Search arXivSearch

arXiv · 2302.12083

Size effects in the toughening of brittle materials by heterogeneities: a non-linear analysis of front deformations

Abstract

Traditional computational approaches in simulating crack propagation in perfectly brittle materials rely on the estimate of stress intensity factors along the rupture front. This proves highly challenging in 3D when the crack geometry departs from very specific cases for which analytical solutions are available, like e.g. the penny-shaped crack geometry. Here, we extend the first-order theory of Gao and Rice (1987), and predict the distribution of the mode I stress intensity factor $K_\mathrm{I}$ along the front of a tensile coplanar crack that is slightly perturbed from a reference penny-shaped configuration, up to second order in the perturbation amplitude. Our theory is validated against analytical solutions available for embedded elliptical cracks, and its range of validity is further assessed using numerical simulations performed on cosine front perturbations of varying mode and amplitude. It is then used to develop a homogenization framework for the toughness of weakly disordered media. The effective toughness and its fluctuations are bridged quantitatively to the intensity of the toughness fluctuations and their spatial structure. Our theoretical predictions are compared to the results of ~1 million simulations of crack propagation building on our second-order theory and Fast Fourier Transforms. We show that the impact of toughness heterogeneities is size-dependent, as they generally weaken the material when the crack size is lower or comparable to the typical heterogeneity size, but reinforces it otherwise. It results in an apparent R-curve behavior of the brittle composite at the macroscale.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Mathias Lebihain, Manish Vasoya, Véronique Lazarus. 2023-06-26. Size effects in the toughening of brittle materials by heterogeneities: a non-linear analysis of front deformations. https://doi.org/10.1016/j.ijsolstr.2023.112392

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Structure and dynamics of the negative thermal expansion material Cd(CN)$_2$ under hydrostatic pressure

We use a combination of variable-temperature / variable-pressure neutron powder diffraction, variable-pressure inelastic neutron scattering, and quantum chemical calculations to interrogate the behaviour of the negative thermal expansion (NTE) material $^{114}$Cd(CN)$_2$ under hydrostatic pressure. We determine the equation of state of the ambient-pressure phase, and discover the so-called `warm hardening' effect whereby the material becomes elastically stiffer as it is heated. We also identify a number of high-pressure phases, and map out the phase behaviour of Cd(CN)$_2$ over the range $0\leq p\leq0.5$\,GPa, $100\leq T\leq300$\,K. As expected for an NTE material, the low-energy phonon frequencies are found to soften under pressure, and we determine an effective Gr{ü}neisen parameter for these modes. Finally, we show that the elastic behaviour of Cd(CN)$_2$ is sensitive to the local Cd coordination environment, which suggests an interplay between short- (phononic) and long-timescale (cyanide flips) fluctuations in Cd(CN)$_2$.

cond-mat.mtrl-sci

Unconventional Magnetism, Sliding Ferroelectricity, and Magneto-Optical Kerr Effect in Multiferroic Bilayers

Antiferromagnetic (AFM) materials provide a platform to couple altermagnetic (AM) spin-splitting with the magneto-optical Kerr effect (MOKE), offering potential for next-generation quantum technologies. In this work, first-principles calculations, symmetry analysis, and kp modeling are employed to show that interlayer sliding in AFM multiferroic bilayers enables control of electronic, magnetic, and magneto-optical properties. This study reveals an intriguing dimension-driven AM crossover: the 2D paraelectric (PE) bilayer exhibits spin-degenerate bands protected by the [C2||Mc] spin-space symmetry, whereas the 3D counterpart manifests AM spin-splitting along kz \neq 0 paths. Furthermore, interlayer sliding breaks this Mc symmetry and stabilizes a ferroelectric (FE) state with compensated ferrimagnetism, where the Zeeman-like field is responsible for the nonrelativistic spin-splitting. In the FE phase, spin-orbit coupling (SOC) lifts accidental degeneracies and produces `alternating' spin-polarized bands through the interplay of Zeeman and Rashba effects. Crucially, spin polarization, ferrovalley polarization, and the Kerr angle can all be reversed by switching either sliding ferroelectricity or the Neel vector. Our findings reveal the rich coupling among electronic, magnetic, and optical orders in sliding multiferroics, illustrating new prospects for ultralow-power spintronic and optoelectronic devices.

cond-mat.mtrl-sci

Lead-free piezoelectric perovskites for arterial-pulse e-skin: from configurational complexity to equivariant machine-learning potentials

Continuous, non-invasive monitoring of the arterial pulse is a clinical priority for cardiovascular disease, the leading cause of global mortality. Flexible piezoelectric electronic skins can transduce the 1-10 kPa pressure wave into a self-powered voltage, but the best-performing piezoceramics are lead-based, and their toxicity is incompatible with skin contact and with tightening RoHS/REACH regulation. Among lead-free alternatives, the BaTiO$3$-based solid solution BZT-BCT reaches $d{33} \approx 620$ pC/N near its tricritical morphotropic phase boundary, rivalling soft PZT while remaining biocompatible. Exploiting this in a wearable confronts a sensitivity-flexibility paradox and three computational walls: the combinatorial explosion of atomic configurations in a disordered solid solution, the band-gap error of affordable density-functional approximations, which corrupts leakage and insulation estimates, and the 0 K nature of standard calculations against a 310 K operating temperature. We review lead-free piezoelectrics, morphotropic-boundary physics and fabricated flexible devices, then argue that equivariant machine-learning interatomic potentials --- coupled to a tiered functional hierarchy and finite-temperature lattice dynamics --- can survey the full configurational ensemble at body temperature and close the gap to a clinically viable lead-free pulse sensor.

cond-mat.mtrl-sci