arXiv subjects

S. Hartmann

Publications and source records attributed to S. Hartmann.

17 recordsLinked to original sources

arXiv2022

Sessile drop evaporation in a gap -- crossover between diffusion-limited and phase transition-limited regime

We consider the time evolution of a sessile drop of volatile partially wetting liquid on a rigid solid substrate. Thereby, the drop evaporates under strong confinement, namely, it sits on one of the two parallel plates that form a narrow gap. First, we develop an efficient mesoscopic thin-film description in gradient dynamics form. It couples the diffusive dynamics of the vertically averaged vapour density in the narrow gap to an evolution equation for the profile of the volatile drop. The underlying free energy functional incorporates wetting, interface and bulk energies of the liquid and gas entropy. The model allows us to investigate the transition between diffusion-limited and phase transition-limited evaporation for shallow droplets. Its gradient dynamics character also allows for a full-curvature formulation. Second, we compare results obtained with the mesoscopic model to corresponding direct numerical simulations solving the Stokes equation for the drop coupled to the diffusion equation for the vapour as well as to selected experiments. In passing, we discuss the influence of contact line pinning.

physics.flu-dyn↗

arXiv2022

Combined experimental and theoretical study of hydrostatic (He-gas) pressure effects in $\alpha$-RuCl$_3$

We report a detailed experimental and theoretical study on the effect of hydrostatic pressure on the structural and magnetic aspects of the layered honeycomb antiferromagent $\alpha$-RuCl$_{3}$. Magnetic susceptibility measurements performed under almost ideal hydrostatic-pressure conditions yield that the phase transition to zigzag-type antiferromagnetic order at $T_N$ = 7.3 K can be rapidly suppressed to about 6.1 K. A further suppression with increasing pressure is impeded due to the occurrence of a pressure-induced structural transition at $p \geq$ 104 MPa, accompanied by a strong dimerization of Ru-Ru bonds, which gives rise to a collapse of the magnetic susceptibility. Whereas the dimerization transition is strongly first order, as reflected by large discontinuous changes in $\chi$ and pronounced hysteresis effects, the magnetic transition under varying pressure and magnetic field also reveals indications for a weakly first-order transition. We assign this observation to a strong magnetoelastic coupling in this system. Measurements of $\chi$ under varying pressure in the paramagnetic regime ($T > T_N$) and before dimerization ($p <$ 100 MPa) reveal a considerable increase of $\chi$ with pressure. These experimental observations are consistent with the results of ab-initio Density Functional Theory (DFT) calculations on the pressure-dependent structure and the corresponding pressure-dependent magnetic model. Comparative susceptibility measurements on a second crystal showing two consecutive magnetic transitions instead of one, indicating the influence of stacking faults. Using different temperature-pressure protocols the effect of these stacking faults can be temporarily overcome, transforming the magnetic state from a multiple-$T_N$ into a single-$T_N$ state.

cond-mat.str-el↗

arXiv2017

Kondo-like phonon scattering in thermoelectric clathrates

Crystalline solids are generally known as excellent heat conductors, amorphous materials or glasses as thermal insulators. It has thus come as a surprise that certain crystal structures defy this paradigm. A prominent example are type-I clathrates and other materials with guest-host structures. They sustain low-energy Einstein-like modes in their phonon spectra, but are also prone to various types of disorder and phonon-electron scattering and thus the mechanism responsible for their ultralow thermal conductivities has remained elusive. While recent ab initio lattice dynamics simulations show that the Einstein-like modes enhance phonon-phonon Umklapp scattering, they reproduce experimental data only at low temperatures. Here we show that a new effect, an "all phononic Kondo effect", can resolve this discrepancy. This is evidenced by our thermodynamic and transport measurements on various clathrate single crystal series and their comparison with ab initio simulations. Our new understanding devises design strategies to further suppress the thermal conductivity of clathrates and other related materials classes, with relevance for the field of thermoelectric waste heat recovery but also more generally for phononic applications. More fundamentally, it may trigger theoretical work on strong correlation effects in phonon systems.

cond-mat.str-el↗

arXiv2017

Evolution of the Kondo lattice and non-Fermi liquid excitations in a heavy-fermion metal

