arXiv subjects

Pengcheng Dai

Publications and source records attributed to Pengcheng Dai.

At least 19 recordsLinked to original sources

arXiv2026

Resolving magnetic order and dynamics with polarized neutron scattering: a practical guide to longitudinal polarization analysis

Neutron scattering provides microscopic information on magnetic order and spin dynamics. Most experiments, however, use unpolarized neutrons and do not fully exploit the information carried by the neutron spin. Longitudinal polarization analysis (LPA), established in the pioneering work of Moon, Riste, and Koehler at Oak Ridge National Laboratory in the late 1960s, separates magnetic and nonmagnetic scattering contributions through their different effects on the neutron spin. In this review, we illustrate how LPA can distinguish weak magnetic scattering from nonmagnetic contributions, constrain small moment components, and resolve the spin-space anisotropy of magnetic excitations. We introduce the formalism connecting measured polarization channels to magnetic quantities and discuss scattering geometry, crystallographic projections, and corrections for finite polarization. Our aim is to provide a practical guide for neutron scatterers using LPA to determine magnetic structures and characterize spin excitations in quantum materials. We conclude with opportunities in altermagnets, unconventional superconductors, and kagome magnets.

cond-mat.str-el↗

arXiv2026

Distributed scalable coupled policy algorithm for networked multi-agent reinforcement learning

This paper studies networked multi-agent reinforcement learning (NMARL) with interdependent rewards and coupled policies. In this setting, each agent's reward depends on its own state-action pair as well as those of its direct neighbors, and each agent's policy is parameterized by its local parameters together with those of its $κ_{p}$-hop neighbors, with $κ_{p}\geq 1$ denoting the coupled radius. To address the challenge of interdependent policies in collaborative optimization, we introduce a novel concept termed the ``neighbors' averaged $Q$-function'' and derive a new expression for the coupled-policy gradient. Based on these theoretical foundations, we develop a distributed scalable coupled policy (DSCP) algorithm, where each agent relies only on the state-action pairs of its $κ_{p}$-hop neighbors and the rewards of its $(κ_{p}+1)$-hop neighbors. Specifically, in the DSCP algorithm, we employ a geometric 2-horizon sampling method that does not require storing a full $Q$-table to obtain an unbiased estimate of the surrogate coupled-policy gradient under the executed policy. Moreover, each agent interacts exclusively with its direct neighbors to obtain accurate policy parameters, while maintaining local estimates of other agents' parameters to execute its local policy and collect samples for optimization. These estimates and policy parameters are updated in a distributed manner through local information exchange among direct neighbors, enabling coordinated policy updates across the network. We prove that the gradient norm of the objective function along the joint policy sequence produced by the proposed algorithm converges to zero almost surely. Finally, the effectiveness of the DSCP algorithm is demonstrated through simulations in a robot path planning environment, showing clear improvement over the compared algorithms in the tested setting.

cs.MA↗

arXiv2026

Spontaneous Circular Dichroism and Memory Effect from Surface Defects in Altermagnetic MnTe

Altermagnetism has emerged as a new class of magnetism with vanishing magnetization and macroscopic time reversal symmetry breaking. Hexagonal MnTe is a g-wave altermagnet with a 307 K Néel temperature, large spin splitting, and an anomalous Hall effect. However, the relationship between altermagnetism and the anomalous Hall effect in MnTe remains debated. Here, using optical magnetic circular dichroism, we observe hysteresis and a memory effect in a MnTe bulk crystal below 250 K. No hysteresis is seen after polishing the bulk crystal and in thin films. We conclude that the hysteresis in magnetic circular dichroism in the bulk crystal is from surface defects. The similar temperature dependence and a sign change between circular dichroism and the anomalous Hall effect indicate that the origin of the anomalous Hall effect in transport is likely not intrinsic.

cond-mat.mtrl-sci↗

arXiv2026

Signatures of bi-altermagnetism revealed by sublattice-specific circular dichroism in resonant inelastic X-ray scattering

