Search arXivSearch

arXiv · 2606.02238

Sub-cycle field-driven dynamical Berry phase in solids

Abstract

In quantum mechanics, a wavepacket acquires a geometric phase, known as the Berry phase, as it evolves along a closed trajectory in parameter space. In condensed matter systems, the Berry phase underlies a broad range of phenomena, including the anomalous Hall effect, orbital magnetism, and electric polarization. However, in centrosymmetric materials possessing time-reversal (TR) symmetry, its manifestation is suppressed and effectively vanishes. When a system is driven by a strong terahertz (THz) field, it can be coherently driven far from equilibrium, transiently reshaping its symmetry on sub-picosecond timescales. This capability opens new avenues for quantum control with potential applications in information processing and sensing. Here, we experimentally demonstrate that a strong THz field can transiently break inversion symmetry in MgO, inducing a dynamical complex Berry phase, thereby manipulating the topological properties of the material. Applying high-harmonic generation (HHG) spectroscopy, we directly resolve the Berry phase, accessing both its real and imaginary components. The first is associated with coherent intraband dynamics while the second with quantum tunneling through a potential barrier. This observation enables the reconstruction of the time-dependent evolution of the Berry phase within the cycle of the THz field. The coherent manipulation of solids with strong fields, combined with attosecond-resolved HHG spectroscopy, represents a fundamental step toward unveiling and controlling geometric quantum phenomena in condensed matter systems.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Lior Faeyrman, Jianing Zhang, Misha Ivanov, Liang-You Peng, Nirit Dudovich, Riccardo Piccoli. 2026-06-01. Sub-cycle field-driven dynamical Berry phase in solids. https://arxiv.org/abs/2606.02238

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Incommensurate structural and magnetic modulations in potassium-rich cryptomelane, K$_x$Mn$_8$O$_{16}$ ($x\approx1.45$)

Cryptomelane is a hollandite-like material consisting of K$^+$ cations in an $α$-MnO$_2$ tunnel-like crystallographic motif. Cryptomelane with stoichiometry K$_x$Mn$_8$O$_{16}$ ($x\approx1.45$) has been synthesized and its magnetic properties investigated using variable-temperature magnetic susceptibility, heat capacity, and neutron powder diffraction. Three distinct transitions at $T_1=184$\,K, $T_2=54.5$\,K, and $T_3=24$\,K are observed. At $T_1$ there is a subtle tetragonal$\rightarrow$monoclinic transition associated with emergence of a set of non-magnetic superstructure peaks indexable to a $\vec{k}_\mathrm{struc}\approx0.74\vec{c^*}$ incommensurate modulation parallel to the $α$-MnO$_2$ tunnels. Our findings are consistent with a relation previously reported in titanate hollandites, that $x\approx2|\vec{k}_\mathrm{struc}|$. Magnetic Bragg peaks emerge below $T_2=54.5$\,K, and their positions indicate an incommensurate modulated magnetic structure. The model consistent with the data is a dual-$\vec{k}_\mathrm{mag}$ structure with a ferromagnetic $|\vec{k}_\mathrm{mag}|=0$ component and an incommensurate $\vec{k}_\mathrm{mag}\approx0.37\vec{c^*}$, with the latter most likely to be helical. The period of oscillation of the incommensurate magnetic component is in line with predictions based on a Heisenberg spin Hamiltonian [Mandal \textit{et al}. Phys. Rev. B 90, 104420 (2014)]. Below $T_3=24$\,K, there is a magnetic transition, which gives rise to a different set of magnetic Bragg peaks indicative of a highly complex magnetic structure.

cond-mat.mtrl-sci

An anisotropic functional for two-dimensional material systems

Density function theory is the workhorse of modern electronic structure theory. However, its accuracy in practical calculations is limited by the choice of the exchange-correlation potential. In this respect, two-dimensional materials pose a special challenge, as all these materials and their heterostructures have a crucial similarity. The underlying atomic structures are strongly spatially inhomogeneous, implying that current exchange-correlation functionals, that in almost all cases are isotropic, are ill-prepared for an accurate description. We present an anisotropic screened-exchange potential, that remedies this problem and reproduces the band-gap of 2D materials as well as the piecewise linearity of the total energy with fractional occupation number.

cond-mat.mtrl-sci

Thermally-driven reorientation of the Néel vector in altermagnetic MnTe

Altermagnets are novel magnetic systems that possess a spin-polarized electronic band structure without a net magnetic moment, making them promising for device applications. Hexagonal MnTe, a prototypical altermagnet, arguably exhibits the most properties consistent with theoretical predictions, including an anomalous Hall effect despite a vanishing net magnetization, and altermagnetinduced electronic band splitting. However, fundamental questions remain, including why some effects only appear significantly below the magnetic ordering temperature. Here, we resolve this discrepancy by revealing a reorientation of the Néel vector in single-crystalline MnTe. The Néel vector points 30° from the a-axis at low $T$, before aligning directly with the a-axis around $T\simeq 260$ K. We attribute this to single-ion anisotropy, which depends on temperature-dependent lattice parameters. We obtained these results using muon-spin spectroscopy, magnetization measurements, and X-ray diffraction; we show that the findings are consistent with neutron diffraction. Manipulating this effect, for example through strain, could unlock sensitive electronic detection schemes for external stimuli, paving the way for functional altermagnetic devices.

cond-mat.mtrl-sci