arXiv subjects

R. Mathieu

Publications and source records attributed to R. Mathieu.

At least 19 recordsLinked to original sources

arXiv2026

Switching magnetic spin-states using small magnetic fields in compositionally complex Sm(M7)O$_3$

High-entropy perovskites (HEPs) offer a unique platform for exploring magnetic phenomena arising from extreme B-site chemical disorder. In Sm(M7)O$_3$, where there are 7 cations in equal amounts at the B-site; M = Ti, Cr, Mn, Fe, Co, Ni, Cu), we observe long-range antiferromagnetic ordering near 105 K accompanied by a small but robust excess magnetic moment intrinsic to the chemically disordered lattice. This uncompensated moment is evident from ZFC-FC irreversibility, shifts in the isothermal M(H) loops, and discrete remanent states identified through direct-current-demagnetization measurements. Remarkably, cooling fields as small as $\pm$ 20 Oe are sufficient to select the direction of the excess moment, and the chosen magnetic state remains stable against applied fields up to 50 kOe. A low-temperature anomaly in the remanent magnetization further reveals a secondary contribution from the Sm$^{3+}$ sublattice, although the primary origin of the excess moment resides in the B-site AFM sublattice.

cond-mat.mtrl-sci↗

arXiv2026

Temperature Dependent Magnetic and Structural Properties of Al Substituted Nanostructured Ferrites with Large Coercive Fields

We report a comprehensive study of the temperature-dependent structural, magnetic, vibrational, and dielectric properties of Al-substituted M-type hexaferrites SrFe$_{12-x}$Al$_x$O$_{19}$. Neutron powder diffraction and M\"ossbauer spectrometry show that Al$^{3+}$ preferentially replaces Fe$^{3+}$ at spin-up octahedral sites (2a, 12k), disrupting the exchange coupling with the spin-down 4f tetrahedral sites and leading to a progressive reduction of site-specific magnetic moments and a systematic decrease in the Curie temperature, supported by temperature dependent susceptibility measurements. Raman spectroscopy reveals pronounced phonon anomalies near $T_C$, particularly in modes associated with bipyramidal Fe-O vibrations, reflecting the weakening of both 4e-12k and 4e-4f exchange pathways. However, the coercive field exhibits a dramatic increase, reaching $\mu_0H_C$ $\sim$ 1.2 T for SrFe$_{9.6}$Al$_{2.4}$O$_{19}$, among the largest values reported for this class. Susceptibility measurements suggest that Al substitution, while weakening the superexchange network, contributes to the stabilization of single-domain behavior.

cond-mat.mtrl-sci↗

arXiv2025

A systematic method to identify runaways from star clusters produced from single-binary interactions: A case study of M67

One hypothesis for runaway stars (RSs) is that they are ejected from star clusters with high velocities relative to the cluster center-of-mass motion. There are two competing mechanisms for their production: supernova-based ejections in binaries, where one companion explodes, leaves no remnant, and launches the other companion at the instantaneous orbital velocity, and the disintegration of triples (or higher-order multiples), which produces a recoiled runaway binary (RB) and an RS. We search for RS candidates using data from the Gaia DR3 survey with a focus on triple disintegration since in this case the product is always a binary and a single star that should be moving in opposite directions. We created a systematic methodology to look for candidate RS-RB runaway pairs produced from the disintegration of bound three-body systems formed from single-binary interactions based on momentum conservation and causality. The method we use is general and can be applied to any cluster with a 5D kinematic data set. We used our criteria to search for these pairs in a 150 pc circular field of view surrounding the open cluster M67, which we used as a benchmark cluster to test the robustness of our method. Our results reveal only one RS-RB pair that is consistent with all of our selection criteria out of an initial sample of $10^8$ pairs.

astro-ph.SR↗

arXiv2021

Age and helium content of the open cluster NGC 6791 from multiple eclipsing binary members. III. Constraints from a subgiant

