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Teng Wu

Publications and source records attributed to Teng Wu.

29 records · Page 2Linked to original sources

Search for axion-like dark matter using solid-state nuclear magnetic resonance

We report the results of an experimental search for ultralight axion-like dark matter in the mass range 162 neV to 166 neV. The detection scheme of our Cosmic Axion Spin Precession Experiment (CASPEr) is based on a precision measurement of $^{207}$Pb solid-state nuclear magnetic resonance in a polarized ferroelectric crystal. Axion-like dark matter can exert an oscillating torque on $^{207}$Pb nuclear spins via the electric-dipole moment coupling $g_d$, or via the gradient coupling $g_{\text{aNN}}$. We calibrated the detector and characterized the excitation spectrum and relaxation parameters of the nuclear spin ensemble with pulsed magnetic resonance measurements in a 4.4 T magnetic field. We swept the magnetic field near this value and searched for axion-like dark matter with Compton frequency within a 1 MHz band centered at 39.65 MHz. Our measurements place the upper bounds $|g_d|<9.5\times10^{-4}\,\text{GeV}^{-2}$ and $|g_{\text{aNN}}|<2.8\times10^{-1}\,\text{GeV}^{-1}$ (95% confidence level) in this frequency range. The constraint on $g_d$ corresponds to an upper bound of $1.0\times 10^{-21}\,\text{e}\cdot\text{cm}$ on the amplitude of oscillations of the neutron electric dipole moment, and $4.3\times 10^{-6}$ on the amplitude of oscillations of CP-violating $θ$ parameter of quantum chromodynamics. Our results demonstrate the feasibility of using solid-state nuclear magnetic resonance to search for axion-like dark matter in the nano-electronvolt mass range.

hep-ex↗

Adaptive Change Point Monitoring for High-Dimensional Data

In this paper, we propose a class of monitoring statistics for a mean shift in a sequence of high-dimensional observations. Inspired by the recent U-statistic based retrospective tests developed by Wang et al.(2019) and Zhang et al.(2020), we advance the U-statistic based approach to the sequential monitoring problem by developing a new adaptive monitoring procedure that can detect both dense and sparse changes in real-time. Unlike Wang et al.(2019) and Zhang et al.(2020), where self-normalization was used in their tests, we instead introduce a class of estimators for $q$-norm of the covariance matrix and prove their ratio consistency. To facilitate fast computation, we further develop recursive algorithms to improve the computational efficiency of the monitoring procedure. The advantage of the proposed methodology is demonstrated via simulation studies and real data illustrations.

stat.ME↗

All-Optical Single-Species Cesium Atomic Comagnetometer with Optical Free Induction Decay Detection

Atomic comagnetometers, which measure the spin precession frequencies of overlapped species simultaneously, are widely applied to search for exotic spin-dependent interactions. Here we propose and implement an all-optical single-species Cs atomic comagnetometer based on the optical free induction decay (FID) signal of Cs atoms in hyperfine levels $F_g=3~\&~4$ within the same atomic ensemble. We experimentally show that systematic errors induced by magnetic field gradients and laser fields are highly suppressed in the comagnetometer, but those induced by asynchronous optical pumping and drift of residual magnetic field in the shield dominate the uncertainty of the comagnetometer. With this comagnetometer system, we set the constraint on the strength of spin-gravity coupling of the proton at a level of $10^{-18}$ eV, comparable to the most stringent one. With further optimization in magnetic field stabilization and spin polarization, the systematic errors can be effectively suppressed, and signal-to-noise ratio (SNR) can be improved, promising to set more stringent constraints on spin-gravity interactions.

physics.atom-ph↗

Zero- to Ultralow-Field Nuclear Magnetic Resonance $J$-Spectroscopy with Commercial Atomic Magnetometers