An altermagnet is a recently identified class of magnets that exhibit a zero net magnetic moment but break symmetry under the combined operations of parity and time reversal. It typically consists of two magnetic sites of opposite spins related by rotation within the unit cell. Here, we use circular dichroism (CD) in resonant inelastic X-ray scattering (RIXS) to reveal symmetry signatures of a distinct form of altermagnetism, namely bi-altermagnetism, in the correlated insulator Fe2Mo3O8, which comprises two altermagnetic sublattices: one with alternating quasi-octahedral Fe environments and the other with alternating tetrahedral Fe environments. We experimentally revealed the emergence of CD in an achiral, zero-magnetization system, thereby probing mirror-symmetry breaking associated with altermagnetic order. Notably, the CD appeared at sublattice-specific excitations of the octahedral and tetrahedral sites, indicating symmetry breaking in both altermagnetic sublat- tices. Calculations based on a model with the bi-altermagnetic order along the c axis successfully reproduce the observed CD. Our findings support the realization of bi-altermagnetism in Fe2Mo3O8, and showcase the use of RIXS-CD as a probe of magnetic sublattices in systems with zero net magnetization.

cond-mat.str-el↗

arXiv2026

Easy-plane anisotropy of magnetic fluctuations in UTe2

The large directional anisotropy of superconducting UTe2 along the lattice a, b, c directions in magnetic susceptibility, upper critical fields, and Knight shift suggests spin-triplet Cooper pairing. If spin fluctuations bind the Cooper pair, one needs to determine their anisotropy in spin space to characterize the superconducting state. Here we use polarised and unpolarised inelastic neutron scattering (INS) experiments to show that antiferromagnetic (AFM) spin fluctuations at the Y point are highly isotropic within the ac-plane but have no observable magnitude along the b-axis. Our results rule out the assumed Ising anisotropy and constrain the possible pairing channels. AFM exchange is no longer pair forming in the triplet channel and the d vector along b is strongly favoured. We capture the experimental observations within a microscopic framework that encompasses the dual nature of 5f electrons. We include itinerant and localized 5f-moments in a tight-binding model fitted to quantum oscillations data. In congruence with INS, the exchange between localized moments generically consists of a strong FM intra-dimer interaction, maxima close to the Y and T points, mediated by 5p_y and 6d_{3z^2-r^2} orbitals respectively, and magnetically decoupled ab-planes. We find that anisotropy and dimerization of the moments can lead to gapped excitations that, in combination with Landau damping, can produce the observed overdamped response at the Y point. We suggest that enhancement of the response and its observed near-O(2)-symmetry could both be driven by proximity to a quantum critical point where the dimer excitation gap closes and gives place to incommensurate helical order. Analysis of the linearized gap equation for a nearest-neighbour pairing interaction favours the B1u triplet with a dominant d-vector component along b, although the possibility of spin singlet pairing cannot be ruled out.

cond-mat.str-el↗

arXiv2026

Structural Phase Separation Couples to Charge-Density-Wave Formation in Kagome Metal FeGe

The intertwining of charge, spin, and lattice degrees of freedom underlies the emergent properties of correlated materials. A recent prominent example is the kagome metal FeGe, which hosts coexisting charge density wave (CDW) and antiferromagnetic orders, accompanied by a lattice distortion associated with partial Ge-Ge dimerization. Using temperature-dependent high-resolution X-ray diffraction measurements, we observed a robust splitting of the lattice reflection into two coexisting peaks with distinct lattice constants at the CDW transition temperature TCDW, providing direct evidence for a first-order structural phase transition that is absent in samples with suppressed CDW order. Furthermore, the long-range CDW order was found to be only commensurate with lattice structures with the compressed out-of-plane lattice constant. The Landau free energy analysis shows that strong lattice-charge coupling is a key factor in stabilizing long-range CDW order. Our work clarifies the critical role of structural transformation in the CDW formation and opens opportunities for strain control of electronic phases in FeGe.

cond-mat.mtrl-sci↗

arXiv2026

Scalable Policy Optimization for Networked Multi-Agent Reinforcement Learning with Continuous State-Action Spaces

