-mat.str-el↗

Chiral Weyl--Kondo semimetal and circular photogalvanic effect in a prototype Kondo lattice system

Chiral Weyl--Kondo semimetals (cWKSM) provide a setting in which chiral Weyl quasiparticles emerge in the immediate vicinity of the Fermi energy from a Kondo-driven reconstruction of the strongly correlated electronic states in chiral heavy fermion systems (K.-S. Lin et al., arXiv:2602.22185). A defining characteristic of this strongly correlated topological state is the Kramers chiral Weyl fermions in the low-energy quasiparticle states. Recently, experiments in CeGaGe have emerged as a concrete realization of the proposed effect (Arushi et al., preprint). Motivated by these findings, here we go beyond the materials-specific effects by constructing a prototype Kondo lattice model; it incorporates only the essential couplings that respect the associated tetragonal crystalline symmetries. This simplification allows us to robustly demonstrate the symmetry-enforced Kramers Weyl fermions and related topological nodal states in the spectrum of heavy quasiparticles. Furthermore, the simplification provides a tractable setting to determine the salient features in the system's nonlinear optical response, the circular photogalvanic effect, in chiral Weyl--Kondo semimetals. Both analytical and numerical calculations identify sharp peaks in the frequency domain as signatures of the Kondo-driven chiral Weyl nodes; the sharpness of the spectrum reflects the resonant nature of the underlying strongly correlated electronic excitations. Thus, cWKSM provides a unique setting to spectroscopically identify topological fermions that are induced by strong electron correlations. As such, our results are expected to bring about much needed new insights into the understanding of strongly correlated gapless topological matter.

cond-mat.str-el↗

Quantum Fisher information of magnetic quantum phase transition on Kondo lattice

Strange metals exemplify highly collective quantum many-body systems that call for new means of characterization, and there is considerable potential for quantum information approaches contributing to the cause. We investigate multipartite entanglement across the quantum phase transition of a Kondo lattice model using the quantum Fisher information (QFI). We show that the QFI associated with the spin components transverse to the order parameter characterizes the destruction of heavy quasiparticles in the Kondo-destroyed magnetic-ordered phase. The physical origin of this observation is elucidated through an analysis of the antiferromagnetic Heisenberg model. We propose to test the results in terms of both unpolarized and polarized inelastic neutron scattering measurements in the ordered part of the heavy fermion phase diagram. Our findings illustrate how different operators of a many-body system can be employed to not only witness multipartite entanglement in different sectors and but also elucidate the overall physics across different parts of the phase diagram.

cond-mat.str-el↗

Amplified response of cavity-coupled quantum-critical systems

A quantum critical point develops when matter undergoes a continuous transformation between distinct ground states at absolute zero. It hosts pronounced quantum fluctuations, which render the system highly susceptible to external perturbations. While light-matter coupling has rapidly moved forward as a means to probe and control quantum materials, the capacity of quantum critical fluctuations in the photon-mediated responses has been largely unexplored. Here we advance the notion that directly coupling a quantum critical mode to a quantized cavity field dramatically facilitates the realization of the elusive superradiant phase transition in equilibrium, circumventing at once the key obstacles that have prevented its attainment in spite of decades of pursuit. The superradiant phase transition develops far below the ultrastrong regime of light-matter couplings, and the transition is accompanied by the hybrid system showing strongly enhanced intrinsic squeezing and amplified quantum Fisher information. We also identify candidate cavity quantum materials platforms for validating the proposed effect. Our findings suggest a general principle by which quantum criticality amplifies the response to cavity photons. They also demonstrate that cavity coupling accesses the elevated quantum entanglement of the underlying matter at quantum criticality, thereby pointing to a pathway towards realizing the potential of highly collective quantum materials to expand the capacities of quantum information science.

