arXiv subjects

Thomas Pohl

Publications and source records attributed to Thomas Pohl.

At least 19 recordsLinked to original sources

arXiv2026

Static-Field Shielding of Bosonic Molecules: Evaporation to Degeneracy and Self-Bound Droplets

The strong, tunable dipolar interactions of ultracold molecules make them a powerful platform for quantum many-body physics, but reaching degeneracy by evaporative cooling requires suppressing inelastic collisions. Microwave collisional shielding has enabled the preparation of degenerate Fermi gases and Bose-Einstein condensates of polar molecules, whereas static electric field shielding has been limited to fermionic species, which are less prone to inelastic loss. We demonstrate static-field F\"{o}rster shielding of bosonic $^{23}$Na$^{87}$Rb molecules, suppressing two-body loss by up to four orders of magnitude. Within a bound-state-free electric-field window, three-body loss is also strongly suppressed, enabling efficient evaporation. Evaporating with an efficiency of 2.09(9), we increase the phase-space density of the gas by two orders of magnitude, reaching degeneracy with 7200(1000) molecules. We observe self-bound droplets at the end of evaporation over a wide range of field strengths, emerging from either degenerate or non-degenerate parent gases. We perform Path Integral Monte Carlo simulations, which suggest that the observed droplets are filamentary in nature, and find good agreement with the experimentally observed droplet formation temperatures. Our results establish F\"{o}rster shielding as a single-field route to prepare degenerate gases and self-bound droplets of bosonic polar molecules.

cond-mat.quant-gas↗

arXiv2026

Fast Quantum Interconnects via Neutral Atom Ensembles

Distributing entanglement between distant qubits is a crucial element of scalable quantum computing. Here, we describe a scalable quantum interconnect that generates remote entanglement at rates approaching those compatible with two-qubit gates of current neutral-atom quantum processors. The proposed approach exploits the strong dipole-dipole interactions between atomic Rydberg states to generate entanglement between stationary qubits and propagating photons, without the need for an optical cavity. We provide a thorough description of the optimal conditions for the developed entanglement-generation protocol for realistic experimental parameters and demonstrate that entanglement-generation rates $\gtrsim 3\times 10^5$ s$^{-1}$ can be achieved using Rydberg states of ytterbium atoms. Given the inherent scalability and design flexibility of the proposed interconnect, our results suggest a promising approach towards distributed networks based on neutral-atom quantum architectures.

quant-ph↗

arXiv2026

Equilibrium and non-equilibrium phases of microwave-dressed polar molecules beyond rotational symmetries

Recent experiments on molecular droplets have opened a new frontier of self-organization in strongly dipolar quantum matter. Microwave-dressing of polar molecules permits to tune both the strength and the angular structure of long-range interactions, potentially promoting a rich spectrum of quantum phases, from superfluid droplets with varying geometry and insulating or supersolid droplet arrays to strongly correlated crystals of individual molecules. Using path-integral Monte Carlo simulations of large molecular ensembles, we demonstrate that experimentally observed droplet arrays emerge as a metastable non-equilibrium state from the quenching of a gas-droplet phase transition under entirely broken rotational symmetry of the microwave-induced interaction potential. We moreover find that a crystalline phase of molecules, predicted for antidipolar interactions, is absent under conditions of recent experiments. This is traced back to the lack of angular symmetry in currently employed microwave-dressing, which qualitatively reshapes the many-body energy landscape and cannot be captured by effective scalar interaction parameters. Our results provide the first direct comparison of ab initio simulations and experiments and establish interaction anisotropy as a key aspect of molecular quantum gases.

cond-mat.quant-gas↗

arXiv2026

Extensive mixed-state entanglement in kinetically constrained superradiance

Dicke superradiance by an ensemble of quantum emitters produces a collective burst of radiation, but no entanglement in the mixed state of the emitters. We show that adding a local kinetic constraint between the emitters generates extensive mixed-state entanglement, while otherwise preserving all key features of Dicke superradiance. Specifically, for any local Boolean constraint, we analytically derive a lower bound for the emission rate which implies a peak intensity $\propto N^2$ and a peak time $\propto (\log N)/N$ with number of spins $N$. This effect enables the superradiantly accelerated preparation of entangled dark states. Hereby, Hilbert-space fragmentation of the Dicke ladder leads to an exponentially branching decay tree that generates a hierarchy of dark states. Importantly, these disconnected manifolds include exponentially many long-range entangled singlet dark states. The explored kinetic constraints and superradiant dynamics can be realized in neutral-atom arrays coupled to an optical cavity, and we suggest a simple and accessible witness to detect the predicted mixed-state entanglement in such experiments. Moreover, we show that entanglement generation is robust against atomic decay and collective dephasing, and should be observable under recently reported experimental conditions. Our results, thereby, offer a general framework and experimentally viable approach for the dissipative engineering of entangled dark states enhanced by superradiance.

