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arXiv · 2407.14902

Infrared magneto-polaritons in MoTe$_2$ mono- and bilayers

Bo Han·Jamie M. Fitzgerald·Lukas Lackner·Roberto Rosati·Martin Esmann·Falk Eilenberger·Takashi Taniguchi·Kenji Watanabe·Marcin Syperek·Ermin Malic·Christian Schneider
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Abstract

MoTe$_2$ monolayers and bilayers are unique within the family of van-der-Waals materials since they pave the way towards atomically thin infrared light-matter quantum interfaces, potentially reaching the important telecommunication windows. Here, we report emergent exciton-polaritons based on MoTe$_2$ monolayer and bilayer in a low-temperature open micro-cavity in a joint experiment-theory study. Our experiments clearly evidence both the enhanced oscillator strength and enhanced luminescence of MoTe$_2$ bilayers, signified by a 38 \% increase of the Rabi-splitting and a strongly enhanced relaxation of polaritons to low-energy states. The latter is distinct from polaritons in MoTe$_2$ monolayers, which feature a bottleneck-like relaxation inhibition. Both the polaritonic spin-valley locking in monolayers and the spin-layer locking in bilayers are revealed via the Zeeman effect, which we map and control via the light-matter composition of our polaritonic resonances.

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Bo Han, Jamie M. Fitzgerald, Lukas Lackner, Roberto Rosati, Martin Esmann, Falk Eilenberger, Takashi Taniguchi, Kenji Watanabe, Marcin Syperek, Ermin Malic, Christian Schneider. 2024-07-20. Infrared magneto-polaritons in MoTe$_2$ mono- and bilayers. https://arxiv.org/abs/2407.14902

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