Models of stellar structure and evolution can be constrained using accurate measurements of the parameters of eclipsing binary members of open clusters. Multiple binary stars provide the means to tighten the constraints and, in turn, to improve the precision and accuracy of the age estimate of the host cluster. In the previous two papers of this series, we have demonstrated the use of measurements of multiple eclipsing binaries in the old open cluster NGC6791 to set tighter constraints on the properties of stellar models than was previously possible, thereby improving both the accuracy and precision of the cluster age. We identify and measure the properties of a non-eclipsing cluster member, V56, in NGC\,6791 and demonstrate how this provides additional model constraints that support and strengthen our previous findings. We analyse multi-epoch spectra of V56 from FLAMES in conjunction with the existing photometry and measurements of eclipsing binaries in NGC6971. The parameters of the V56 components are found to be $M_{\rm p}=1.103\pm 0.008 M_{\odot}$ and $M_{\rm s}=0.974\pm 0.007 M_{\odot}$, $R_{\rm p}=1.764\pm0.099 R_{\odot}$ and $R_{\rm s}=1.045\pm0.057 R_{\odot}$, $T_{\rm eff,p}=5447\pm125$ K and $T_{\rm eff,s}=5552\pm125$ K, and surface [Fe/H]=$+0.29\pm0.06$ assuming that they have the same abundance. The derived properties strengthen our previous best estimate of the cluster age of $8.3\pm0.3$ Gyr and the mass of stars on the lower red giant branch (RGB), which is $M_{\rm RGB} = 1.15\pm0.02M_{\odot}$ for NGC6791. These numbers therefore continue to serve as verification points for other methods of age and mass measures, such as asteroseismology.

astro-ph.SR↗

arXiv2018

Constraints on blue straggler formation mechanisms in Galactic globular clusters from proper motion velocity distributions

For a sample of 38 Galactic globular clusters (GCs), we confront the observed distributions of blue straggler (BS) proper motions and masses (derived from isochrone fitting) from the BS catalog of Simunovic & Puzia with theoretical predictions for each of the two main competing BS formation mechanisms. These are mass transfer from an evolved donor on to a main-sequence (MS) star in a close binary system, and direct collisions involving MS stars during binary encounters. We use the \texttt{FEWBODY} code to perform simulations of single-binary and binary-binary interactions. This provides collisional velocity and mass distributions for comparison to the observed distributions. Most clusters are consistent with BSs derived from a dynamically relaxed population, supportive of the binary mass-transfer scenario. In a few clusters, including all the post-core collapse clusters in our sample, the collisional velocities provide the best fit.

astro-ph.SR↗

arXiv2018

The blue straggler V106 in NGC6791: A prototype progenitor of old single giants masquerading as young

We determine the properties of the binary star V106 in the old open cluster NGC6791. We identify the system to be a blue straggler cluster member by using a combination of ground-based and Kepler photometry and multi-epoch spectroscopy. The properties of the primary component are found to be $M_{\rm p}\sim1.67 \rm M_{\odot}$, more massive than the cluster turn-off, with $R_{\rm p}\sim1.91 \rm R_{\odot}$ and $T_{\rm eff}=7110\pm100$ K. The secondary component is highly oversized and overluminous for its low mass with $M_{\rm s}\sim0.182 \rm M_{\odot}$, $R_{\rm s}\sim0.864 \rm R_{\odot}$ and $T_{\rm eff}=6875\pm200$ K. We identify this secondary star as a bloated (proto) extremely low-mass helium white dwarf. These properties of V106 suggest that it represents a typical Algol-paradox system and that it evolved through a mass-transfer phase which provides insight into its past evolution. We present a detailed binary stellar evolution model for the formation of V106 using the MESA code and find that the mass-transfer phase only ceased about 40 Myr ago. Due to the short orbital period (P=1.4463 d) another mass-transfer phase is unavoidable once the current primary star evolves towards the red giant phase. We argue that V106 will evolve through a common-envelope phase within the next 100 Myr and merge to become a single over-massive giant. The high mass will make it appear young for its true age, which is revealed by the cluster properties. Therefore, V106 is potentially a prototype progenitor of old field giants masquerading as young.

astro-ph.SR↗

arXiv2016

The K2 M67 Study: Revisiting old friends with K2 reveals oscillating red giants in the open cluster M67

