Curvature-stabilized three-dimensional spiral states and local-field nucleation of skyrmions on spherical caps
The combination of polystyrene particles and multilayers with chiral interfacial interactions offers an interesting platform to study the interplay between topology, chirality, and curvature. Here, we investigate Pt/Co/Ta multilayers sputtered onto self-assembled polystyrene particles with a diameter of 919 nm, which show a magnetic reversal distinctly different from that of planar films. Using non-invasive scanning transmission X-ray microscopy and in-vacuum magnetic force microscopy (MFM) with low-moment tips, we observe maze domains in the planar films, whereas the curvilinear films host three-dimensional spiraling stripe states. Repeated scanning with a conventional higher-moment MFM tip ruptures these spirals into metastable skyrmions at the top of the particles. Micromagnetic simulations of spherical caps reveal that increasing curvature renders a single spiral stripe energetically favorable over an isolated skyrmion, and that this stabilization is predominantly of magnetostatic origin. Our results identify the spiral states as intrinsic to the curvilinear geometry and the skyrmions as metastable states nucleated by local magnetic fields, underlining the value of non-invasive imaging to distinguish intrinsic curvature effects from probe-induced magnetic textures.