arXiv subjects

R. Popescu

Publications and source records attributed to R. Popescu.

7 recordsLinked to original sources

arXiv2026

ALMA Chemical Evolution (ACE) survey: The gas fundamental metallicity relation at cosmic noon

Chemical enrichment shapes how galaxies form and evolve. The gas-phase metallicity is directly linked to the stellar mass, star formation rate, and cold gas of the interstellar medium. Thus, the cold gas fundamental metallicity relation (GFMR) is a powerful tool for probing galaxy evolution, bridging large-scale gas flows modulating the cold gas reservoir and small-scale metal enrichment tracing the cumulative impact of star formation. Constraining all these properties for the same representative sample of galaxies remains challenging yet essential. Using CO(3--2) band 3 observations from the Atacama Large Millimeter/submillimeter Array Chemical Evolution (ACE) survey, we investigated the GFMR in a sample of 26 main-sequence (log(M_*, med)=9.96), subsolar-metallicity (12+log(O/H)_med=8.44) star-forming galaxies (SFGs) at z~2. With 17/26 CO detections, including some of the lowest-metallicity CO detections at cosmic noon, we find that the stellar mass remains the primary driver of the chemical evolution in our sample (sigmaMZR~0.10). Whereas the molecular gas likely plays a secondary role (sigmaGFMR~0.11) similar to that of the star formation rate (sigmaFMR~0.13). This likely reflects our sensitivity to only the CO-bright component of the molecular reservoir. Our results remain consistent with gas-regulator models and suggest the existence of efficient molecular outflows, with an average mass loading factor of eta~4, regulating star formation and chemical enrichment.

astro-ph.GA↗

arXiv2026

ALMA Chemical Evolution (ACE) survey: dust-to-gas ratios in sub-solar metallicity galaxies at cosmic noon

Dust is a fundamental component of the interstellar medium and provides a key tracer of the baryon cycle that regulates galaxy evolution. The dust-to-gas ratio links metals in the gas phase to those locked into dust grains, making it a sensitive diagnostic of dust production, grain growth, and destruction. We present measurements of the dust-to-molecular-gas ratio ($\rm DGR_{mol}$), for typical star-forming galaxies ($\log M_\star \approx 10$) at sub-solar metallicites, at $z\simeq2-2.5$ from the ALMA Chemical Evolution (ACE) survey. By combining ALMA CO and dust-continuum observations with robust gas-phase metallicity measurements, ACE extends direct dust and molecular-gas measurements to lower stellar masses and lower metallicities than previously available at this epoch, reaching down to $0.4\,Z_{\odot}$. This enables the first constraints on the $\rm DGR_{mol}$--metallicity relation for typical unlensed galaxies at cosmic noon. We find that $\rm DGR_{mol}$ increases with metallicity, with a log-space slope of $1.2 \pm 0.7$, indicating that metal-poor galaxies have systematically lower $\rm DGR_{mol}$ than their more metal-rich counterparts. For the detected ACE galaxies, we measure a mean value of $\log_{10}(M_{\rm dust}/M_{\rm mol})=-2.37\pm0.05$ for a mean metallicity of 12+$\log (\rm O/H) = 8.45 \pm 0.02$. We find agreement with $\rm DGR_{mol}$ in the local Universe at fixed metallicities, indicating that the same dust-growth physics, likely grain growth in the ISM, dominates at metallicities of $8.3 \leq 12+\log(\rm O/H) \leq 8.7$ at cosmic noon. These measurements provide novel empirical constraints for models of dust enrichment and galaxy evolution during the peak epoch of cosmic star formation. Additionally, ACE provides a sub-solar metallicity reference for the calibration of dust continuum as tracer of molecular gas, essential for studying metal-poor, high-redshift systems.

astro-ph.GA↗

arXiv2026

ALMA Chemical Evolution (ACE) survey: the dust content of subsolar metallicity galaxies at cosmic noon