Observations of stellar clusters have had a tremendous impact in forming our understanding of stellar evolution. The open cluster M67 has a particularly important role as a calibration benchmark for stellar evolution theory due to its near solar composition and age. As a result, it has been observed extensively, including attempts to detect solar-like oscillations in its main sequence and red giant stars. However, any asteroseismic inference has so far remained elusive due to the difficulty in measuring these extremely low amplitude oscillations. Here we report the first unambiguous detection of solar-like oscillations in the red giants of M67. We use data from the Kepler ecliptic mission, K2, to measure the global asteroseismic properties. We find a model-independent seismic-informed distance of 816+/-11pc, or (m-M)o=9.57+/-0.03mag, an average red-giant mass of 1.36+/-0.01Msun, in agreement with the dynamical mass from an eclipsing binary near the cluster turn-off, and ages of individual stars compatible with isochrone fitting. We see no evidence of strong mass loss on the red giant branch. We also determine seismic log g of all the cluster giants with a typical precision of ~0.01dex. Our results generally show good agreement with independent methods and support the use of seismic scaling relations to determine global properties of red giant stars with near solar metallicity. We further illustrate that the data are of such high quality, that future work on individual mode frequencies should be possible, which would extend the scope of seismic analysis of this cluster.

astro-ph.SR↗

arXiv2016

Thermally induced magnetic relaxation in square artificial spin ice

The properties of natural and artificial assemblies of interacting elements, ranging from Quarks to Galaxies, are at the heart of Physics. The collective response and dynamics of such assemblies are dictated by the intrinsic dynamical properties of the building blocks, the nature of their interactions and topological constraints. Here we report on the relaxation dynamics of the magnetization of artificial assemblies of mesoscopic spins. In our model nano-magnetic system - square artificial spin ice - we are able to control the geometrical arrangement and interaction strength between the magnetically interacting building blocks by means of nano-lithography. Using time resolved magnetometry we show that the relaxation process can be described using the Kohlrausch law and that the extracted temperature dependent relaxation times of the assemblies follow the Vogel-Fulcher law. The results provide insight into the relaxation dynamics of mesoscopic nano-magnetic model systems, with adjustable energy and time scales, and demonstrates that these can serve as an ideal playground for the studies of collective dynamics and relaxations.

cond-mat.mes-hall↗

arXiv2014

Temperature evolution of structural and magnetic properties of stoichiometric LiCu2O2: correlation of thermal expansion coefficient and magnetic order

Temperature-dependent crystallographic and magnetic studies on stoichiometric single crystals of LiCu2O2 are reported. The magnetic properties are similar to earlier findings demonstrating antiferromagnetic ordering below 25 K. Evidence of magnetoelastic coupling is observed in the thermal expansion along the c-direction; not only at the low temperature antiferromagnetic transitions, but an anomalous behavior of the thermal expansion indicate magnetoelastic coupling also to the magnetic ordering related to a weak spontaneous magnetic moment appearing at 150 K. Ac-susceptibility measurements at different frequencies and superposed dc- fields are employed to further characterize this magnetic anomaly.

cond-mat.mtrl-sci↗

arXiv2014

Re-entrant superspin glass phase in La$_{0.82}$Ca$_{0.18}$MnO$_3$ ferromagnetic insulator

We report results of magnetization and ac susceptibility measurements down to very low fields on a single crystal of the perovskite manganite, La$_{0.82}$Ca$_{0.18}$MnO$_3$. This composition falls in the intriguing ferromagnetic insulator region of the manganite phase diagram. In contrast to earlier beliefs, our investigations reveal that the system is magnetically (and in every other sense) single-phase with a ferromagnetic ordering temperature of $\sim$ 170 K. However, this ferromagnetic state is magnetically frustrated, and the system exhibits pronounced glassy dynamics below 90 K. Based on measured dynamical properties, we propose that this quasi-long-ranged ferromagnetic phase, and associated superspin glass behavior, is the true magnetic state of the system, rather than being a macroscopic mixture of ferromagnetic and antiferromagnetic phases as often suggested. Our results provide an understanding of the quantum phase transition from an antiferromagnetic insulator to a ferromagnetic metal via this ferromagnetic insulating state as a function of $x$ in La$_{1-x}$Ca$_x$MnO$_3$, in terms of the possible formation of magnetic polarons.

