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At least 19 recordsLinked to original sources

arXiv2007

Plasmon Amplification through Stimulated Emission at Terahertz Frequencies in Graphene

We show that plasmons in two-dimensional graphene can have net gain at terahertz frequencies. The coupling of the plasmons to interband electron-hole transitions in population inverted graphene layers can lead to plasmon amplification through the process of stimulated emission. We calculate plasmon gain for different electron-hole densities and temperatures and show that the gain values can exceed $10^{4}$ cm$^{-1}$ in the 1-10 terahertz frequency range, for electron-hole densities in the $10^{9}$-$10^{11}$ cm$^{-2}$ range, even when plasmon energy loss due to intraband scattering is considered. Plasmons are found to exhibit net gain for intraband scattering times shorter than 100 fs. Such high gain values could allow extremely compact terahertz amplifiers and oscillators that have dimensions in the 1-10 $μ$m range.

cond-mat.mes-hall↗

arXiv2007

Orbital currents in the Colle-Salvetti correlation energy functional and the degeneracy problem

Popular density functionals for the exchange-correlation energy typically fail to reproduce the degeneracy of different ground states of open-shell atoms. As a remedy, functionals which explicitly depend on the current density have been suggested. We present an analysis of this problem by investigating functionals that explicitly depend on the Kohn-Sham orbitals. Going beyond the exact-exchange approximation by adding correlation in the form of the Colle-Salvetti functional we show how current-dependent terms enter the Colle-Salvetti expression and their relevance is evaluated. A very good description of the degeneracy of ground-states for atoms of the first and second row of the periodic table is obtained.

cond-mat.mtrl-sci↗

arXiv2007

Carbon Nanotube Thin Film Field Emitting Diode: Understanding the System Response Based on Multiphysics Modeling

In this paper, we model the evolution and self-assembly of randomly oriented carbon nanotubes (CNTs), grown on a metallic substrate in the form of a thin film for field emission under diode configuration. Despite high output, the current in such a thin film device often decays drastically. The present paper is focused on understanding this problem. A systematic, multiphysics based modelling approach is proposed. First, a nucleation coupled model for degradation of the CNT thin film is derived, where the CNTs are assumed to decay by fragmentation and formation of clusters. The random orientation of the CNTs and the electromechanical interaction are then modeled to explain the self-assembly. The degraded state of the CNTs and the electromechanical force are employed to update the orientation of the CNTs. Field emission current at the device scale is finally obtained by using the Fowler-Nordheim equation and integration over the computational cell surfaces on the anode side. The simulated results are in close agreement with the experimental results. Based on the developed model, numerical simulations aimed at understanding the effects of various geometric parameters and their statistical features on the device current history are reported.

cond-mat.mtrl-sci↗

arXiv2007

Modeling the Field Emission Current Fluctuation in Carbon Nanotube Thin Films

Owing to their distinct properties, carbon nanotubes (CNTs) have emerged as promising candidate for field emission devices. It has been found experimentally that the results related to the field emission performance show variability. The design of an efficient field emitting device requires the analysis of the variabilities with a systematic and multiphysics based modeling approach. In this paper, we develop a model of randomly oriented CNTs in a thin film by coupling the field emission phenomena, the electron-phonon transport and the mechanics of single isolated CNT. A computational scheme is developed by which the states of CNTs are updated in time incremental manner. The device current is calculated by using Fowler-Nordheim equation for field emission to study the performance at the device scale.

cond-mat.mtrl-sci↗

arXiv2007

Counting and manipulating single electrons using a carbon nanotube transistor

We report on the electric measurements of an individual Au nanoparticle with an ultra-high contact resistance of about $10^{19} Ω$. The high-impedance measurements have been carried out by counting the electrons that are transferred onto the particle. In order to do this, a carbon nanotube is used as the electrode for the supply of electrons but also as the detector of the charge transfer. Measurements using single-electron detection allow us to determine the separation between the electron states in the Au nanoparticle, which is about 4 meV, consistent with the charging energy of the particle. Single-electron detection with nanotubes offers great promise for the study of electron transfer in highly resistive molecular systems.

cond-mat.mes-hall↗

arXiv2007

Bound Polaron in CuCl and GaAs Quantum Dots

We calculated the binding energy of a polaron bound to a hydrogenic donor impurity located in a spherical quantum dot by means of a variational and numerical technique for finite potential models. The polaronic effect has been considered taking into account the ion-phonon coupling under the Lee Low Pines approach. The results show that the binding energies are drastically affected by the dot radius, the potential barrier height and the polaronic effects.

cond-mat.other↗

arXiv2008

Molecular dynamics studies on spatial scale of low energy excitation in a simple polymer system

