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arXiv · 0804.0504

Spin dependent impurity effects in the 2D frustrated magnetism of NiGa$_2$S$_4$

Yusuke Nambu·Satoru Nakatsuji·Yoshiteru Maeno·Edem K. Okudzeto·Julia Y. Chan
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Abstract

Impurity effects on the triangular antiferromagnets Ni$_{1-x}M_x$Ga$_2$S$_4$ ($M=$ Mn, Fe, Co and Zn) are studied. The 2D frozen spin-disordered state of NiGa$_2$S$_4$ is stable against the substitution of Zn$^{2+}$ ($S=0$) and Heisenberg Fe$^{2+}$ ($S=2$) spins, and exhibits a $T^2$-dependent magnetic specific heat, scaled by the Weiss temperature. In contrast, the substitutions with Co$^{2+}$ ($S=3/2$) spin with Ising-like anisotropy and Heisenberg Mn$^{2+}$ ($S=5/2$) spin induce a conventional spin glass phase. From these comparisons, it is suggested that integer size of Heisenberg spins is important to stabilize the 2D coherent behavior observed in the frozen spin-disordered state.

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Yusuke Nambu, Satoru Nakatsuji, Yoshiteru Maeno, Edem K. Okudzeto, Julia Y. Chan. 2008-04-03. Spin dependent impurity effects in the 2D frustrated magnetism of NiGa$_2$S$_4$. https://arxiv.org/abs/0804.0504

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