Zero- to ultralow-field nuclear magnetic resonance (ZULF NMR) is an alternative spectroscopic method to high-field NMR, in which samples are studied in the absence of a large magnetic field. Unfortunately, there is a large barrier to entry for many groups, because operating the optical magnetometers needed for signal detection requires some expertise in atomic physics and optics. Commercially available magnetometers offer a solution to this problem. Here we describe a simple ZULF NMR configuration employing commercial magnetometers, and demonstrate sufficient functionality to measure samples with nuclear spins prepolarized in a permanent magnet or initialized using parahydrogen. This opens the possibility for other groups to use ZULF NMR, which provides a means to study complex materials without magnetic susceptibility-induced line broadening, and to observe samples through conductive materials.

physics.chem-ph↗

Constraints on bosonic dark matter from ultralow-field nuclear magnetic resonance

The nature of dark matter, the invisible substance making up over $80\%$ of the matter in the Universe, is one of the most fundamental mysteries of modern physics. Ultralight bosons such as axions, axion-like particles or dark photons could make up most of the dark matter. Couplings between such bosons and nuclear spins may enable their direct detection via nuclear magnetic resonance (NMR) spectroscopy: as nuclear spins move through the galactic dark-matter halo, they couple to dark-matter and behave as if they were in an oscillating magnetic field, generating a dark-matter-driven NMR signal. As part of the Cosmic Axion Spin Precession Experiment (CASPEr), an NMR-based dark-matter search, we use ultralow-field NMR to probe the axion-fermion "wind" coupling and dark-photon couplings to nuclear spins. No dark matter signal was detected above background, establishing new experimental bounds for dark-matter bosons with masses ranging from $1.8\times 10^{-16}$ to $7.8\times 10^{-14}$ eV.

hep-ex↗

Search for axionlike dark matter with a liquid-state nuclear spin comagnetometer

We report the results of a search for axionlike dark matter using nuclear magnetic resonance (NMR) techniques. This search is part of the multi-faceted Cosmic Axion Spin Precession Experiment (CASPEr) program. In order to distinguish axionlike dark matter from magnetic fields, we employ a comagnetometry scheme measuring ultralow-field NMR signals involving two different nuclei ($^{13}$C and $^{1}$H) in a liquid-state sample of acetonitrile-2-$^{13}$C ($^{13}$CH$_{3}$CN). No axionlike dark matter signal was detected above background. This result constrains the parameter space describing the coupling of the gradient of the axionlike dark matter field to nucleons to be $g_{aNN}<6\times 10^{-5}$ GeV$^{-1}$ (95$\%$ confidence level) for particle masses ranging from $10^{-22}$ eV to $1.3\times10^{-17}$ eV, improving over previous laboratory limits for masses below $10^{-21}$ eV. The result also constrains the coupling of nuclear spins to the gradient of the square of the axionlike dark matter field, improving over astrophysical limits by orders of magnitude over the entire range of particle masses probed.

hep-ex↗

Magnetic Gradiometer for Detection of Zero- and Ultralow-Field Nuclear Magnetic Resonance

Magnetic sensors are important for detecting nuclear magnetization signals in nuclear magnetic resonance (NMR). As a complementary analysis tool to conventional high-field NMR, zero- and ultralow-field (ZULF) NMR detects nuclear magnetization signals in the sub-microtesla regime. Current ZULF NMR systems are always equipped with high-quality magnetic shieldings to ensure that ambient magnetic field noise does not dwarf the magnetization signal. An alternative approach is to separate the magnetization signal from the noise based on their differing spatial profiles, as can be achieved using a magnetic gradiometer. Here, we present a gradiometric ZULF NMR spectrometer with a magnetic gradient noise of 17 fT_{rms}{cm}^{-1}{Hz}^{-1/2} in the frequency range of 100-400 Hz, based on a single vapor cell (0.7x0.7x1.0{cm}^3). With applied white magnetic-field noise, we show that the gradiometric spectrometer achieves 13-fold enhancement in the signal-to-noise ratio (SNR) compared to the single-channel configuration. By reducing the influence of common-mode magnetic noise, this work enables the use of compact and low-cost magnetic shields. Gradiometric detection may also prove to be beneficial for eliminating systematic errors in ZULF-NMR experiments searching for exotic spin-dependent interactions and molecular parity violation.

