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Ronny Thomale

Publications and source records attributed to Ronny Thomale.

At least 181 records · Page 10Linked to original sources
arXiv2019

Ultrafast electron calorimetry uncovers a new long-lived metastable state in 1T-TaSe$_2$ mediated by mode-selective electron-phonon coupling

Quantum materials represent one of the most promising frontiers in the quest for faster, lightweight, energy efficient technologies. However, their inherent complexity and rich phase landscape make them challenging to understand or manipulate in useful ways. Here we present a new ultrafast electron calorimetry technique that can systematically uncover new phases of quantum matter. Using time- and angle-resolved photoemission spectroscopy, we measure the dynamic electron temperature, band structure and heat capacity. We then show that this is a very sensitive probe of phase changes in materials, because electrons react very quickly, and moreover generally are the smallest component of the total heat capacity. This allows us to uncover a new long-lived metastable state in the charge density wave material 1T-TaSe$_2$, that is distinct from all of the known equilibrium phases: it is characterized by a significantly reduced effective heat capacity that is only 30% of the normal value, due to selective electron-phonon coupling to a subset of phonon modes. As a result, significantly less energy is required to melt the charge order and transform the state of the material than under thermal equilibrium conditions.

cond-mat.mtrl-sci↗
arXiv2019

Quantum and Classical Phases of the Pyrochlore Heisenberg Model with Competing Interactions

We investigate the quantum Heisenberg model on the pyrochlore lattice for a generic spin $S$ in the presence of nearest-neighbor $J_{1}$ and second-nearest-neighbor $J_{2}$ exchange interactions. By employing the pseudofermion functional renormalization group method, we find, for $S=1/2$ and $S=1$, an extended quantum-spin-liquid phase centered around $J_{2}=0$, which is shown to be robust against the introduction of breathing anisotropy. The effects of temperature, quantum fluctuations, breathing anisotropies, and a $J_{2}$ coupling on the nature of the scattering profile, and the pinch points, in particular, are studied. For the magnetic phases of the $J_{1}$-$J_{2}$ model, quantum fluctuations are shown to renormalize phase boundaries compared to the classical model and to modify the ordering wave vectors of spiral magnetic states, while no new magnetic orders are stabilized.

cond-mat.str-el↗
arXiv2018

Towards Topological Quasi-Freestanding Stanene via Substrate Engineering

In search for a new generation of spintronics hardware, material candidates for room temperature quantum spin Hall effect (QSHE) have become a contemporary focus of investigation. Inspired by the original proposal for QSHE in graphene, several heterostructures have been synthesized, aiming at a hexagonal monolayer of heavier group IV elements in order to promote the QSHE bulk gap via increased spin-orbit coupling. So far, however, the monolayer/substrate coupling, which can manifest itself in strain, deformation, and hybridization, has proven to be detrimental to the aspired QSHE conditions for the monolayer. Specifically focusing on stanene, the Sn analogue of graphene, we investigate how an interposing buffer layer mediates between monolayer and substrate in order to optimize the QSHE setting. From a detailed density functional theory study, we highlight the principal mechanisms induced by such a buffer layer to accomplish quasi-free standing stanene in its QSHE phase. We complement our theoretical predictions by presenting the first real attempts to grow a buffer layer on SiC(0001) on which stanene can be deposited.

cond-mat.mtrl-sci↗
arXiv2018

Unconventional superconductivity in a doped quantum spin Hall insulator

A monolayer of jacutingaite (Pt$_2$HgSe$_3$) has recently been identified as a novel quantum spin Hall insulator. By first-principles calculations, we study its Fermiology in the doped regime and unveil a type-I and type-II van Hove singularity for hole and electron doping, respectively. We find that the common link between the propensity for a topological band gap at pristine filling and unconventional superconductivity at finite doping roots in the longer ranged hybridization integrals on the honeycomb lattice. In a combined effort of random phase approximation and functional renormalization group, we find chiral $d$-wave order for the type-I and odd-parity $f$-wave order for the type-II regime.

