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arXiv · 2106.00440

Multiple field-induced phases in the frustrated triangular magnet Cs$_3$Fe$_2$Br$_9$

D. Brüning·T. Fröhlich·D. Gorkov·I. Císařová·Y. Skourski·L. Rossi·B. Bryant·S. Wiedmann·M. Meven·A. Ushakov·S. V. Streltsov·D. Khomskii·P. Becker·L. Bohatý·M. Braden·T. Lorenz
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Abstract

The recently discovered material Cs$_3$Fe$_2$Br$_9$ contains Fe$_2$Br$_9$ bi-octahedra forming triangular layers with hexagonal stacking along the $c$ axis. In contrast to isostructural Cr-based compounds, the zero-field ground state is not a nonmagnetic $S=0$ singlet-dimer state. Instead, the Fe$_2$Br$_9$ bi-octahedra host semiclassical $S=5/2$ Fe$^{3+}$ spins with a pronounced easy-axis anisotropy along $c$ and interestingly, the intra-dimer spins are ordered ferromagnetically. The high degree of magnetic frustration due to (various) competing intra- and inter-dimer couplings leads to a surprisingly rich magnetic phase diagram. Already the zero-field ground state is reached via an intermediate phase, and the high-field magnetization and thermal expansion data for $H\parallel c$ identify ten different ordered phases. Among them are phases with constant magnetization of 1/3, respectively 1/2 of the saturation value, and several transitions are strongly hysteretic with pronounced length changes reflecting strong magnetoelastic coupling.

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D. Brüning, T. Fröhlich, D. Gorkov, I. Císařová, Y. Skourski, L. Rossi, B. Bryant, S. Wiedmann, M. Meven, A. Ushakov, S. V. Streltsov, D. Khomskii, P. Becker, L. Bohatý, M. Braden, T. Lorenz. 2021-06-01. Multiple field-induced phases in the frustrated triangular magnet Cs$_3$Fe$_2$Br$_9$. https://doi.org/10.1103/physrevb.104.064418

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