Learning local policies for continuous networked systems requires accounting for the effects of decisions beyond each agent's observation neighborhood. Spatial decay limits these effects, but a finite critic must also control representation and estimation errors throughout policy optimization. We analyze the Continuous Distributed Coupled Policy Gradient (CDCPG) algorithm using local random Fourier features and least-squares temporal-difference critics. For features that retain the boundary inputs required by the local dynamics, we derive an action-value representation with separate spatial and finite-feature residuals. A global integrated transition-approximation bound and a projected Bellman argument control population prediction error without an inverse-conditioning multiplier. We then quantify the dependence of critic estimation on feature excitation and dimension, and construct simultaneous lower confidence bounds for temporal-difference conditioning along the executed iterates. Combining critic error with localized reward aggregation bounds the expected squared projected-gradient mapping by an optimization term and an explicit residual separating spatial approximation, finite features, and omitted distant rewards. For fixed neighborhoods and feature dimension, the shared-oracle sample count is inverse-squared in the excess squared-stationarity accuracy, up to logarithmic factors. The guarantee assumes known local dynamics and rewards, independent discounted-occupancy samples, and stated excitation, decay, and smoothness conditions, and is conditional on favorable feature draws. Numerical studies illustrate related implementations on a linear-coupled-quadratic benchmark.

cs.MA↗

arXiv2026

Distributed primal-dual algorithm for constrained multi-agent reinforcement learning under coupled policies

This paper investigates constrained multi-agent reinforcement learning (CMARL) in coupled environments, where agents collaboratively maximize the sum of local objectives while satisfying individual safety constraints. Existing studies face two limitations: (1) most rely on independent policies that fail to capture complex interactions in coupled environments; and (2) agents require the global Lagrange multipliers, which are sensitive learned variables whose global sharing risks exposing private agent-specific information. To overcome these issues, we propose a framework where agents adopt coupled policies that depend on both the states and policy parameters of their $κ_p$-hop neighbors, where $κ_p>0$ denotes the coupling distance, and develop a distributed and scalable primal-dual (DSPD) algorithm wherein each agent accesses only information within a prescribed local neighborhood. In the proposed algorithm, agents exchange sensitive parameters only with immediate neighbors over a separate time-varying network, while maintaining local estimates to execute the coupled policy. We establish that the proposed algorithm achieves $ε$-policy stationary convergence with approximation error $\mathcal{O}(γ^{\frac{κ+1}{κ_{p}}})$, where $κ>0$ is the truncated distance and $γ\in(0,1)$ is discount factor. Simulations on a wireless access-control network demonstrate that the proposed algorithm outperforms existing state-of-the-art algorithms, validating its effectiveness.

cs.MA↗

arXiv2026

Crystal electric field excitations and an effective-spin-$1/2$ ground doublet in the hyperkagome magnet Yb$_3$Sc$_2$Ga$_3$O$_{12}$

We use inelastic neutron scattering (INS) to determine the crystal electric field (CEF) excitations of Yb$^{3+}$ in the rare-earth hyperkagome magnet Yb$_3$Sc$_2$Ga$_3$O$_{12}$. Three nearly dispersionless magnetic excitations are observed near 58, 68, and 74~meV, corresponding to transitions from the ground-state Kramers doublet to the three excited doublets of the $J=7/2$ multiplet. A Stevens-operator analysis constrained by the local $222$ ($D_2$) symmetry reproduces the excitation energies and spectral weights and yields an Ising-type ground-state $g$ tensor. The first excited doublet lies approximately 58~meV above the ground state, establishing a well-isolated effective $J_{\mathrm{eff}}=1/2$ degree of freedom over the low-temperature regime relevant to collective magnetism. Notably, the directly measured CEF spectrum substantially revises the level scheme previously inferred from bulk measurements, while preserving the essential low-energy pseudospin description. Two independent fitting protocols give consistent excitation energies, ground-doublet wave functions, and $g$ tensors, despite the nonuniqueness of the individual CEF parameters. The resulting single-ion model also reproduces the characteristic susceptibility, magnetization, and field evolution of the Schottky anomaly in specific heat. These results establish the microscopic single-ion basis needed to construct an effective exchange Hamiltonian and to interpret future measurements of low-energy collective excitations in Yb$_3$Sc$_2$Ga$_3$O$_{12}$.