cond-mat.str-el↗

arXiv2013

Chemical pressure effects on structural, dielectric and magnetic properties of solid solutions Mn3-xCoxTeO6

The effects of Co2+ doping on the structural, magnetic and dielectric properties of the multiferroic frustrated antiferromagnet Mn3TeO6 have been investigated. Ceramic samples of the solid solution series Mn3-xCoxTeO6 were prepared by a solid-state reaction route. X-ray and neutron powder diffraction and electron microscopy techniques were combined with calorimetric, dielectric and magnetic measurements to investigate the dependence of the crystal structure and physical properties on temperature and composition. It is shown that the compounds with x up to 2.4 all adopt the trigonal corundum-related structure of pure Mn3TeO6 (space group R-3) in the temperature range 5-295 K and that the lattice parameters a and c and the unit-cell volume V decrease linearly with increasing Co2+ concentration. The low- temperature magnetic susceptibility and heat capacity data evidence the antiferromagnetic ordering of all samples. The Neel temperature linearly increases with Co2+ concentration x. Curie-Weiss fits of the high temperature susceptibility indicate that the magnetic frustration decreases with x. The derived magnetic structure of Mn3TeO6 can be described as an incommensurately modulated magnetic spin state with k = [0, 0, kz] and an elliptical spin- spiral order of spins within the chains of MnO6 octahedra. With increasing Co2+ concentration the propagation vector kz changes from 0.453 (x = 0) to 0.516 (x = 2.4). The magnetic anisotropy changes as well, leading to a reorientation of the spiral-basal plane. A possible coexistence of long-range order of electrical dipoles and magnetic moments in Mn3-xCoxTeO6 is discussed.

cond-mat.mtrl-sci↗

arXiv2013

Enhancement of antiferromagnetic interaction and transition temperature in M3TeO6 systems (M = Mn, Co, Ni, Cu)

Several M3 TeO6 (M = Mn, Co, Ni, Cu) oxides order antiferromagnetically at low temperatures (near or below 60 K), while displaying interesting dielectric properties at high temperatures (ferroelectricity below 1000 K in M = Ni case). We have investigated and analyzed the structural and magnetic properties of Mn-doped Co3 TeO6 and Ni3 TeO6, which order antiferromagnetically at temperatures higher than their undoped counterparts.

cond-mat.str-el↗

arXiv2013

Electronic superlattice revealed by resonant scattering from random impurities in Sr3Ru2O7

Resonant elastic x-ray scattering (REXS) is an exquisite element-sensitive tool for the study of subtle charge, orbital, and spin superlattice orders driven by the valence electrons, which therefore escape detection in conventional x-ray diffraction (XRD). Although the power of REXS has been demonstrated by numerous studies of complex oxides performed in the soft x-ray regime, the cross section and photon wavelength of the material-specific elemental absorption edges ultimately set the limit to the smallest superlattice amplitude and periodicity one can probe. Here we show -- with simulations and REXS on Mn-substituted Sr$_3$Ru$_2$O$_7$ -- that these limitations can be overcome by performing resonant scattering experiments at the absorption edge of a suitably-chosen, dilute impurity. This establishes that -- in analogy with impurity-based methods used in electron-spin-resonance, nuclear-magnetic resonance, and M\"ossbauer spectroscopy -- randomly distributed impurities can serve as a non-invasive, but now momentum-dependent probe, greatly extending the applicability of resonant x-ray scattering techniques.

cond-mat.str-el↗

arXiv2013

Phase transition in a super superspin glass

We here confirm the occurrence of spin glass phase transition and extract estimates of associated critical exponents of a highly monodisperse and densely compacted system of bare maghemite nanoparticles. This system has earlier been found to behave like an archetypal spin glass, with e.g. a sharp transition from paramagnetic to non-equilibrium behavior, suggesting that this system undergoes a spin-glass phase transition at a relatively high temperature, $T_g$ $\sim$ 140 K.