Dust plays a key role in galaxy evolution by influencing star formation and shaping the observed spectrum of galaxies. However, at z~2 (cosmic noon) our knowledge of the dust mass budget is currently limited to the most massive, metal-rich systems, which are not representative of the bulk galaxy population. Here, we probe the lower mass, subsolar metallicity regime by measuring the dust mass of 25 galaxies at z~2.3 from the ALMA Chemical Evolution (ACE) Large Program. The sample contains star-forming galaxies in the COSMOS field with robust strong-line metallicities down to ~0.3 $Z_\odot$. Using the dust continuum emission detected at 873micron or 1.3mm we constrain the dust mass by assuming an optically thin single-temperature modified blackbody. The resulting dust masses average $10^{8}\,\mathrm{M}_\odot$, and they are three to nine times larger than those of z=0 galaxies at a matched metallicity and stellar mass. We also find positive correlations between dust mass and stellar mass, metallicity, and star formation rate (SFR). In contrast, we find that the $M_\mathrm{dust}/M_\mathrm{stars}$ (DtS) ratio scatters around $10^{-2.2}$ but shows no evidence of correlation with metallicity. This result is consistent with dust evolution models that predict a constant DtS once the ISM reaches the critical metallicity, at which metal accretion onto grains becomes the main mode of dust buildup. The correlation between $M_\mathrm{dust}/\mathrm{SFR}$ and metallicity also suggest that ACE galaxies have already surpassed the critical metallicity. Finally, we find that the DtS ratio is correlated to the specific SFR (sSFR). Since the sSFR are high ($> 10^{-8}\,\mathrm{yr}^{-1}$) this explains the DtS excess over z~0 galaxies. In turn, both sSFR and DtS are likely driven by the molecular gas fraction, as supported by CO(3-2) measurements taken as part of ACE.

astro-ph.GA↗

arXiv2020

Phonon density of states in lanthanide-based nanocrystals

We report a combined inelastic neutron and X-ray scattering study of the phonon density of states of the nano- and microcrystalline lanthanide-based materials NaY$_{0.8}$Yb$_{0.18}$Er$_{0.02}$F$_4$ and NaGd$_{0.8}$Yb$_{0.18}$Er$_{0.02}$F$_4$. While large (20 nm) nanocrystals display the same vibrational spectra as their microcrystalline counterparts, we find an enhanced phonon density of states at low energies, $E \leq 15\,\rm{meV}$, in ultra-small (5 nm) NaGd$_{0.8}$Yb$_{0.18}$Er$_{0.02}$F$_4$ nanocrystals which we assign to an increased relative spectral weight of surface phonon modes. Based on our observations for ultra-small nanocrystals, we rationalize that an increase of the phonon density of states in large nanocrystals due to surface phonons is too small to be observed in the current measurements. The experimental approach described in this report constitutes the first step toward the rationalization of size effects on the modification of the absolute upconversion quantum yield of upconverting nanocrystals.

cond-mat.mes-hall↗

arXiv2011

Quantitative High-Resolution Transmission Electron Microscopy of Single Atoms

Single atoms can be considered as basic objects for electron microscopy to test the microscope performance and basic concepts for modeling of image contrast. In this work high-resolution transmission electron microscopy was applied to image single platinum atoms in an aberration-corrected transmission electron microscope. The atoms are deposited on a self-assembled monolayer substrate which induces only negligible contrast. Single-atom contrast simulations were performed on the basis of Weickenmeier-Kohl and Doyle-Turner scattering factors. Experimental and simulated intensities are in full agreement on an absolute scale.

cond-mat.mtrl-sci↗

arXiv2007

Increase of the mean inner Coulomb potential in Au clusters induced by surface tension and its implication for electron scattering

Electron holography in a transmission electron microscope was applied to measure the phase shift induced by Au clusters as a function of the cluster size. Large phase shifts Df observed for small Au clusters cannot be described by the well-known equation Df=C_E V_0 t (C_E: interaction constant, V_0: mean inner Coulomb potential (MIP) of bulk gold, t: cluster thickness). The rapid increase of the Au MIP with decreasing cluster size derived from Df, can be explained by the compressive strain of surface atoms in the cluster.

cond-mat.mtrl-sci↗

arXiv2002

Generalized Isoscaling of Isotopic Distributions

Generalized isoscaling relationships are proposed that may permit one to relate the isotopic distributions of systems that may not be at the same temperature. The proposed relationships are applied to multifragmentation excitation functions for central Kr+Nb and Ar+Sc collisions.

nucl-ex↗