In-plane vector-field imaging of propagating surface phonon polaritons

Abstract

Polariton interferometry through optical near-field microscopy has become a powerful tool in nanophotonics, enabling direct spatial access to the propagation characteristics of strongly confined, evanescent polariton modes. Scattering-type near-field optical microscopy has matured as the prime tool for such studies, yet mostly the out-of-plane components of the optical near fields are probed, owing to the elongated geometry of the nanotip. Here, we demonstrate a complementary far-field nonlinear microscopy approach which allows to selectively probe in-plane polariton field components. Accessing the full vector field is interesting when studying complex mode patterns such as hyperbolic polaritons or skyrmions, where the in-plane field components are typically only inferred from the out-of-plane component but not measured directly. To this end, we use nonlinear infrared-visible wide-field sum-frequency generation microscopy, where the short visible wavelength of the nonlinear signal provides the high spatial resolution to access evanescent modes in the infrared. The symmetry selection rules of the nonlinear process further enable polarization-selective imaging of both in-plane polariton field components through spatial interferometry. The concept is demonstrated experimentally using surface phonon polaritons at the AlN-air interface launched by a gold antenna. A simple, semi-analytical model reproduces the peculiar propagation patterns. Hyperspectral imaging with a tunable narrowband laser further gives access to the polariton dispersion. The wide-field methodology holds high promise for in-depth and high-throughput studies of infrared nanophotonic structures.