arXiv subjects

Raphael Lopes

Publications and source records attributed to Raphael Lopes.

At least 19 recordsLinked to original sources

arXiv2026

Coexisting Regular and Chaotic Dynamics in the Dysprosium Feshbach Spectrum

Strongly dipolar gases, such as dysprosium, erbium and thulium, exhibit dense Feshbach spectra whose level statistics have been associated with quantum chaos arising from couplings among many molecular channels. Here, we combine a precise calibration of the Feshbach spectrum of $^{162}$Dy with spectroscopic measurements of the differential magnetic moments of bound states associated with more than 80 resonances between 0 and 30 G. These magnetic moments provide an eigenstate-sensitive probe of the molecular states underlying the resonance spectrum. We find that the level statistics are not uniform: resonances associated with states near the center of the magnetic-moment distribution display enhanced level repulsion, whereas those near the lower edge remain close to Poisson statistics. Our results reveal hidden structure within the chaotic dysprosium Feshbach spectrum and identify molecular-state composition as a key ingredient in the emergence of quantum chaos in strongly dipolar scattering.

cond-mat.quant-gas↗

arXiv2026

Determination of the ground state polarizability of $^{162}$Dy near 530 nm

Open-shell lanthanide atoms, and dysprosium in particular, combine a large ground-state angular momentum with dense electronic spectra, making their dynamical polarizability strongly dependent on wavelength and internal state and therefore particularly challenging to characterize accurately. This issue has become especially relevant with the recent development of single-atom trapping of dysprosium in optical-tweezer arrays, where precise knowledge of the polarizability is needed to design optimized trapping architectures. Here, we exploit the strong spin-dependent light shift near the $J'=J-1$ intercombination line at 530.306 nm to determine the background scalar and vector polarizabilities of $^{162}$Dy in its ground state near this wavelength. Our measurements quantitatively agree with atomic-structure calculations and provide new insight into the contributions of nearby transitions in a spectral region relevant to emerging dysprosium tweezer platforms.

cond-mat.quant-gas↗

arXiv2026

A two-dimensional realization of the parity anomaly

Quantum anomalies arise when symmetries of a classical theory cannot be preserved upon quantization, leading to unconventional topological responses. A prominent example is the parity anomaly of a single two-dimensional Dirac fermion, which enforces a half-quantized Hall response. Anomaly inflow mechanism allows this effect to be observed at the surfaces of three-dimensional topological insulators, however, its realization in a genuinely two-dimensional system has remained elusive. Here we report the observation of a parity-anomalous Hall response at the critical point of a quantum Hall topological phase transition in a synthetic two-dimensional system of ultracold dysprosium atoms. By coupling a continuous spatial dimension to a finite synthetic dimension encoded in atomic spin states, we engineer tunable Chern bands with C = 0 and 1. At the transition, the bulk gap closes at a single Dirac point, where we observe a robust half-quantized Hall drift despite strong non-adiabatic excitations. We show that this response originates from the global structure of the band topology, is protected by an emergent parity symmetry at criticality, and disappears when parity is explicitly broken. Our work establishes synthetic quantum systems as a powerful platform to probe quantum anomalies and their interplay with topology and non-equilibrium dynamics.

cond-mat.quant-gas↗

arXiv2025

Two-Body Contact Dynamics in a Bose Gas near a Fano-Feshbach Resonance

We investigate the real-time buildup of short-range correlations in a nondegenerate ultracold Bose gas near a narrow Fano-Feshbach resonance. Using rapid optical control, we quench the closed-channel molecular energy to resonance on submicrosecond timescales and track the evolution of the two-body contact through photodissociation losses. Repeated pulse sequences enhance sensitivity to early-time two-body losses and reveal long-lived coherence between atom pairs and molecular states. The observed dynamics are accurately reproduced by our dynamical two-channel zero-range theory, which explicitly accounts for the resonance's narrow width and finite closed-channel decay, establishing a predictive framework for correlation dynamics in quantum gases near Fano-Feshbach resonances.

cond-mat.quant-gas↗

arXiv2024

Production and stabilization of a spin mixture of ultracold dipolar Bose gases

Mixtures of ultracold gases with long-range interactions are expected to open new avenues in the study of quantum matter. Natural candidates for this research are spin mixtures of atomic species with large magnetic moments. However, the lifetime of such assemblies can be strongly affected by the dipolar relaxation that occurs in spin-flip collisions. Here we present experimental results for a mixture composed of the two lowest Zeeman states of $^{162}$Dy atoms, that act as dark states with respect to a light-induced quadratic Zeeman effect. We show that, due to an interference phenomenon, the rate for such inelastic processes is dramatically reduced with respect to the Wigner threshold law. Additionally, we determine the scattering lengths characterizing the s-wave interaction between these states, providing all necessary data to predict the miscibility range of the mixture, depending on its dimensionality.