quant-ph↗

arXiv2026

Establishing the $^{40}$Ca$(p,p \alpha)$ reaction at 392 MeV under quasi-free scattering conditions

The $(p,p \alpha)$ reaction offers a direct means to probe preformed $\alpha$-cluster structures in nuclei under quasi-free scattering conditions. Previous studies around 100 MeV provided valuable insights into $\alpha$ clustering, but quantitative comparison with microscopic cluster wave functions remained limited due to strong distortion effects. At higher energies, the reaction mechanism becomes simpler and the distorted-wave impulse approximation (DWIA) provides a more reliable framework for quantitative analysis. In the present work, the $^{40}$Ca$(p,p\alpha)$ reaction was measured at an incident energy of 392 MeV using the high-resolution Grand Raiden and LAS spectrometers at RCNP. Despite the small cross section in this energy region, the achieved resolution allowed clear separation of the ground and excited states of the residual $^{36}$Ar nucleus, and corresponding momentum distributions were extracted. DWIA calculations using a Woods-Saxon $\alpha + ^{36}$Ar bound-state wave function yielded an experimental spectroscopic factor of $ S_{\mathrm{FAC}}^{\mathrm{WS}} = 0.51 \pm 0.05 $, consistent with the previous result at 101.5 MeV $(0.52 \pm 0.23 )$. This agreement demonstrates that the reaction mechanism is well described across a wide energy range. The present study establishes the feasibility of high-precision $(p,p\alpha)$ measurements at several hundred MeV and highlights their potential as a quantitative probe of $\alpha$ clustering in medium-mass nuclei, forming the basis for systematic studies in both stable and unstable systems.

nucl-ex↗

arXiv2025

Strongly dipolar molecular Bose-Einstein condensates: From few- to many-body physics

Recent advances in molecular cooling have enabled the realization of strongly dipolar Bose--Einstein condensates (BECs) of molecules, and BECs of many different molecular species may become experimentally accessible in the near future. Here, we explore the unique properties of such BECs and the new insights they may offer into dipolar quantum fluids and many-body physics. We explore which parameter regimes can realistically be achieved using currently available experimental techniques, discuss how to implement these techniques, and outline which molecular species are particularly well suited to explore exotic new states of matter. We further determine how state-of-the-art beyond mean-field theories, originally developed for weakly dipolar magnetic gases, can be pushed to their limits and beyond, and what other long-standing questions in the field of dipolar physics may realistically come within reach using molecular systems.

cond-mat.quant-gas↗

arXiv2025

Observation of non-Hermitian many-body phase transition in a Rydberg-atom array

Non-Hermitian quantum mechanics with parity-time (PT) symmetry offers a powerful framework for exploring the complex interplay of dissipation and coherent interactions in open quantum systems. While PT-symmetry breaking has been studied in various physical systems, its observation on a quantum many-body level remains elusive. Here, we experimentally realize a non-Hermitian XY model in a strongly-interacting Rydberg-atom array. By measuring the Loschmidt Echo of a fully polarized state, we observe distinct dynamical signatures of a PT-symmetry-breaking phase transition. Dipole interactions are found to play a crucial role, not only determining the transition point but also triggering a non-Hermitian many-body blockade effect that protects the Loschmidt Echo from decay with a non-monotonic dependence on the system size. Our results reveal intricate interaction-induced effects on PT-symmetry breaking and open the door for exploring non-Hermitian many-body dynamics beyond single-particle and mean-field paradigms.

quant-ph↗

arXiv2025

Phenomenological model of decaying Bose polarons

Cold atom experiments show that a mobile impurity particle immersed in a Bose-Einstein condensate forms a well-defined quasiparticle (Bose polaron) for weak to moderate impurity-boson interaction strengths, whereas a significant line broadening is consistently observed for strong interactions. Motivated by this, we introduce a phenomenological theory based on the assumption that the most relevant states are characterized by the impurity correlated with at most one boson, since they have the largest overlap with the uncorrelated states to which the most common experimental probes couple. These experimentally relevant states can however decay to lower energy states characterised by correlations involving multiple bosons, and we model this using a minimal variational wave function combined with a complex impurity-boson interaction strength. We first motivate this approach by comparing to a more elaborate theory that includes correlations with up to two bosons. Our phenomenological model is shown to recover the main results of two recent experiments probing both the spectral and the non-equilibrium properties of the Bose polaron. Our work offers an intuitive framework for analyzing experimental data and highlights the importance of understanding the complicated problem of the Bose polaron decay in a many-body setting.