A molecular dynamics simulation is performed to investigate spatial scale of low energy excitation (LEE) in a single linear chain of united atoms. The self part of the dynamic structure function, $S_\mathrm{S}(q,ω)$, is obtained in a wide range in frequency space ($ω$) and reciprocal space ($q$). A broad peak corresponding to the LEE is detected at $ω/2π=2.5 \times 10^{11} \mathrm{s^{-1}}$ ($\equiv ω_{\mathrm{LEE}}/2π$) on the contour maps of $S_\mathrm{S}(q,ω)$, near and below the glass transition temperature ($T_{\mathrm{g}}$=230 K). The $S_\mathrm{S}(q,ω_{\mathrm{LEE}})$ is symmetric around a maximum along the logarithm of $q$. The inverse of $q_{\mathrm{max}}$, giving the maximum position of $S_\mathrm{S}(q,ω_{\mathrm{LEE}})$, depends on temperature as $2π/q_{\mathrm{max}}\sim T^{0.52}$ for $60 \mathrm{K}<T<T_{\mathrm{g}}$ and $2π/q_{\mathrm{max}}\sim T^{0.97}$ for $T_{\mathrm{g}}<T<600 \mathrm{K}$, which is the spatial scale of the motion corresponding to the LEE at low temperatures. Based on a Gaussian approximation for the displacements of monomer groups which give rise to the motion relevant to the LEE, it is found that the number of monomers contained in a group is about 6.

cond-mat.mtrl-sci↗

arXiv2007

Current-Induced Switching of a Single-Molecule Magnet with Arbitrary Oriented Easy Axis

The main objective of this work is to investigate theoretically how tilting of an easy axis of a single-molecule magnet (SMM) from the orientation collinear with magnetic moments of the leads affects the switching process induced by current flowing through the system. To do this we consider a model system that consists of a SMM embedded in the nonmagnetic barrier of a magnetic tunnel junction. The anisotropy axis of the SMM forms an arbitrary angle with magnetic moments of the leads (the latter ones are assumed to be collinear). The reversal of the SMM's spin takes place due to exchange interaction between the molecule and electrons tunneling through the barrier. The current flowing through the system as well as the average z-component of the SMM's spin are calculated in the second-order perturbation description (Fermi golden rule).

cond-mat.mes-hall↗

arXiv2008

Equilibrium and absolute minimal states of Mumford-Shah functionals and brittle fracture propagation

By a combination of geometrical and configurational analysis we study the properties of absolute minimal and equilibrium states of general Mumford-Shah functionals, with applications to models of quasistatic brittle fracture propagation. The main results concern the mathematical relations between physical quantities as energy release rate and energy concentration for 3D cracks with complex shapes, seen as outer measures living on the crack edge.

math.AP↗

arXiv2007

Hidden Symmetry, Excitonic Transitions and Two-Dimensional Kane's Exciton in the Quantum Well

In this article it is shown that, Sommerfeld's coefficients for excitonic transitions in quantum wells are determined only with the principle quantum number within the framework of two-dimensional Coulomb potential. This is a consequence of hidden symmetry of two-dimensional Coulomb problem, conditioned by the existence of two-dimensional analog of the Runge-Lentz vector. For the narrow gap semiconductor quantum well with the non-parabolic dispersion law of electron and hole in the two-band Kane model it is shown that two-dimensional excitonic states are described in the frames of an analog of Klein-Gordon equation with the two-dimensional Coulomb potential. The non-stability of the ground state of the two-dimensional Kane's exciton is show.

cond-mat.other↗

arXiv2007

Experimental study of the coherent A1 phonons in Te with tailored femtosecond pulses

We tailor the shape and phase of the pump pulse spectrum in order to study the coherent lattice dynamics in tellurium. Employing the coherent control via splitting the pump pulse into a two-pulse sequence, we show that the oscillations due to A1 coherent phonons can be cancelled but not enhanced as compared to single pulse excitation. We further demonstrate that a decisive factor for the coherent phonon generation is the bandwidth of the pulse spectrum and not the steepness of the pulse envelope. We also observe that the coherent amplitude for long pump pulses decreases exponentially independent of the shape of the pulse spectrum. Finally, by varying the pulse chirp, we show that the coherent amplitude is independent of while the oscillation lifetime is dependent on the chirp sign.

cond-mat.mtrl-sci↗

arXiv2007

Quantum Hall Effect in a Graphene p-n Junction

We report on the fabrication and transport studies of a single-layer graphene p-n junction. Carrier type and density in two adjacent regions are individually controlled by electrostatic gating using a local top gate and a global back gate. A functionalized Al203 oxide that adheres to graphene and does not significantly affect its electronic properties is described. Measurements in the quantum Hall regime reveal new plateaus of two-terminal conductance across the junction at 1 and 3/2 times the quantum of conductance, e2/h, consistent with theory.