cond-mat.quant-gas↗

arXiv2024

Dynamics of spatial phase coherence in a dissipative Bose-Hubbard atomic system

We investigate the loss of spatial coherence of one-dimensional bosonic gases in optical lattices illuminated by a near-resonant excitation laser. Because the atoms recoil in a random direction after each spontaneous emission, the atomic momentum distribution progressively broadens. Equivalently, the spatial correlation function (the Fourier-conjugate quantity of the momentum distribution) progressively narrows down as more photons are scattered. Here we measure the correlation function of the matter field for fixed distances corresponding to nearest-neighbor (n-n) and next-nearest-neighbor (n-n-n) sites of the optical lattice as a function of time, hereafter called n-n and n-n-n correlators. For strongly interacting lattice gases, we find that the n-n correlator $C_1$ decays as a power-law at long times, $C_1\propto 1/t^{\alpha}$, in stark contrast with the exponential decay expected for independent particles. The power-law decay reflects a non-trivial dissipative many-body dynamics, where interactions change drastically the interplay between fluorescence destroying spatial coherence, and coherent tunnelling between neighboring sites restoring spatial coherence at short distances. The observed decay exponent $\alpha \approx 0.54(6) $ is in good agreement with the prediction $\alpha=1/2$ from a dissipative Bose-Hubbard model accounting for the fluorescence-induced decoherence. Furthermore, we find that the n-n correlator $C_1$ controls the n-n-n correlator $C_2$ through the relation $C_2 \approx C_1^2$, also in accordance with the dissipative Bose-Hubbard model.

cond-mat.quant-gas↗

arXiv2023

Loss features in ultracold $^{162}$Dy gases: two- versus three-body processes

Dipolar gases like erbium and dysprosium have a dense spectrum of resonant loss features associated with their strong anisotropic interaction potential. These resonances display various behaviours with density and temperature, implying diverse microscopic properties. Here, we quantitatively investigate the low-field ($B < 6\,\text{G}$) loss features in ultracold thermal samples of $^{162}$Dy, revealing two- and three-body dominated loss processes. We investigate their temperature dependence and detect a feature compatible with a $d$-wave Fano-Feshbach resonance, which has not been observed before. We also analyse the expansion of the dipolar Bose-Einstein condensate as a function of the magnetic field and interpret the changes in size close to the resonances with a variation in the scattering length.

cond-mat.quant-gas↗

arXiv2023

Realizing the entanglement Hamiltonian of a topological quantum Hall system

Topological quantum many-body systems, such as Hall insulators, are characterized by a hidden order encoded in the entanglement between their constituents. Entanglement entropy, an experimentally accessible single number that globally quantifies entanglement, has been proposed as a first signature of topological order. Conversely, the full description of entanglement relies on the entanglement Hamiltonian, a more complex object originally introduced to formulate quantum entanglement in curved spacetime. As conjectured by Li and Haldane, the entanglement Hamiltonian of a many-body system appears to be directly linked to its boundary properties, making it particularly useful for characterizing topological systems. While the entanglement spectrum is commonly used to identify complex phases arising in numerical simulations, its measurement remains an outstanding challenge. Here, we perform a variational approach to realize experimentally, as a genuine Hamiltonian, the entanglement Hamiltonian of a synthetic quantum Hall system. We use a synthetic dimension, encoded in the electronic spin of dysprosium atoms, to implement spatially deformed Hall systems, as suggested by the Bisognano-Wichmann prediction. The spectrum of the optimal variational Hamiltonian exhibits a chiral dispersion akin to a topological edge mode, revealing the fundamental link between entanglement and boundary physics. Our variational procedure can be easily generalized to interacting many-body systems on various platforms, marking an important step towards the exploration of exotic quantum systems with long-range correlations, such as fractional Hall states, chiral spin liquids and critical systems.