cond-mat.supr-con↗
arXiv2018

Custodial glide symmetry of quantum spin Hall edge modes in WTe$_2$ monolayer

A monolayer of WTe$_2$ has been shown to display quantum spin Hall (QSH) edge modes persisting up to 100~K in transport experiments. Based on density-functional theory calculations and symmetry-based model building including the role of correlations and substrate support, we develop an effective electronic model for WTe$_2$ which fundamentally differs from other prototypical QSH settings: we find that the extraordinary robustness of quantum spin Hall edge modes in WTe$_2$ roots in a glide symmetry due to which the topological gap opens away from high-symmetry points in momentum space. While the indirect bulk gap is much smaller, the glide symmetry implies a large direct gap of up to 1~eV in the Brillouin zone region of the dispersing edge modes, and hence enables sharply boundary-localized QSH edge states depending on the specific boundary orientation.

cond-mat.mes-hall↗
arXiv2018

Testing Topological Protection of Edge States in Hexagonal Quantum Spin Hall Candidate Materials

We analyze the detailed structure of topological edge mode protection occuring in hexagonal quantum spin Hall (QSH) materials. We focus on bismuthene, antimonene, and arsenene on a SiC substrate, which, due to their large bulk gap, may offer new opportunities for room-temperature QSH applications. While time reversal symmetry is responsible for the principal symmetry protected character of QSH states, the hexagonal edge terminations yield further aspects of crystal symmetry which affect the topological protection. We show that armchair QSH edge states remain gapless under an in-plane magnetic field in the direction along the edge, a hallmark of their topological crystalline protection. In contrast, an out-of-plane magnetic field opens a gap of the order of a few meV within realistic ranges of parameters. We use these intriguing signatures of armchair QSH edge states to predict experimentally testable fingerprints of their additional topological crystalline character and their helicity emerging in tunneling spectroscopy and ballistic magnetotransport.

cond-mat.mes-hall↗
arXiv2018

Chiral voltage propagation in a self-calibrated topolectrical Chern circuit

We propose an electric circuit array with topologically protected uni-directional voltage modes at its boundary. Instead of external bias fields or floquet engineering, we employ negative impedance converters with current inversion (INICs) to accomplish a non-reciprocal, time-reversal symmetry broken electronic network we call topolectrical Chern circuit (TCC). The TCC features an admittance bulk gap fully tunable via the resistors used in the INICs, along with a chiral voltage boundary mode reminiscent of the Berry flux monopole present in the admittance band structure. The active circuit elements in the TCC can be calibrated to compensate for dissipative loss.

cond-mat.mes-hall↗
arXiv2018

Multiple topological states in iron-based superconductors

Topological insulators and semimetals as well as unconventional iron-based superconductors have attracted major recent attention in condensed matter physics. Previously, however, little overlap has been identified between these two vibrant fields, even though the principal combination of topological bands and superconductivity promises exotic unprecedented avenues of superconducting states and Majorana bound states (MBSs), the central building block for topological quantum computation. Along with progressing laser-based spin-resolved and angle-resolved photoemission spectroscopy (ARPES) towards high energy and momentum resolution, we have resolved topological insulator (TI) and topological Dirac semimetal (TDS) bands near the Fermi level ($E_{\text{F}}$) in the iron-based superconductors Li(Fe,Co)As and Fe(Te,Se), respectively. The TI and TDS bands can be individually tuned to locate close to $E_{\text{F}}$ by carrier doping, allowing to potentially access a plethora of different superconducting topological states in the same material. Our results reveal the generic coexistence of superconductivity and multiple topological states in iron-based superconductors, rendering these materials a promising platform for high-$T_{\text{c}}$ topological superconductivity.

cond-mat.supr-con↗
arXiv2018

Substrate-supported triplet superconductivity in Dirac semimetals

Stimulated by the success of graphene and its emerging Dirac physics, the quest for versatile and tunable electronic properties in atomically thin systems has led to the discovery of various chemical classes of 2D compounds. In particular, honeycomb lattices of group-IV elements, such as silicene and germanene, have been found experimentally. Whether it is a necessity of synthesis or a desired feature for application purposes, most 2D materials demand a supporting substrate. In this work, we highlight the constructive impact of substrates to enable the realization of exotic electronic quantum states of matter, where the buckling emerges as the decisive material parameter adjustable by the substrate. At the example of germanene deposited on MoS$_2$, we find that the coupling between the monolayer and the substrate, together with the buckled hexagonal geometry, conspire to provide a highly suited scenario for unconventional triplet superconductivity upon adatom-assisted doping.