physics.atom-ph↗

Nuclear-spin comagnetometer based on a liquid of identical molecules

Atomic comagnetometers are used in searches for anomalous spin-dependent interactions. Magnetic field gradients are one of the major sources of systematic errors in such experiments. Here we describe a comagnetometer based on the nuclear spins within an ensemble of identical molecules. The dependence of the measured spin-precession frequency ratio on the first-order magnetic field gradient is suppressed by over an order of magnitude compared to a comagnetometer based on overlapping ensembles of different molecules. Our single-species comagnetometer is shown to be capable of measuring the hypothetical spin-dependent gravitational energy of nuclei at the $10^{-17}$ eV level, comparable to the most stringent existing constraints. Combined with techniques for enhancing the signal such as parahydrogen-induced polarization, this method of comagnetometry offers the potential to improve constraints on spin-gravity coupling of nucleons by several orders of magnitude.

physics.atom-ph↗

The Cosmic Axion Spin Precession Experiment (CASPEr): a dark-matter search with nuclear magnetic resonance

The Cosmic Axion Spin Precession Experiment (CASPEr) is a nuclear magnetic resonance experiment (NMR) seeking to detect axion and axion-like particles which could make up the dark matter present in the universe. We review the predicted couplings of axions and axion-like particles with baryonic matter that enable their detection via NMR. We then describe two measurement schemes being implemented in CASPEr. The first method, presented in the original CASPEr proposal, consists of a resonant search via continuous-wave NMR spectroscopy. This method offers the highest sensitivity for frequencies ranging from a few Hz to hundreds of MHz, corresponding to masses $ m_{\rm a} \sim 10^{-14}$--$10^{-6}$ eV. Sub-Hz frequencies are typically difficult to probe with NMR due to the diminishing sensitivity of magnetometers in this region. To circumvent this limitation, we suggest new detection and data processing modalities. We describe a non-resonant frequency-modulation detection scheme, enabling searches from mHz to Hz frequencies ($m_{\rm a} \sim 10^{-17}$--$10^{-14} $ eV), extending the detection bandwidth by three decades.

physics.ins-det↗

Experimental Benchmarking of Quantum Control in Zero-Field Nuclear Magnetic Resonance

Zero-field nuclear magnetic resonance (NMR) provides complementary analysis modalities to those of high-field NMR and allows for ultra-high-resolution spectroscopy and measurement of untruncated spin-spin interactions. Unlike for the high-field case, however, universal quantum control -- the ability to perform arbitrary unitary operations -- has not been experimentally demonstrated in zero-field NMR. This is because the Larmor frequency for all spins is identically zero at zero field, making it challenging to individually address different spin species. We realize a composite-pulse technique for arbitrary independent rotations of $^1$H and $^{13}$C spins in a two-spin system. Quantum-information-inspired randomized benchmarking and state tomography are used to evaluate the quality of the control. We experimentally demonstrate single-spin control for $^{13}$C with an average gate fidelity of $0.9960(2)$ and two-spin control via a controlled-not (CNOT) gate with an estimated fidelity of $0.99$. The combination of arbitrary single-spin gates and a CNOT gate is sufficient for universal quantum control of the nuclear spin system. The realization of complete spin control in zero-field NMR is an essential step towards applications to quantum simulation, entangled-state-assisted quantum metrology, and zero-field NMR spectroscopy.

quant-ph↗

Miniature cavity-enhanced diamond magnetometer

We present a highly sensitive miniaturized cavity-enhanced room-temperature magnetic-field sensor based on nitrogen-vacancy (NV) centers in diamond. The magnetic resonance signal is detected by probing absorption on the 1042\,nm spin-singlet transition. To improve the absorptive signal the diamond is placed in an optical resonator. The device has a magnetic-field sensitivity of 28 pT/$\sqrt{\rm{Hz}}$, a projected photon shot-noise-limited sensitivity of 22 pT/$\sqrt{\rm{Hz}}$ and an estimated quantum projection-noise-limited sensitivity of 0.43 pT/$\sqrt{\rm{Hz}}$ with the sensing volume of $\sim$ 390 $μ$m $\times$ 4500 $μ$m$^{2}$. The presented miniaturized device is the basis for an endoscopic magnetic field sensor for biomedical applications.

quant-ph↗