Strong electron correlations can give rise to extraordinary properties of metals with renormalized quasiparticles which are at the basis of Landau's Fermi liquid theory. Near a quantum critical point, these quasiparticles can be destroyed and non-Fermi liquid behavior ensues. YbRh$_2$Si$_2$ is a prototypical correlated metal as it exhibits quasiparticles formation, formation of Kondo lattice coherence and quasiparticle destruction at a field-induced quantum critical point. Here we show how, upon lowering the temperature, the Kondo lattice coherence develops and finally gives way to non-Fermi liquid electronic excitations. By measuring the single-particle excitations through scanning tunneling spectroscopy down to 0.3 K, we find the Kondo lattice peak emerging below the Kondo temperature $T_{\rm K} \sim$ 25 K, yet this peak displays a non-trivial temperature dependence with a strong increase around 3.3 K. At the lowest temperature and as a function of an external magnetic field, the width of this peak is minimized in the quantum critical regime. Our results provide a striking demonstration of the non-Fermi liquid electronic excitations in quantum critical metals, thereby elucidating the strange-metal phenomena that have been ubiquitously observed in strongly correlated electron materials.

cond-mat.str-el↗

arXiv2017

Nanomechanics of CNTs for Sensor Application

A nanoscopic simulation for an acceleration sensor is aimed based on the piezoresistive effect of carbon nanotubes (CNTs). Therefore, a compact model is built from density functional theory (DFT), compared with results of molecular dynamics (MD) that describes the mechanics of carbon nanotubes in a parameterized way. The results for the interesting kind of CNTs [(6,3) and (7,4)] within the two approaches agree in a satisfying way, when DFT-calculations are performed with atomic configurations obtained by MD geometry optimization. Geometry optimization yields the Poisson ratio for CNTs. Thus, values from MD and DFT are compared. The simulation finally aims the modeling of the conductive behavior of CNTs when strain is applied, but this needs further verification. Here, we present the prediction of the tight binding model for suitable CNTs.

cond-mat.mes-hall↗

arXiv2016

The gaseous debris disk of the white dwarf SDSS J1228+1040. HST/COS search for far-ultraviolet signatures

Gaseous and dust debris disks around white dwarfs (WDs) are formed from tidally disrupted planetary bodies. This offers an opportunity to determine the composition of exoplanetary material by measuring element abundances in the accreting WD's atmosphere. A more direct way to do this is through spectral analysis of the disks themselves. Currently, the number of chemical elements detected through disk emission-lines is smaller than that of species detected through lines in the WD atmospheres. We assess the far-ultraviolet (FUV) spectrum of one well-studied object (SDSS J122859.93+104032.9) to search for disk signatures at wavelengths <1050 angstrom, where the broad absorption lines of the Lyman series effectively block the WD photospheric flux. We performed FUV observations (950-1240 angstrom) with the Hubble Space Telescope/Cosmic Origins Spectrograph and used archival optical spectra. We compared them with non-local thermodynamic equilibrium model spectra. In addition, we investigate the Ca II infrared triplet (IRT) line profiles to constrain disk geometry and composition. No disk emission-lines were detected in the FUV spectrum, indicating that the disk effective temperature is about 5000K. The long-time variability of the Ca II IRT was reproduced with a precessing disk model of bulk Earth-like composition, having a surface mass density of 0.3g/cm2 and an extension from 55 to 90 WD radii. The disk has a spiral shape that precesses with a period of approximately 37 years, confirming previous results.

astro-ph.SR↗

arXiv2014

Tailored quantum statistics from broadband states of light

We analyze the statistics of photons originating from amplified spontaneous emission generated by a quantum dot superluminescent diode. Experimentally detectable emission properties are taken into account by parametrizing the corresponding quantum state as a multi-mode phase-randomized Gaussian density operator. The validity of this model is proven in two subsequent experiments using fast two-photon-absorption detection observing second order equal-time- as well as second order fully time-resolved intensity correlations on femtosecond timescales. In the first experiment, we study the photon statistics when the number of contributing longitudinal modes is systematically reduced by applying well-controlled optical feedback. In a second experiment, we add coherent light from a single-mode laserdiode to quantum dot superluminescent diode broadband radiation. Tuning the power ratio, we realize tailored second order correlations ranging from Gaussian to Poissonian statistics. Both experiments are very well matched by theory, thus giving first insights into quantum properties of radiation from quantum dot superluminescent diodes.