cond-mat.mes-hall↗

arXiv2007

Planar spin-transfer device with a dynamic polarizer

In planar nano-magnetic devices magnetization direction is kept close to a given plane by the large easy-plane magnetic anisotropy, for example by the shape anisotropy in a thin film. In this case magnetization shows effectively in-plane dynamics with only one angle required for its description. Moreover, the motion can become overdamped even for small values of Gilbert damping. We derive the equations of effective in-plane dynamics in the presence of spin-transfer torques. The simplifications achieved in the overdamped regime allow to study systems with several dynamic magnetic pieces (``free layers''). A transition from a spin-transfer device with a static polarizer to a device with two equivalent magnets is observed. When the size difference between the magnets is less than critical, the device does not exhibit switching, but goes directly into the ``windmill'' precession state.

cond-mat.mtrl-sci↗

arXiv2008

Elementary excitations in a supersolid

We study elementary low energy excitations inside a supersolid. We find that the coupling between the longitudinal lattice vibration mode and the superfluid mode leads to two longitudinal modes (one upper branch and one lower branch) inside the supersolid, while the transverse modes in the supersolid stay the same as those inside a normal solid. We also work out various experimental signatures of these novel elementary excitations by evaluating the Debye-Waller factor, density-density correlation, vortex loop-vertex loop interactions, specific heat and excess entropy from the vacancies per mole.

cond-mat.mtrl-sci↗

arXiv2007

Set of equations for transient enhanced diffusion in shallow ion-implanted layers

To simulate the transient enhanced diffusion near the surface or interface, a set of equations describing the impurity diffusion and quasichemical reactions of dopant atoms and point defects in ion-implanted layers is proposed and analyzed. The diffusion equations obtained take into account different charge states of mobile or immobile species and drift the mobile species in the built-in electric field and field of elastic stresses. The absorption of self-interstitials on the surface and drift of the defects due to elastic stresses result in the nonuniform distributions of point defects. It was shown analytically and by means of numerical calculations that consideration of the nonuniform defect distributions enables one to explain the phenomenon of "uphill" impurity diffusion near the surface during annealing of ion-implanted layers. The performed calculations of the boron concentration profile after annealing of a shallow implanted layer agree well with the experimental data confirming the efficiency of the proposed equations.

cond-mat.mtrl-sci↗

arXiv2012

Some problems of low-dimensional physics

Fermi and kinetic energy are usually calculated in periodic boundary conditions model, which is not self-consistent for low-dimensional problems, where particles are confined. Thus for confined particles the potential box model was used self-consistently to calculate Fermi and kinetic energies in 3-, 2-, and 1-dimensional cases. This approach is much more logical and self-consistent. Then the conditions for neglecting dimensions, that is conditions under which the movement of particles in the box could be considered as 2- and 1- dimensional, were derived.

cond-mat.mtrl-sci↗

arXiv2007

Dual-Threshold Percolation

For thermoelectric, galvanomagnetic and some other effects there may simultaneously exist two percolation thresholds, close to which the effective kinetic coefficients of macroscopically disordered media are critically dependent on the proximity to percolation thresholds, their behavior being described by universal critical indexes.

cond-mat.mtrl-sci↗

arXiv2008

Analysis of long range order

A first principles analysis of order-disorder transition in alloys shows that ordering energy is a function of temperature due to thermal vibrations. The inter-nuclear potential energy term converges if zero point vibrations are incorporated and this method can replace the Ewald sum method. Core energy contributions to the ordering energy are stored exclusively in superlattice lines. The effect of electron-phonon interactions on ordering energy is of the same order of magnitude as ordering energy near transition temperatures and cannot be ignored. Ising model and variants are incorrect in explaining alloy phase transitions as they ignore the role of electron-phonon interactions without justification. A theoretical formalism that incorporates the Debye-Waller Factor component of electron-phonon interactions in electronic structure calculations already exists and must be adopted when modeling temperature dependent phenomena. It is suggested that DWF correction will account substantially for the discrepancy between experimental and theoretical ordering energy in Ni3V. Thermal vibrations alter magnetic ordering energy at finite temperatures. The role of electron-phonon interactions in alloy and magnetic phase transitions cannot be ignored and must be incorporated in all models. This will also ensure consistency with x-ray and electron diffraction (alloy transitions) and neutron diffraction (magnetic transitions) results. An isotope effect is predicted for (magnetic) phase transitions if the transition temperature is below Debye temperature. Recent observations of an isotope effect in magnetic phase transitions confirm our above conclusions and imply that the role of electron-phonon interactions must be incorporated in all theories and models of magnetism to avoid contradictions.

cond-mat.mtrl-sci↗