cond-mat.supr-con↗
arXiv2018

Stability of the spiral spin liquid in MnSc$_2$S$_4$

We investigate the stability of the spiral spin liquid phase in MnSc$_2$S$_4$ against thermal and quantum fluctuations as well as against perturbing effects of longer-range interactions. Employing $ab~initio$ density functional theory (DFT) calculations we propose a realistic Hamiltonian for MnSc$_2$S$_4$, featuring second ($J_2$) and third $(J_3)$ neighbor Heisenberg interactions on the diamond lattice that are considerably larger than previously assumed. We argue that the combination of strong $J_2$ and $J_3$ couplings reproduces the correct magnetic Bragg peak position measured experimentally. Calculating the spin-structure factor within the pseudofermion functional-renormalization group technique we find that close to the magnetic phase transition the sizable $J_3$ couplings induce a strong spiral selection effect, in agreement with experiments. With increasing temperature the spiral selection becomes weaker such that in a window around three to five times the ordering temperature an approximate spiral spin liquid is realized in MnSc$_2$S$_4$.

cond-mat.str-el↗
arXiv2018

Demonstration of a two-dimensional PT-symmetric crystal: Bulk dynamics, topology, and edge states

In 1998, Carl Bender challenged the perceived wisdom of quantum mechanics that the Hamiltonian operator describing any quantum mechanical system has to be Hermitian. He showed that Hamiltonians that are invariant under combined parity-time (PT) symmetry transformations likewise can exhibit real eigenvalue spectra. These findings had a particularly profound impact in the field of photonics, where PT-symmetric potential landscapes can be implemented by appropriately distributing gain and loss. Following this approach, several hallmark features of PT symmetry were shown, such as the existence of non-orthogonal eigenmodes, non-reciprocal light evolution, diffusive coherent transport, and to study their implications in settings including PT-symmetric lasers and topological phase transitions. Similarly, PT-symmetry has enriched other research fields ranging from PT-symmetric atomic diffusion, superconducting wires, and PT-symmetric electronic circuits. Nevertheless, to this date, all experimental implementations of PT-symmetric systems have been restricted to one dimension, which is mostly due to limitations in the technologies at hand for realizing appropriate non-Hermitian potential landscapes. In this work, we report on the experimental realization and characterization of a two-dimensional PT-symmetric system by means of photonic waveguide lattices with judiciously designed refractive index landscape with alternating loss. A key result of our work is the demonstration of a non-Hermitian two-dimensional topological phase transition that coincides with the emergence of mid-gap edge states. Our findings pave the grounds for future investigations exploring the full potential of PT-symmetric photonics in higher dimensions. Moreover, our approach may even hold the key for realizing two-dimensional PT-symmetry also in other systems beyond photonics, such as matter waves and electronics.

physics.optics↗
arXiv2018

A new paradigm for the quantum spin Hall effect at high temperatures

The quantum spin Hall effect (QSHE) has formed the seed for contemporary research on topological quantum states of matter. Since its discovery in HgTe/CdTe quantum wells and AlGaAs/GaAs heterostructures, all such systems have so far been suffering from extremely low operating temperatures, rendering any technological application out of reach. We formulate a theoretical paradigm to accomplish the high temperature QSHE in monolayer-substrate heterostructures. Specifically, we explicate our proposal for hexagonal compounds formed by monolayers of heavy group-V elements (As, Sb, Bi) on a SiC substrate. We show how orbital filtering due to substrate hybridization, a tailored multi-orbital density of states at low energies, and large spin-orbit coupling can conspire to yield QSH states with bulk gaps of several hundreds of meV. Combined with the successful realization of Bi/SiC (0001), with a measured bulk gap of 800 meV reported previously [Reis et al., 10.1126/science.aai8142 (2017)], our paradigm elevates the QSHE from an intricate quantum phenomenon at low temperatures to a scalable effect amenable to device design and engineering.

cond-mat.str-el↗
arXiv2018

Band structure engineering and reconstruction in electric circuit networks

We develop an approach to design, engineer, and measure band structures in a synthetic crystal composed of electric circuit elements. Starting from the nodal analysis of a circuit lattice in terms of currents and voltages, our Laplacian formalism for synthetic matter allows us to investigate arbitrary tight-binding models in terms of wave number resolved Laplacian eigenmodes, yielding an admittance band structure of the circuit. For illustration, we model and measure a honeycomb circuit featuring a Dirac cone admittance bulk dispersion as well as flat band admittance edge modes at its bearded and zigzag terminations. We further employ our circuit band analysis to measure a topological phase transition in the topolectrical Su-Schrieffer-Heeger circuit.