quant-ph↗

arXiv2014

Non-LTE spectral models for the gaseous debris-disk component of Ton 345

For a fraction of single white dwarfs with debris disks, an additional gaseous disk was discovered. Both dust and gas are thought to be created by the disruption of planetary bodies. The composition of the extrasolar planetary material can directly be analyzed in the gaseous disk component, and the disk dynamics might be accessible by investigating the temporal behavior of the Ca II infrared emission triplet, hallmark of the gas disk. We obtained new optical spectra for the first helium-dominated white dwarf for which a gas disk was discovered (Ton 345) and modeled the non-LTE spectra of viscous gas disks composed of carbon, oxygen, magnesium, silicon, sulfur, and calcium with chemical abundances typical for solar system asteroids. Iron and its possible line-blanketing effects on the model structure and spectral energy distribution was still neglected. A set of models with different radii, effective temperatures, and surface densities as well as chondritic and bulk-Earth abundances was computed and compared with the observed line profiles of the Ca II infrared triplet. Our models suggest that the Ca II emission stems from a rather narrow gas ring with a radial extent of R=0.44-0.94 Rsol, a uniform surface density Sigma=0.3 g/cm2, and an effective temperature of Teff=6000 K. The often assumed chemical mixtures derived from photospheric abundances in polluted white dwarfs - similar to a chondritic or bulk-Earth composition - produce unobserved emission lines in the model and therefore have to be altered. We do not detect any line-profile variability on timescales of hours, but we confirm the long-term trend over the past decade for the red-blue asymmetry of the double-peaked lines.

astro-ph.SR↗

arXiv2013

Thermal and Electrical Transport across a Magnetic Quantum Critical Point

A quantum critical point (QCP) arises at a continuous transition between competing phases at zero temperature. Collective excitations at magnetic QCPs give rise to metallic properties that strongly deviate from the expectations of Landau's Fermi liquid description, the standard theory of electron correlations in metals. Central to this theory is the notion of quasiparticles, electronic excitations which possess the quantum numbers of the bare electrons. Here we report measurements of thermal and electrical transport across the field-induced magnetic QCP in the heavy-fermion compound YbRh$_2$Si$_2$. We show that the ratio of the thermal to electrical conductivities at the zero-temperature limit obeys the Wiedemann-Franz (WF) law above the critical field, $B_c$. This is also expected at $B < B_c$, where weak antiferromagnetic order and a Fermi liquid phase form below 0.07 K ($B = 0$). However, at the critical field the low-temperature electrical conductivity suggests a non-Fermi-liquid ground state and exceeds the thermal conductivity by about 10%. This apparent violation of the WF law provides evidence for an unconventional type of QCP at which the fundamental concept of Landau quasiparticles breaks down. These results imply that Landau quasiparticles break up, and that the origin of this disintegration is inelastic scattering associated with electronic quantum critical fluctuations. Our finding brings new insights into understanding deviations from Fermi-liquid behaviour frequently observed in various classes of correlated materials.

cond-mat.str-el↗

arXiv2012

Observations and NLTE Modeling of the Gaseous Planetary Debris Disk around Ton 345

Debris disks around single white dwarfs are thought to be the remains of planetary bodies disrupted by tidal forces. Ongoing accretion of the hereby produced dust allows to detect the planetary material in the white dwarf photosphere and to conclude on its chemical composition. As an alternative, the composition can in principle be determined directly from the emission lines of the sometimes additionally observed gaseous component of the disks. To this aim, we perform spectral modeling with our non-LTE code for accretion disks. We have obtained new observations of Ton 345 in order to look for long- and short-term variations in the disk line-profiles. We find that the prominent red-violet asymmetry of the Ca II infrared triplet almost disappeared. Line-profile variations during one night are not seen without doubt.

astro-ph.SR↗

arXiv2011

Non-LTE models for the gaseous metal component of circumstellar discs around white dwarfs

Gaseous metal discs around single white dwarfs have been discovered recently. They are thought to develop from disrupted planetary bodies. Spectroscopic analyses will allow us to study the composition of extrasolar planetary material. We investigate in detail the first object for which a gas disc was discovered (SDSS J122859.93+104032.9). Therefor we perform non-LTE modelling of viscous gas discs by computing the detailed vertical structure and line spectra. The models are composed of carbon, oxygen, magnesium, silicon, calcium, and hydrogen with chemical abundances typical for Solar System asteroids. Line asymmetries are modelled by assuming spiral-arm and eccentric disc structures as suggested by hydrodynamical simulations. The observed infrared Ca II emission triplet can be modelled with a hydrogen-deficient metal gas disc located inside of the tidal disruption radius, with an effective temperature of about 6000 K and a surface mass density of 0.3 g/cm^2. The inner radius is well constrained at about 0.64 Solar radii. The line profile asymmetry can be reproduced by either a spiral-arm structure or an eccentric disc, the latter being favoured by its time variability behaviour. Such structures, reaching from 0.64 to 1.5 Solar radii, contain a mass of about 3 to 6*10^21 g, the latter equivalent to the mass of a 135-km diameter Solar System asteroid.

astro-ph.SR↗

arXiv2011

Asymmetric Line Profiles in Spectra of Gaseous Metal Disks Around Single White Dwarfs

