Stretch-independent magnetization in incompressible magnetorheological elastomers

Abstract

In this study, we perform a critical examination of the phenomenon where the magnetization is stretch-independent in incompressible hard-magnetic magnetorheological elastomers (h-MREs), as observed in several recent experimental and numerical investigations. We demonstrate that the fully dissipative model proposed by Mukherjee et al. (2021) may be reduced, under physically consistent assumptions, to that of Yan et al. (2023), but not that of Zhao et al. (2019). In cases where the h-MRE solid undergoes non-negligible stretching, the model of Zhao et al. (2019) provides predictions that are in disagreement with experimental observations, given that, by construction, that model produces a magnetization response that is not stretch-independent. By contrast, the other two models are able to describe this important feature present in h-MREs, as well as in incompressible magnetically soft s-MRES. Note that in cases where stretching is negligible, such as for inextensible slender structures under bending deformation, the Zhao et al. (2019) model provides accurate predictions despite its underlying assumptions. Additionally, our analysis reveals two key points about the magnetization vector in the context of the more general, fully dissipative model. First, the magnetization can be related to an internal variable in that theory. However, it cannot be formally used as an internal variable except in the special case of an ideal magnet, and, as such, it is subject to constitutive assumptions. Furthermore, we clarify that the magnetization vector alone is insufficient to describe entirely the magnetic response of an MRE solid; instead, the introduction of one of the original Maxwell fields is always necessary for a complete representation.