cond-mat.quant-gas↗

arXiv2025

Self-bound monolayer crystals of ultracold polar molecules

We investigate the physics of ultracold dipolar molecules using path-integral quantum Monte Carlo simulations, and construct the complete phase diagram extending from weak to strong interactions and from small to mesoscopic particle numbers. Our calculations predict the formation of self-bound quantum droplets at interaction strengths lower than previously anticipated. For stronger interactions, the droplet continuously loses superfluidity as correlations develop, and is eventually found to undergo a transition to a crystalline monolayer that remains self-bound without external confinement. The spontaneous formation of such two-dimensional phases from a three-dimensional quantum gas is traced back to the peculiar anisotropic form of the dipole-dipole interaction generated by microwave-dressing of rotational molecular states. For sufficiently large particle numbers, crystallization takes place for comparably low interaction strengths that do not promote two-body bound states and should thus be observable in ongoing experiments without limitations from three-body recombination.

cond-mat.quant-gas↗

arXiv2025

Quantum Dissipative Continuous Time Crystals

Continuous time crystals, i.e., nonequilibrium phases with a spontaneously broken continuous time-translational symmetry, have been studied and recently observed in the long-time dynamics of open quantum systems. Here, we investigate a lattice of interacting three-level particles and find two distinct time-crystal phases that cannot be described within mean-field theory. Remarkably, one of them emerges only in the presence of correlations, upon accounting for beyond-mean-field effects. Our findings extend explorations of continuous time-translational symmetry breaking in dissipative systems beyond the classical phenomenology of periodic orbits in a low-dimensional nonlinear system. The proposed model applies directly to the laser-driven dynamics of interacting Rydberg states in neutral atom arrays and suggests that the predicted time-crystal phases are observable in such experiments.

quant-ph↗

arXiv2025

Transitional supersolidity in ion doped helium droplets

$^4$He nanodroplets doped with an alkali ion feature a snowball of crystallized layers surrounded by superfluid helium. For large droplets, we predict that a transitional supersolid layer can form, bridging between the solid core and the liquid bulk, where the $^4$He density displays modulations of icosahedral group symmetry. To identify the different phases, we combine density functional theory with the semiclassical Gaussian time-dependent Hartree method for localized many-body systems. This hybrid approach can handle large particle numbers and provides insight into the physical origin of the supersolid layer. For small droplets, we verify that the predictions of our approach are in excellent agreement with Path-Integral Monte Carlo calculations.

cond-mat.quant-gas↗

arXiv2025

Signatures of collective photon emission and ferroelectric ordering of excitons near their Mott insulating state in a WSe$_2$/WS$_2$ heterobilayer

Spontaneous symmetry breaking, arising from the competition of interactions and quantum fluctuations, is fundamental to understanding ordered electronic phases. Although electrically neutral, optical excitations like excitons can interact through their dipole moment, raising the possibility of optically active ordered phases. The effects of spontaneous ordering on optical properties remain largely unexplored. Recent observations of the excitonic Mott insulating state in semiconducting moir\'e crystals make them promising for addressing this question. Here, we present evidence for an in-plane ferroelectric phase of dipolar moir\'e excitons driven by strong exciton-exciton interactions. We discover a surprising speed-up of photon emission at late times and low densities in excitonic decay. This counterintuitive behavior is attributed to collective radiance, linked to the transition between disordered and symmetry-broken ferroelectric phases of moir\'e excitons. Our findings provide first evidence for strong dipolar inter-site interactions in moir\'e lattices, demonstrate collective photon emission as a probe for moir\'e quantum materials, and pave the way for exploring cooperative optical phenomena in strongly correlated systems.

cond-mat.mes-hall↗

arXiv2024

Superradiance of Strongly Interacting Dipolar Excitons in Moir\'e Quantum Materials

Moir\'e lattices created in two-dimensional heterostructures exhibit rich many-body physics of interacting electrons and excitons and, at the same time, suggest promising optoelectronic applications. Here, we study the cooperative radiance of moir\'e excitons that is demonstrated to emerge from the deep subwavelength nature of the moir\'e lattice and the strong excitonic on-site interaction. In particular, we show that the static dipole-dipole interaction between interlayer excitons can strongly affect their cooperative optical properties, suppressing superradiance of disordered states while enhancing superradiance of ordered phases of moir\'e excitons. Moreover, we show that doping permits direct control of optical cooperativity, e.g., by generating supperradiant dynamics of otherwise subradiant states of excitons. Our results show that interlayer moir\'e excitons offer a unique platform for exploring cooperative optical phenomena in strongly interacting many-body systems, thus, holding promise for applications in quantum nonlinear optics.

