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arXiv · 2303.00740

Demonstration of NV-detected $^{13}$C NMR at 4.2 T

Yuhang Ren·Cooper Selco·Dylan Kawashiri·Michael Coumans·Benjamin Fortman·Louis S. Bouchard·Karoly Holczer·Susumu Takahashi
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Abstract

The nitrogen-vacancy (NV) center in diamond has enabled studies of nanoscale nuclear magnetic resonance (NMR) and electron paramagnetic resonance with high sensitivity in small sample volumes. Most NV-detected NMR (NV-NMR) experiments are performed at low magnetic fields. While low fields are useful in many applications, high-field NV-NMR with fine spectral resolution, high signal sensitivity, and the capability to observe a wider range of nuclei is advantageous for surface detection, microfluidic, and condensed matter studies aimed at probing micro- and nanoscale features. However, only a handful of experiments above 1 T were reported. Herein, we report $^{13}$C NV-NMR spectroscopy at 4.2 T, where the NV Larmor frequency is 115 GHz. Using an electron-nuclear double resonance technique, we successfully detect NV-NMR of two diamond samples. The analysis of the NMR linewidth based on the dipolar broadening theory of Van Vleck shows that the observed linewidths from sample 1 are consistent with the intrinsic NMR linewidth of the sample. For sample 2 we find a narrower linewidth of 44 ppm. This work paves the way for new applications of nanoscale NV-NMR.

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Yuhang Ren, Cooper Selco, Dylan Kawashiri, Michael Coumans, Benjamin Fortman, Louis S. Bouchard, Karoly Holczer, Susumu Takahashi. 2023-03-01. Demonstration of NV-detected $^{13}$C NMR at 4.2 T. https://doi.org/10.1103/physrevb.108.045421

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