cond-mat.mes-hall↗
arXiv2018

Landau level quantization of Dirac electrons on the sphere

Interactions in Landau levels can stabilize new phases of matter, such as fractionally quantized Hall states. Numerical studies of these systems mostly require compact manifolds like the sphere or a torus. For massive dispersions, a formalism for the lowest Landau level on the sphere was introduced by Haldane [F.D.M. Haldane, PRL 51, 605 (1983)]. Graphene and surfaces of 3D topological insulators, however, display massless (Dirac) dispersions, and hence require a different description. We generalize a formalism previously developed for Dirac electrons on the sphere in zero field to include the effect of an external, uniform magnetic field.

cond-mat.str-el↗
arXiv2018

Persistence of the gapless spin liquid in the breathing kagome Heisenberg antiferromagnet

The nature of the ground state of the spin $S=1/2$ Heisenberg antiferromagnet on the kagome lattice with breathing anisotropy (i.e., with different superexchange couplings $J_{\vartriangle}$ and $J_{\triangledown}$ within elementary up- and down-pointing triangles) is investigated within the framework of Gutzwiller projected fermionic wave functions and Monte Carlo methods. We analyze the stability of the U(1) Dirac spin liquid with respect to the presence of fermionic pairing that leads to a gapped $\mathbb{Z}_{2}$ spin liquid. For several values of the ratio $J_{\triangledown}/J_{\vartriangle}$, the size scaling of the energy gain due to the pairing fields and the variational parameters are reported. Our results show that the energy gain of the gapped spin liquid with respect to the gapless state either vanishes for large enough system size or scales to zero in the thermodynamic limit. Similarly, the optimized pairing amplitudes (responsible for opening the spin gap) are shown to vanish in the thermodynamic limit. Our outcome is corroborated by the application of one and two Lanczos steps to the gapless and gapped wave functions, for which no energy gain of the gapped state is detected when improving the quality of the variational states. Finally, we discuss the competition with the "simplex" $\mathbb{Z}_{2}$ resonating-valence-bond spin liquid, valence-bond crystal, and nematic states in the strongly anisotropic regime, i.e., $J_{\triangledown} \ll J_{\vartriangle}$.

cond-mat.str-el↗
arXiv2018

Topological Dirac semimetal phase in the iron-based superconductor Fe(Te,Se)

Topological Dirac semimetals (TDSs) exhibit bulk Dirac cones protected by time reversal and crystal symmetry, as well as surface states originating from non-trivial topology. While there is a manifold possible onset of superconducting order in such systems, few observations of intrinsic superconductivity have so far been reported for TDSs. We observe evidence for a TDS phase in FeTe$_{1-x}$Se$_x$ ($x$ = 0.45), one of the high transition temperature ($T_c$) iron-based superconductors. In angle-resolved photoelectron spectroscopy (ARPES) and transport experiments, we find spin-polarized states overlapping with the bulk states on the (001) surface, and linear magnetoresistance (MR) starting from 6 T. Combined, this strongly suggests the existence of a TDS phase, which is confirmed by theoretical calculations. In total, the topological electronic states in Fe(Te,Se) provide a promising high $T_c$ platform to realize multiple topological superconducting phases.

cond-mat.supr-con↗
arXiv2018

Direct observation of multiple topological phases in the iron-based superconductor Li(Fe,Co)As

Topological insulators/semimetals and unconventional iron-based superconductors have attracted major attentions in condensed matter physics in the past 10 years. However, there is little overlap between these two fields, although the combination of topological states and superconducting states will produce more exotic topologically superconducting states and Majorana bound states (MBS), a promising candidate for realizing topological quantum computations. With the progress in laser-based spin-resolved and angle-resolved photoemission spectroscopy (ARPES) with very high energy- and momentum-resolution, we directly resolved the topological insulator (TI) phase and topological Dirac semimetal (TDS) phase near Fermi level ($E_F$) in the iron-based superconductor Li(Fe,Co)As. The TI and TDS phases can be separately tuned to $E_F$ by Co doping, allowing a detailed study of different superconducting topological states in the same material. Together with the topological states in Fe(Te,Se), our study shows the ubiquitous coexistence of superconductivity and multiple topological phases in iron-based superconductors, and opens a new age for the study of high-Tc iron-based superconductors and topological superconductivity.

cond-mat.supr-con↗