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arXiv · 2310.16180

Revisiting spin ice physics in the ferromagnetic Ising pyrochlore Pr$_2$Sn$_2$O$_7$

Brenden R. Ortiz·Paul M. Sarte·Ganesh Pokharel·Miles J. Knudston·Steven J. Gomez Alvarado·Andrew F. May·Stuart Calder·Lucile Mangin-Thro·Andrew R. Wildes·Haidong Zhou·Gabriele Sala·Chris R. Wiebe·Stephen D. Wilson·Joseph A. M. Paddison·Adam A. Aczel
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Abstract

Pyrochlore materials are characterized by their hallmark network of corner-sharing rare-earth tetrahedra, which can produce a wide array of complex magnetic ground states. Ferromagnetic Ising pyrochlores often obey the "two-in-two-out" spin ice rules, which can lead to a highly-degenerate spin structure. Large moment systems, such as Ho$_2$Ti$_2$O$_7$ and Dy$_2$Ti$_2$O$_7$, tend to host a classical spin ice state with low-temperature spin freezing and emergent magnetic monopoles. Systems with smaller effective moments, such as Pr$^{3+}$-based pyrochlores, have been proposed as excellent candidates for hosting a "quantum spin ice" characterized by entanglement and a slew of exotic quasiparticle excitations. However, experimental evidence for a quantum spin ice state has remained elusive. Here, we show that the low-temperature magnetic properties of Pr$_2$Sn$_2$O$_7$ satisfy several important criteria for continued consideration as a quantum spin ice. We find that Pr$_2$Sn$_2$O$_7$ exhibits a partially spin-frozen ground state with a large volume fraction of dynamic magnetism. Our comprehensive bulk characterization and neutron scattering measurements enable us to map out the magnetic field-temperature phase diagram, producing results consistent with expectations for a ferromagnetic Ising pyrochlore. We identify key hallmarks of spin ice physics, and show that the application of small magnetic fields ($μ_0 H_c \sim$0.75T) suppresses the spin ice state and induces a long-range ordered magnetic structure. Together, our work clarifies the current state of Pr$_2$Sn$_2$O$_7$ and encourages future studies aimed at exploring the potential for a quantum spin ice ground state in this system.

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Brenden R. Ortiz, Paul M. Sarte, Ganesh Pokharel, Miles J. Knudston, Steven J. Gomez Alvarado, Andrew F. May, Stuart Calder, Lucile Mangin-Thro, Andrew R. Wildes, Haidong Zhou, Gabriele Sala, Chris R. Wiebe, Stephen D. Wilson, Joseph A. M. Paddison, Adam A. Aczel. 2023-10-24. Revisiting spin ice physics in the ferromagnetic Ising pyrochlore Pr$_2$Sn$_2$O$_7$. https://doi.org/10.1103/physrevb.109.134420

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