Offset Dual Microcombs in a Single Microresonator: Kerr-Raman Interleaved Combs
Integrated Kerr microcombs have emerged as a central platform for chip-scale nonlinear photonics. One of their most compelling applications is dual-comb technology, which enables fast, high-resolution, coherent optical spectroscopy, precision metrology, ranging, and ultrasensitive sensing by interfering two frequency combs with slightly different repetition rates. However, no effective strategy yet exists to synergistically excite multiple spatial mode families, manage mode competition and energy partitioning, and precisely engineer dispersion, leaving offset co-propagating dual-microcombs in a single resonator elusive. Here we demonstrate a new mechanism for offset dual microcombs formation via Kerr-Raman interleaving for the first time, by leveraging single Raman-active thin-film lithium niobate microrings. Two spatial mode families with high loaded Q factors up to 5 million are dispersion engineered to have nearly identical free-spectral-ranges but a designed relative frequency offset. Stimulated Raman scattering efficiently generates a Raman comb in one family alongside a Kerr comb in the other. The two combs interleave with a fractional offset to form a broadband, densely interleaved spectrum. Pumping the microring at only 320 mW yields Kerr-Raman interleaved dual combs both featuring nearly identical repetition rates around 102 GHz with a small difference of 675 MHz, a relatively flat envelope exceeding 29 nm and an intrinsic comb-line linewidth of 410 Hz. Our results establish offset dual-comb generation in a single microresonator, enabling compact dual-comb sources for chip-scale precision spectroscopy, Vernier-enhanced sensing, and advanced quantum photonics.