cond-mat.dis-nn↗

arXiv2013

Spin and Dipole Ordering in Ni_2InSbO_6 and Ni_2ScSbO_6 with corundum-related structure

The complex metal oxides Ni2InSbO6 (NISO) and Ni2ScSbO6 (NSSO) have been prepared in form of polycrystalline powders by a solid state reaction route. The crystal structure and magnetic properties of the compounds were investigated using a combination of X-ray and neutron powder diffraction, electron microscopy, calorimetric and magnetic measurements. The compounds adopt a trigonal structure, space group R3, of the corundum related Ni3TeO6 (NTO) type. Only one of the octahedral Ni positions (Ni(2)) of the NTO structure was found to be occupied by In (Sc). NTO has non-centrosymmetric structure and is ferroelectric below 1000 K, dielectric and second harmonic measurements suggest that also NISO and NSSO are correspondingly ferroelectric. Magnetization measurements signified antiferromagnetic ordering below TN=60 K (NSSO) and 76 K (NISO). The magnetic structure is formed by two antiferromagnetically coupled incommensurate helices with the spiral axis along the b-axis and propagation vector k = [0, ky,0] with ky= 0.036(1) (NSSO) and ky= 0.029(1) (NISO). The observed structural and magnetic properties of NISO and NSSO are discussed and compared with those of NTO.

cond-mat.mtrl-sci↗

arXiv2012

High-temperature structural phase transition in multiferroic LiCu_2O_2

LiCu_2O_2 single crystals were studied in the temperature range 300-1100 K by means of heating-cooling curves of differential thermal analysis (DTA), thermogravimetry (TG), X-ray powder diffraction and electrical measurements. A reversible first-order phase transition between orthorhombic and tetragonal phases was found to take place at 993 K. At the transition, a peak is observed in the DTA curves, as well as jumps of the unit cell parameters and electrical resistivity. Considering the crystal structure of LiCu_2O_2 and the entropy change associated with the phase transition, it is concluded that the phase transition is related to processes of order-disorder of the Cu2+ and Li+ cations onto their crystallographic positions.

cond-mat.mtrl-sci↗

arXiv2012

Mn$_2$FeSbO$_6$: a ferrimagnetic ilmenite and an antiferromagnetic perovskite

Due of its polymorphism, Mn$_2$FeSbO$_6$ can be synthesized at high pressures and temperatures as a ferrimagnetic ilmenite or an antiferromagnetic perovskite. The structural phase transformation is discussed in detail, and magnetic structures are proposed for both phases. The high-pressure Mn$_2$FeSbO$_6$ polymorph is a rare example of $A_2 B'B"$O$_6$ perovskite with solely Mn cations on the $A$-site. Fe and Sb cations are ordered on the $B$-sites. Theoretical calculations for the perovskite phase suggest a complex magnetic structure, holding an electronic polarization.

cond-mat.str-el↗

arXiv2012

Preparation, structural, dielectric and magnetic properties of LaFeO3-PbTiO3 solid solutions

Solid solutions of (1-x)LaFeO3-(x)PbTiO3 (0<x<1) have been prepared by conventional solid-state reaction. These complex perovskites have been studied by means of X-ray (XRPD) and neutron powder (NPD) diffraction, complemented with dielectric, magnetic, heat capacity and M\"ossbauer measurements. Complete solubility in the perovskite series was demonstrated. The NPD and XRPD patterns were successfully refined as orthorhombic (x \leq 0.7) and tetragonal (x \geq 0.8). A composition-driven phase transformation occurs within the interval 0.7<x<0.8. The samples with x<0.5 showed evidence of long-range magnetic ordering with an G-type antiferromagnetic arrangement of the magnetic moments of the Fe3+ cations in the B-site with propagation vector k = (0,0,0). Based on the obtained experimental data, a combined structural and magnetic phase diagram has been constructed. The factors governing the structural, dielectric and magnetic properties of (1-x) LaFeO3 - (x)PbTiO3 solid solutions are discussed, as well as their possible multiferroicity.

cond-mat.mtrl-sci↗