cond-mat.str-el↗

arXiv2026

Nanoscale Imaging of Strain-Controlled Altermagnetic Domains in α-MnTe

Altermagnets combine compensated magnetic order with momentum-dependent spin splitting, offering a route to spintronic functionality without the stray fields of conventional ferromagnets. Mechanical strain provides a promising means of controlling their Néel order, yet the microscopic pathway by which strain reorganizes an altermagnetic texture remains unresolved. Here, we combine scanning nitrogen-vacancy magnetometry with a piezo-driven uniaxial strain cell to directly image the strain-driven evolution of magnetic domains in bulk α-MnTe at room temperature. By applying uniaxial stress along the nearest-neighbor Mn-Mn bond direction, we find that compressive strain reorganizes the magnetic texture through domain coalescence, increasing the size of the largest connected domain while reducing the domain-wall density. On sweeping toward tensile strain direction, however, the domain network follows a distinct trajectory from that observed during the compressive sweep. Instead, the large connected regions fragment into a new metastable configuration, producing pronounced hysteresis in the maximum domain size and stray-field distribution. These results identify domain connectivity and topology as key carriers of strain-induced magnetic memory. Our work reveals domain coalescence and hysteretic fragmentation as the microscopic pathway of strain control in α-MnTe and establishes a route toward strain-programmable altermagnetic textures and reconfigurable spintronic devices.

cond-mat.mtrl-sci↗

arXiv2026

Spin nematic liquid crystal and scalar spin chirality in tetragonal lattice YbMnBi$_2$

A spin nematic order, analogous to the nematic liquid crystal, characterizes the spontaneous breaking of spin-space rotational symmetry while preserving time-reversal ($T$) symmetry. In contrast, scalar spin chirality (SSC), a composite three-spin order, breaks $T$ symmetry and is known to induce an anomalous Hall effect (AHE). Although a spin nematic phase has been suggested in frustrated magnets and the square-lattice iridate, how it might affect magnetotransport properties is unknown. Here we use polarized neutron scattering to show that tetragonal $A$MnBi$_2$ ($A$ = Ca, Yb) is a strictly $c$-axis-aligned collinear antiferromagnet (C-type), with $T_N \approx 270$ K and 290 K, respectively. On cooling from 450 K to $T_N$, low-energy spin excitations in YbMnBi$_2$ spontaneously change from isotropic to anisotropic in spin space within the tetragonal plane, forming a dynamic spin nematic phase around 400 K due to heavy Yb-induced spin-orbit coupling, before gapping out below $T_N$. Similar measurements on CaMnBi$_2$ reveal isotropic paramagnetic scattering without a spin nematic phase above $T_N$. Under an in-plane magnetic field, the Yb$^{3+}$ moments may interact with the dynamic spin nematic phase to induce nonzero SSC, giving rise to AHE and an anomalous Nernst effect (ANE) in YbMnBi$_2$ that are absent in CaMnBi$_2$ above $T_N$. A symmetry-based Ginzburg-Landau analysis shows that coupling terms between the nematic order and SSC are allowed under an external magnetic field, which could explain the rapid increase of AHE with field in YbMnBi$_2$. Our results provide compelling evidence for dynamic SSC-induced AHE and ANE in the paramagnetic phase of a compensated collinear antiferromagnet, opening a new avenue for the physics of composite spin orders and room-temperature spintronics without magnetic order.

cond-mat.str-el↗

arXiv2026

$d$-spacing distributions as a probe of nematoelastic response in iron-based superconductors

Electronic nematicity in iron-based superconductors (FeSCs) couples bilinearly to orthorhombic strain, allowing nematic correlations to appear in the lattice response. Here we use neutron Larmor diffraction to measure the temperature-dependent distribution of relative $d$ spacings in electron-doped Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$, hole-doped Ba$_{0.83}$K$_{0.17}$Fe$_2$As$_2$, FeSe, and Fe$_{1.07}$Te. In Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ crystals without intentionally applied uniaxial stress, the in-plane distribution width, $\varepsilon_{\rm FWHM}$, increases on cooling in the tetragonal phase and can be described phenomenologically by a Curie--Weiss-like form. The fitted scale $T^*$ decreases with Co doping and evolves similarly to the nematic phase diagram inferred from elastoresistance, although the two experiments probe different response functions. Related broadening in Ba$_{0.83}$K$_{0.17}$Fe$_2$As$_2$ and FeSe supports extending this interpretation beyond electron-doped BaFe$_2$As$_2$. By contrast, Fe$_{1.07}$Te shows no extended Curie--Weiss-like regime without applied stress, whereas uniaxial pressure produces a strongly anisotropic broadening that can contain contributions from both the field-biased lattice response and inhomogeneous loading. A mean-field model with bilinear nematoelastic coupling and spatially varying symmetry-breaking stress explains the Curie--Weiss-like broadening in terms of the renormalized orthorhombic compliance. Neutron Larmor diffraction therefore provides a bulk-sensitive probe of nematic-related lattice broadening that complements electronic and elastic measurements.

