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arXiv · 2503.09689

Itinerant Magnetism in Twisted Bilayer WSe$_2$ and MoTe$_2$

Liangtao Peng·Christophe De Beule·Yiyang Lai·Du Li·Li Yang·E. J. Mele·Shaffique Adam
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Abstract

Using a self-consistent Hartree-Fock theory, we show that the recently observed ferromagnetism in twisted bilayer WSe$_2$ [Nat. Commun. 16, 1959 (2025)] can be understood as a Stoner-like instability of interaction-renormalized moiré bands. We quantitatively reproduce the observed Lifshitz transition as function of hole filling and applied electric field that marks the boundary between layer-hybridized and layer-polarized regimes. The former supports a ferromagnetic valley-polarized ground state below half-filling, developing a topological charge gap at half-filling for smaller twist angles. At larger twist angles, the system hosts a gapped triangular Néel antiferromagnet. On the other hand, the layer-polarized regime supports a stripe antiferromagnet below half-filling and a wing-shaped multiferroic ground state above half-filling. We map the evolution of these states as a function of filling factor, electric field, twist angle, and interaction strength. Our results demonstrate that long-range exchange in a symmetry-unbroken parent state with strongly renormalized moiré bands provides a broadly applicable framework to understand itinerant magnetism in moiré TMDs.

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Liangtao Peng, Christophe De Beule, Yiyang Lai, Du Li, Li Yang, E. J. Mele, Shaffique Adam. 2025-12-16. Itinerant Magnetism in Twisted Bilayer WSe$_2$ and MoTe$_2$. https://arxiv.org/abs/2503.09689

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