quant-ph↗

arXiv2024

Chiral Quantum-Optical Elements for Waveguide-QED with Sub-wavelength Rydberg-Atom Arrays

We describe an approach to achieve near-perfect unidirectional light-matter coupling to an effective quantum emitter that is formed by a subwavelength array of atoms in the Rydberg-blockade regime. The nonlinear reflection and transmission of such two-dimensional superatoms are exploited in different interferometric setups for the deterministic generation of tunable single photons and entangling two-photon operations with high fidelities, $\mathcal{F}\gtrsim0.999$. The described setup can function as a versatile nonlinear optical element in a free-space photonic quantum network with simple linear elements and without the need of additional mode confinement, optical resonators, or optical isolators.

quant-ph↗

arXiv2024

Green's function approach to interacting lattice polaritons and optical nonlinearities in subwavelength arrays of quantum emitters

Sub-wavelength arrays of quantum emitters offer an efficient free-space approach to coherent light-matter interfacing, using ultracold atoms or two-dimensional solid-state quantum materials. The combination of collectively suppressed photon-losses and emerging optical nonlinearities due to strong photon-coupling to mesoscopic numbers of emitters holds promise for generating nonclassical light and engineering effective interactions between freely propagating photons. While most studies have thus far relied on numerical simulations, we describe here a diagrammatic Green's function approach that permits analytical investigations of nonlinear processes. We illustrate the method by deriving a simple expression for the scattering matrix that describes photon-photon interactions in an extended two-dimensional array of quantum emitters, and reproduces the results of numerical simulations of coherently driven arrays. The approach yields intuitive insights into the nonlinear response of the system and offers a promising framework for a systematic development of a theory for interacting photons and many-body effects on collective radiance in two-dimensional arrays of quantum emitters.

cond-mat.quant-gas↗

arXiv2024

Nonreciprocal recovery of electromagnetically induced transparency by wavenumber mismatch in hot atoms

For multi-level systems in hot atomic vapors the interplay between the Doppler shift due to atom velocity and the wavenubmer mismatch between driving laser fields strongly influences transmission and absorption properties of the atomic medium. In a three-level atomic ladder-system, Doppler broadening limits the visibility of electromagnetically-induced transparency (EIT) when the probe and control fields are co-propagating, while EIT is recovered under the opposite condition of counter-propagating geometry and $k_{p} < k_{c}$, with $k_{p}$ and $k_{c}$ being the wavenumbers of the probe and control fields, respectively. This effect has been studied and experimentally demonstrated as an efficient mechanism to realize non-reciprocal probe light transmission, opening promising avenues for example for realization of magnetic-field free optical isolators. In this tutorial we discuss the theoretical derivation of this effect and show the underlying mechanism to be an avoided crossing of the states dressed by the coupling laser as a function of atomic velocities when $k_{p}<k_{c}$. We investigate how the non-reciprocity scales with wavelength mismatch and show how to experimentally demonstrate the effect in a simple Rydberg-EIT system using thermal Rubidium atoms.

quant-ph↗

arXiv2024

Self-Induced Superradiant Masing

In cavity quantum electrodynamics (cQED) and particularly superradiance, emitters are typically assumed to be independent, interacting only through light shared via a common mode. While such photon-mediated interactions lead to a rich spectrum of collective optical effects, direct dipole-dipole interactions within the emitter ensemble are generally viewed as a source of decoherence. Here, we uncover a new role for direct spin-spin interactions as a drive for the superradiant dynamics of a hybrid system of nitrogen-vacancy center spins in diamond coupled to a superconducting microwave cavity. After an initial fast superradiant burst, we observe an unexpected train of subsequent emission pulses followed by quasi-continuous masing for up to one millisecond. We show that this surprising behavior arises from spectral hole refilling, where spin inversion is redistributed into the superradiant window of spins resonant with the cavity. We report measurements that clearly exclude other cQED-related effects, and performed microscopic simulations of up to one million spins, which demonstrate that the observed self-induced masing is indeed driven by dipole-dipole interactions between the spins. These findings open new pathways for exploring complex spin-spin interactions in dense disordered systems and offer possibilities for ultra-narrow linewidth solid-state superradiant masers powered purely by microwave-driven spin control.

quant-ph↗

arXiv2024

Superfluid-supersolid phase transition of elongated dipolar Bose-Einstein Condensates at finite temperatures

We analyse the finite-temperature phase diagram of a dipolar Bose Einstein Condensate confined in a tubular geometry. The effect of thermal fluctuations is accounted for by means of Bogoliubov theory employing the local density approximation. In the considered geometry, the superfluid-supersolid phase transition can be of first- and second-order. We discuss how the corresponding transition point is affected by the finite temperature of the system.

cond-mat.quant-gas↗