cond-mat.supr-con↗

arXiv2026

Field-induced first order transitions and phase coexistence in the Kitaev quantum spin liquid candidate BaCo2(AsO4)2

BaCo2(AsO4)2 (BCAO) is an insulating Kitaev quantum spin liquid candidate with a rich low-temperature phase diagram. Below 5 K, it exhibits double-zigzag magnetic order. Upon application of an in-plane magnetic field, the magnetic structure first transforms into an up-up-down (UUD) state near 0.12 T and then enters a fully spin-polarized ferromagnetic (FM) state near 0.5 T. In the narrow field regime close to the polarized phase, a finite residual thermal conductivity has been reported, suggesting a possible field-induced quantum spin liquid phase. Using neutron scattering, we show that the field-induced double-zigzag-to-UUD transition near 0.15 T is accompanied by the emergence of a cluster of localized UUD spin excitations that coexist with conventional spin waves. Upon further increasing field, BCAO undergoes a first-order UUD-to-FM transition with coexistence of UUD and FM phases, accompanied by a sharp response in the spin Seebeck coefficient. These results do not support a quantum spin liquid scenario near the UUD-to-FM critical field. Instead, modeling indicates that the broad excitations arise from bound spin-flip pairs, while a low-lying dispersive branch near the FM phase boundary carries the same sign of magnetization as the FM order. These excitations naturally account for the observed sign of the spin Seebeck response and are likely relevant to the thermal conductivity near the critical field.

cond-mat.str-el↗

arXiv2026

Iron-Based Superconductors: A Decade of Materials, Magnetism, and Mechanisms

Since its discovery in 2008, iron-based superconductors (FeSCs) have become a central platform for exploring high-temperature superconductivity in multiband, electron-correlated materials. This review focuses on major developments over the past decade or so, emphasizing experimental advances, pairing mechanisms, and emerging applications. Structural tuning through chemical substitution, pressure, and epitaxial growth enables precise control of the electronic, magnetic, and superconducting ground states, thereby revealing their interplay. In particular, the electronic nematic phase and stripe-type antiferromagnetic order-often coexisting or competing-are central to understanding the phase diagrams. Spin waves in magnetically ordered parent compounds and spin excitations (fluctuations) in doped superconductors are extensively characterized by inelastic neutron scattering. While high-energy spin excitations in doped superconductors retain substantial spectral weight across a wide energy range reminiscent of spin waves in their undoped parents, the low-energy response reveals a collective spin excitation termed "resonance" coupled to superconductivity. The momentum structure of superconductivity-induced resonance provides strong evidence for sign-changing pairing in many FeSCs, while disorder effects, orbital-fluctuation scenarios, quasiparticle damping, and compound-dependent gap structures indicate that $s_{\pm}$, $s_{++}$, nodal $s$, $d$-wave, and multicomponent states must be discussed in a material-specific framework. Advances in thin-film growth, intercalation chemistry, and interface engineering-particularly in FeSe-based systems-have enabled enhanced $T_{c}$ and novel device geometries. With high upper critical fields, moderate anisotropy, and improving current densities, FeSCs continue to drive both fundamental insight and technological applications in superconductivity.

cond-mat.supr-con↗

arXiv2026

Phonons and magnetism of kagome FeGe probed by nuclear resonant scattering

Kagome FeGe hosts a $2\times2\times2$ charge-density wave (CDW) that strongly interplays with antiferromagnetic order. Here, we report $^{57}$Fe nuclear resonant scattering measurement to study FeGe across its long-range CDW and incommensurate magnetic transitions. Upon entering the CDW state, hardening of acoustic phonons and optical phonons around 22~meV, 27~meV, and 31~meV are observed in the Fe partial phonon density of states, which can be qualitatively captured by first-principle calculations. Upon entering the incommensurate magnetic phase, neither the phonon density of states nor the hyperfine interaction parameters change significantly, although a subtle feature associated with the incommensurate magnetic order or slow fluctuations is detected in the time-domain Mössbauer spectra. These findings show that the CDW in kagome FeGe significantly modifies its lattice dynamics and magnetism, evidencing an intertwined nature of the spin, charge, and lattice degrees of freedom.