cond-mat.quant-gas↗

arXiv2022

Realization of an atomic quantum Hall system in four dimensions

Modern condensed matter physics relies on the concept of topology to classify matter, from quantum Hall systems to topological insulators. Engineered systems, benefiting from synthetic dimensions, can potentially give access to novel topological states predicted in dimensions $D > 3$. We report the realization of an atomic quantum Hall system evolving in four dimensions (4D), with two spatial dimensions and two synthetic ones encoded in the large spin of dysprosium atoms. The non-trivial topology is evidenced by measuring a quantized electromagnetic non-linear response and observing anisotropic hyperedge modes. We also excite non-planar cyclotron motion, contrasting with its circular equivalents in $D\leq3$. Our work opens to the investigation of strongly-correlated topological liquids in 4D generalizing fractional quantum Hall states.

cond-mat.quant-gas↗

arXiv2021

Laughlin's topological charge pump in an atomic Hall cylinder

The quantum Hall effect occuring in two-dimensional electron gases was first explained by Laughlin, who envisioned a thought experiment that laid the groundwork for our understanding of topological quantum matter. His proposal is based on a quantum Hall cylinder periodically driven by an axial magnetic field, resulting in the quantized motion of electrons. We realize this milestone experiment with an ultracold gas of dysprosium atoms, the cyclic dimension being encoded in the electronic spin and the axial field controlled by the phases of laser-induced spin-orbit couplings. Our experiment provides a straightforward manifestation of the non-trivial topology of quantum Hall insulators, and could be generalized to strongly-correlated topological systems.

cond-mat.quant-gas↗

arXiv2021

Simulating two-dimensional dynamics within a large-size atomic spin

Encoding a dimension in the internal degree of freedom of an atom provides an interesting tool for quantum simulation, facilitating the realization of artificial gauge fields. We propose an extension of the synthetic dimension toolbox, making it possible to encode two dimensions within a large atomic spin. The protocol combines first- and second-order spin couplings, such that the spin projection $m$ and the remainder $r=m$ (mod 3) of its Euclidian division by 3 act as orthogonal coordinates on a synthetic cylinder. It is suited for an implementation with lanthanide atoms, which feature a large electronic spin and narrow optical transitions for applying the required spin couplings. This method is useful for simulating geometries with periodic boundary conditions, and engineering various types of topological systems evolving in high dimensions.

cond-mat.quant-gas↗

arXiv2021

Partitioning dysprosium's electronic spin to reveal entanglement in non-classical states

Quantum spins of mesoscopic size are a well-studied playground for engineering non-classical states. If the spin represents the collective state of an ensemble of qubits, its non-classical behavior is linked to entanglement between the qubits. In this work, we report on an experimental study of entanglement in dysprosium's electronic spin. Its ground state, of angular momentum $J=8$, can formally be viewed as a set of $2J$ qubits symmetric upon exchange. To access entanglement properties, we partition the spin by optically coupling it to an excited state $J'=J-1$, which removes a pair of qubits in a state defined by the light polarization. Starting with the well-known W and squeezed states, we extract the concurrence of qubit pairs, which quantifies their non-classical character. We also directly demonstrate entanglement between the 14- and 2-qubit subsystems via an increase in entropy upon partition. In a complementary set of experiments, we probe decoherence of a state prepared in the excited level $J'=J+1$ and interpret spontaneous emission as a loss of a qubit pair in a random state. This allows us to contrast the robustness of pairwise entanglement of the W state with the fragility of the coherence involved in a Schr\"odinger cat state. Our findings open up the possibility to engineer novel types of entangled atomic ensembles, in which entanglement occurs within each atom's electronic spin as well as between different atoms.

quant-ph↗

arXiv2021

Radio-frequency evaporation in an optical dipole trap

We present an evaporative cooling technique for atoms trapped in an optical dipole trap that benefits from narrow optical transitions. For an appropriate choice of wavelength and polarization, a single laser beam leads to opposite light-shifts in two internal states of the lowest energy manifold. Radio-frequency coupling between these two states results in evaporative cooling at a constant trap stiffness. The evaporation protocol is well adapted to several atomic species, in particular to the case of Lanthanides such as Er, Dy, and fermionic Yb, but also to alkali-earth metals such as fermionic Sr. We derive the dimensionless expressions that allow us to estimate the evaporation efficiency. As a concrete example, we consider the case of $^{162}$Dy and present a numerical analysis of the evaporation in a dipole trap near the $J'=J$ optical transition at 832 nm. We show that this technique can lead to runaway evaporation in a minimalist experimental setup.

