Theory of Interacting Cavity Rydberg Polaritons

Abstract

Photonic materials are an emerging platform to explore quantum matter and quantum dynamics. The development of Rydberg electromagnetically induced transparency provided a clear route to strong interactions between individual optical photons. In conjunction with carefully designed optical resonators, it is now possible to achieve extraordinary control of the properties of individual photons, introducing tunable gauge fields whilst imbuing the photons with mass and embedding them on curved spatial manifolds. Building on work formalizing Rydberg-mediated interactions between propagating photons, we develop a theory of interacting Rydberg polaritons in multimode optical resonators, where the strong interactions are married with tunable single-particle properties to build and probe exotic matter. In the presence of strong coupling between the resonator field and a Rydberg-dressed atomic ensemble, a quasiparticle called the "cavity Rydberg polariton" emerges. We investigate its properties, finding that it inherits both the fast dynamics of its photonic constituents and the strong interactions of its atomic constituents. We develop tools to properly renormalize the interactions when polaritons approach each other, and investigate the impact of atomic motion on the coherence of multi-mode polaritons, showing that most channels for atom-polariton cross-thermalization are strongly suppressed. Finally, we propose to harness the repeated diffraction and refocusing of the optical resonator to realize interactions which are local in momentum space. This work points the way to efficient modeling of polaritonic quantum materials in properly renormalized strongly interacting effective theories, thereby enabling experimental studies of photonic fractional quantum Hall fluids and crystals, plus photonic quantum information processors and repeaters.