cond-mat.str-el↗

Resolving the Kagome Origin of the Strange Metallicity in Ni$_3$In

Strong correlations promote singular properties such as strange metallicity, which shows considerable commonality across quantum materials platforms. Understanding the mechanism for such emerging universality is an outstanding challenge, given that the underlying degrees of freedom can be complex and varied. Progress may be made in flat band systems, especially kagome and other frustrated-lattice metals with active flat bands. These systems show strange metal behavior that bears a striking resemblance to what happens in heavy-fermion metals. Here, in scanning tunneling spectroscopy of kagome metal Ni$_3$In, we find a zero-bias peak-dip structure whose variation with magnetic field and temperature tracks the evolution of the strange metal properties. We identify the origin of the peak as compact molecular orbitals formed by destructive interference over the kagome sites, resulting in emergent $f$-shell-like localized moments. Using quasi-particle interference, we visualize their interaction with the Dirac light bands. We thus unveil the essential microscopic ingredients of the $d$-electron-based kagome metals that, while distinct from the atomic orbitals of the $f$-electron-based heavy fermion materials, are responsible for a shared phenomenology between the two types of systems. Our findings provide a new window to uncover and interconnect the essential and yet diverse microscopic building blocks in disparate families of quantum materials that drive a convergence towards a universal understanding in the regime of amplified quantum fluctuations.

cond-mat.str-el↗

Correlated flat-band physics in a bilayer kagome metal based on compact molecular orbitals

Flat bands, when located close to the Fermi energy, can considerably enhance the influence of electron correlations on the low energy physics in kagome and other frustrated-lattice metals. A major challenge in describing the interaction effects in such bulk materials is that the flat band is often intermixed with a large number of other bands. Here we show that the recently introduced notion of compact molecular orbitals (CMOs) enable a path forward in describing the dominant effect of the Coulomb interactions in spite of the complexity of the bandstructure. Our materials-based analysis allows for the understanding of the scanning-tunneling-microscopy experiment [J. C. Souza et al., preprint (2024)] of the bilayer kagome metal Ni$_3$In in terms of the CMO notion. From the resulting CMO, an effective Anderson lattice model can be set up. This CMO-based approach enables the calculation of correlation effects that is difficult to do based on the atomic orbitals. Furthermore, it suggests an enriched phase diagram for the strange metal physics of the kagome metal, which can be tested by future experiments. We discuss the implications of our results for the general correlation physics of flat band systems and beyond.

cond-mat.str-el↗

Amplified multipartite entanglement witnessed in a quantum critical metal

Strong correlations in matter promote a landscape of quantum phases and associated quantum critical points. For metallic systems, there is increasing recognition that the quantum criticality goes beyond the Landau framework and, thus, novel means are needed to characterize the quantum critical fluid. Here we do so by studying an entanglement quantity, the quantum Fisher information, in a strange metal system, focusing on the exemplary case of an Anderson/Kondo lattice model near its Kondo destruction quantum critical point. The spin quantum Fisher information peaks at the quantum critical point and indicates a strongly entangled ground state. Our results are supported by the quantum Fisher information extracted from inelastic neutron scattering measurements in heavy fermion metals. Our work elucidates the loss of quasiparticles in strange metals, opens a quantum information avenue to advance the understanding of metallic quantum criticality in a broad range of strongly correlated systems, and points to a novel regime of quantum matter to realize amplified entanglement.

cond-mat.str-el↗

Spectral singularity enhances transverse spin

We study the transverse spin and the Belinfante spin momentum in a gain-loss balanced waveguide, known to be one of the first and most studied examples of $\mathcal{PT}$-symmetric systems. Such a guide supports the spectral singularities leading to infinite scattering amplitudes for both reflection and transmission. We show that near the spectral singularity there can be dramatic enhancement of the transverse spin and the transverse spin momentum. Note that these exotic spin and spin momentum have recently been observed experimentally despite having tiny magnitudes, making it worthy to explore ways and means to enhance these fundamentally important elusive quantities.

physics.optics↗