cond-mat.str-el↗

arXiv2026

Atomic-Scale Observation of Symmetry Breaking in Altermagnetic MnTe

The recent discovery of altermagnetism has sparked growing interest in compensated magnetic systems as promising platforms for highly scalable spintronics. Altermagnetism is a distinct magnetic order where opposite spin sublattices are connected by rotation, yielding zero net magnetization but momentum-dependent spin splitting. To date, experimental verification of altermagnetic order has been achieved predominantly through bulk-sensitive techniques, including spin-dependent electronic spectra and transport responses. However, direct atomic-scale evidence that explicitly correlates crystal symmetry, local structural distortions, and magnetic ordering has remained unexplored. Here, we report the direct atomic-scale observation of coexisting polar distortions and altermagnetic order in MnTe, combining atomic resolution scanning transmission electron microscopy (STEM) imaging with electron magnetic chiral dichroism (EMCD) measurements. We reveal that MnTe is not an ideal uniform P63/mmc g-wave altermagnet at the atomic scale. Instead, it hosts ubiquitous inversion-symmetry-breaking distortions that lower the spin-space-group (SSG) symmetry, admits d-wave altermagnetic components, and in lower-symmetry regimes, even allow s-wave spin splitting (net magnetization). The coexistence of ferroelectric signatures and altermagnetic order establishes local lattice symmetry in MnTe as a control knob for altermagnetic spin splitting, spin current generation, and multiferroic memory applications.

cond-mat.mtrl-sci↗

arXiv2026

Distributed Zeroth-Order Policy Gradient for Networked Multi-agent Reinforcement Learning from Human Feedback

We study a networked multi-agent reinforcement learning (NMARL) problem with human feedback in an infinite-horizon setting, where agents interact over an underlying network with localized state dependencies and aim to collaboratively maximize the average discounted return. Existing approaches with preference feedback are primarily developed for single-agent settings and rely on centralized training, which limits their scalability and applicability to large-scale networked multi-agent systems. To address this, we introduce a novel human feedback mechanism based on spatiotemporally truncated trajectories, defined as $H$-horizon trajectory pairs aggregated over each agent's $κ$-hop neighborhood. Building on this, we develop a distributed zeroth-order policy gradient algorithm, where each agent estimates its local policy gradient using human preference feedback generated from both the current joint policy and a perturbed joint policy drawn from zero-mean Gaussian distribution. Specifically, the algorithm is fully distributed, as the feedback received by each agent depends solely on the state-action information within its $κ$-hop neighborhood and does not require explicit reward signals or centralized control. We further rigorously establish that the proposed algorithm converges to an $ε$-stationary point with polynomial sample complexity. Finally, simulation results in a stochastic GridWorld environment and a predator-prey environment further demonstrate that the effectiveness and scalability of the proposed algorithm in achieving collaborative optimization based solely on human preference feedback.

cs.MA↗

arXiv2026

Winding feature and thermal evolution of the Dirac magnons in CrI$_3$

Two-dimensional honeycomb lattice ferromagnet chromium tri-iodide (CrI$_3$) has attracted tremendous interest because it retains ferromagnetism down to the monolayer limit and hosts intriguing topological magnons. As a prototypical van der Waals magnet, CrI$_3$ provides an ideal platform for exploring the interplay between reduced dimensionality, magnetic order, and nontrivial spin excitations. Here, using inelastic neutron scattering together with improved sample quality, we uncover the magnon winding feature around the $K$-point of the hexagonal Brillouin zone, a key signature of Dirac magnons. In addition, we find that the magnon energy follows a $T^2$-renormalization behavior at elevated temperatures, consistent with magnon-magnon interactions. These results provide previously missing information on the magnon spectrum of CrI$_3$ and further consolidate the topological nature of its spin excitations.

cond-mat.mtrl-sci↗