Metal-rich debris disks were discovered around several single DAZ and DBZ white dwarfs, which may stem from disruption of smaller rocky planetesimals. In some cases, the material in addition forms a gaseous disk. For SDSS J122859.93+104032.9, the double peaked infrared Ca II triplet at about 8500 angstrom exhibits a strong red/violet asymmetry. With the Tuebingen non-LTE Accretion Disk code AcDc we calculated the spectrum and vertical structure of the disk, assuming the chemical mixture of the disk's material being similar to a chondrite-like asteroid, the most prominent type in our own solar system. By modifying the code to simulate different non axis-symmetrical disk geometries, the first preliminary results are in good agreement with the observed asymmetric line profile.

astro-ph.EP↗

arXiv2010

Asymmetric Line Profiles in Spectra of Gaseous Metal Disks Around Single White Dwarfs

Around several single DAZ and DBZ white dwarfs metal-rich disks have been observed, which are mostly believed to originate from disruption of smaller rocky planetesimals. In some cases the material does not (only) form a dusty but gaseous disk. In the case of SDSS J122859.93+104032.9 the double peaked infrared Ca II triplet at about 8500 angstrom, one of only two emission features of the spectra, exhibits a strong red/violet asymmetry. Assuming a composition similar to a chondrite-like asteroid, being the most prominent type in our own solar system, we calculated the spectrum and vertical structure of the disk using the Tuebingen NLTE accretion disk code "AcDc". Modified to simulate different non axis-symmetrical disk geometries, the first preliminary results are in good agreement with the observed asymmetric line profile.

astro-ph.SR↗

arXiv2010

Break up of heavy fermions at an antiferromagnetic instability

We present results of high-resolution, low-temperature measurements of the Hall coefficient, thermopower, and specific heat on stoichiometric YbRh2Si2. They support earlier conclusions of an electronic (Kondo-breakdown) quantum critical point concurring with a field induced antiferromagnetic one. We also discuss the detachment of the two instabilities under chemical pressure. Volume compression/expansion (via substituting Rh by Co/Ir) results in a stabilization/weakening of magnetic order. Moderate Ir substitution leads to a non-Fermi-liquid phase, in which the magnetic moments are neither ordered nor screened by the Kondo effect. The so-derived zero-temperature global phase diagram promises future studies to explore the nature of the Kondo breakdown quantum critical point without any interfering magnetism.

cond-mat.str-el↗

arXiv2009

Violation of critical universality at the antiferromagnetic phase transition of YbRh2Si2

We report on precise low-temperature specific-heat measurements, C(T), of YbRh2Si2 in the vicinity of the antiferromagnetic phase transition on a single crystal of superior quality (RRR 150). We observe a very sharp peak at T_N=72mK with absolute values as high as C/T=8J/molK^2. A detailed analysis of the critical exponent αaround T_N reveals α=0.38 which differs significantly from those of the conventional universality classes in the Ginzburg-Landau theory, where α<0.11. Thermal-expansion measurements corroborate this large positive critical exponent. These results provide insight into the nature of the critical magnetic fluctuations at a temperature-driven phase transition close to a quantum critical point.

cond-mat.str-el↗

arXiv2008

Low-temperature thermopower study of YbRh2Si2

The heavy-fermion compound YbRh2Si2 exhibits an antiferromagnetic (AFM) phase transition at an extremely low temperature of TN = 70 mK. Upon applying a tiny magnetic field of Bc = 60 mT the AFM ordering is suppressed and the system is driven toward a field-induced quantum critical point (QCP). Here, we present low-temperature thermopower S(T) measurements of high-quality YbRh2Si2 single crystals down to 30 mK. S(T) is found negative with comparably large values in the paramagnetic state. In zero field no Landau-Fermi-liquid (LFL) like behavior is observed within the magnetically ordered phase. However, a sign change from negative to positive appears at lowest temperatures on the magnetic side of the QCP. For higher fields B > Bc a linear extrapolation of S to zero clearly evidences the recovery of LFL regime. The crossover temperature is sharply determined and coincides perfectly with the one derived from resistivity and specific heat investigations.

cond-mat.str-el↗

arXiv1996

The Chromo-Dielectric Soliton Model: Quark Self Energy and Hadron Bags

The chromo-dielectric soliton model (CDM) is Lorentz- and chirally-invariant. It has been demonstrated to exhibit dynamical chiral symmetry breaking and spatial confinement in the locally uniform approximation. We here study the full nonlocal quark self energy in a color-dielectric medium modeled by a two parameter Fermi function. Here color confinement is manifest. The self energy thus obtained is used to calculate quark wave functions in the medium which, in turn, are used to calculate the nucleon and pion masses in the one gluon exchange approximation. The nucleon mass is fixed to its empirical value using scaling arguments; the pion mass (for massless current quarks) turns out to be small but non-zero, depending on the model parameters.

nucl-th↗