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arXiv · 1908.03530

Modeling Spin Dynamics in the Singlet Ground State Garnet Ho3Ga5O12

Joseph A. M. Paddison·Paromita Mukherjee·Xiaojian Bai·Zhiling Dun·Christopher R. Wiebe·Haidong Zhou·Jason S. Gardner·Martin Mourigal·Siân E. Dutton
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Abstract

Materials containing non-Kramers magnetic ions can show unusual quantum excitations because of the exact mapping of the two-singlet crystal-field ground state to a quantum model of Ising spins in a transverse magnetic field. Here, we model the magnetic excitation spectrum of garnet-structured Ho3Ga5O12, which has a two-singlet crystal-field ground state. We use a reaction-field approximation to explain published inelastic neutron-scattering data [Zhou et al., Phys. Rev. B 78, 140406(R) (2008)] using a three-parameter model containing the magnetic dipolar interaction, the two-singlet crystal-field splitting, and the nuclear hyperfine coupling. Our study clarifies the magnetic Hamiltonian of Ho3Ga5O12, reveals that the nuclear hyperfine interaction drives magnetic ordering in this system, and provides a framework for quantitative analysis of magnetic excitation spectra of materials with singlet crystal-field ground states.

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Joseph A. M. Paddison, Paromita Mukherjee, Xiaojian Bai, Zhiling Dun, Christopher R. Wiebe, Haidong Zhou, Jason S. Gardner, Martin Mourigal, Siân E. Dutton. 2019-08-09. Modeling Spin Dynamics in the Singlet Ground State Garnet Ho3Ga5O12. https://arxiv.org/abs/1908.03530

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