cond-mat.quant-gas↗

arXiv2020

Observation of first and second sound in a BKT superfluid

Superfluidity in its various forms has fascinated scientists since the observation of frictionless flow in liquid helium II. In three spatial dimensions (3D), it is conceptually associated with the emergence of long-range order (LRO) at a critical temperature $T_{\text{c}}$. One of its hallmarks, predicted by the highly successful two-fluid model and observed in both liquid helium and ultracold atomic gases, is the existence of two kinds of sound excitations, the first and second sound. In 2D systems, thermal fluctuations preclude LRO, but superfluidity nevertheless emerges at a nonzero $T_{\text{c}}$ via the infinite-order Berezinskii-Kosterlitz-Thouless (BKT) transition, which is associated with a universal jump in the superfluid density $n_{\text{s}}$ without any discontinuities in the fluid's thermodynamic properties. BKT superfluids are also predicted to support two sounds, but the observation of this has remained elusive. Here we observe first and second sound in a homogeneous 2D atomic Bose gas, and from the two temperature-dependent sound speeds extract its superfluid density. Our results agree with BKT theory, including the prediction for the universal superfluid-density jump.

cond-mat.quant-gas↗

arXiv2020

Many-body Decay of the Gapped Lowest Excitation of a Bose-Einstein Condensate

We study the decay mechanism of the gapped lowest-lying excitation of a quasi-pure box-trapped atomic Bose-Einstein condensate. Owing to the absence of lower-energy modes, or direct coupling to an external bath, this excitation is protected against one-body (linear) decay and the damping mechanism is exclusively nonlinear. We develop a universal theoretical model that explains this fundamental nonlinear damping as a process whereby two quanta of the gapped lowest excitation mode couple to a higher-energy mode, which subsequently decays into a continuum. We find quantitative agreement between our experiments and the predictions of this model. Finally, by strongly driving the system below its (lowest) resonant frequency we observe third-harmonic generation, a hallmark of nonlinear behavior.

cond-mat.quant-gas↗

arXiv2020

Probing chiral edge dynamics and bulk topology of a synthetic Hall system

Quantum Hall systems are characterized by the quantization of the Hall conductance -- a bulk property rooted in the topological structure of the underlying quantum states. In condensed matter devices, material imperfections hinder a direct connection to simple topological models. Artificial systems, such as photonic platforms or cold atomic gases, open novel possibilities by enabling specific probes of topology or flexible manipulation e.g. using synthetic dimensions. However, the relevance of topological properties requires the notion of a bulk, which was missing in previous works using synthetic dimensions of limited sizes. Here, we realize a quantum Hall system using ultracold dysprosium atoms, in a two-dimensional geometry formed by one spatial dimension and one synthetic dimension encoded in the atomic spin $J=8$. We demonstrate that the large number of magnetic sublevels leads to distinct bulk and edge behaviors. Furthermore, we measure the Hall drift and reconstruct the local Chern marker, an observable that has remained, so far, experimentally inaccessible. In the center of the synthetic dimension -- a bulk of 11 states out of 17 -- the Chern marker reaches 98(5)\% of the quantized value expected for a topological system. Our findings pave the way towards the realization of topological many-body phases.

cond-mat.quant-gas↗

arXiv2019

Probing quantum criticality and symmetry breaking at the microscopic level

We report on an experimental study of the Lipkin-Meshkov-Glick model of quantum spins interacting at infinite range in a transverse magnetic field, which exhibits a ferromagnetic phase transition in the thermodynamic limit. We use Dysprosium atoms of electronic spin $J=8$, subjected to a quadratic Zeeman light shift, to simulate $2J=16$ interacting spins $1/2$. We probe the system microscopically using single magnetic sublevel resolution, giving access to the spin projection parity, which is the collective observable characterizing the underlying $\mathbb{Z}_2$ symmetry. We measure the thermodynamic properties and dynamical response of the system, and study the quantum critical behavior around the transition point. In the ferromagnetic phase, we achieve coherent tunneling between symmetry-broken states, and test the link between symmetry breaking and the appearance of a finite order parameter.

cond-mat.quant-gas↗

arXiv2019

Enhanced magnetic sensitivity with non-gaussian quantum fluctuations

The precision of a quantum sensor can overcome its classical counterpart when its constituents are entangled. In gaussian squeezed states, quantum correlations lead to a reduction of the quantum projection noise below the shot noise limit. However, the most sensitive states involve complex non-gaussian quantum fluctuations, making the required measurement protocol challenging. Here we measure the sensitivity of non-classical states of the electronic spin $J = 8$ of dysprosium atoms, created using light-induced non-linear spin coupling. Magnetic sublevel resolution enables us to reach the optimal sensitivity of non-gaussian (oversqueezed) states, well above the capability of squeezed states and about half the Heisenberg limit.

cond-mat.quant-gas↗