Growth of Altermagnetic α-MnTe Films: Substrate Variation and Surface Modification

M. Dittmar; L. Hirnet; H. Haberkamm; F. Beisler; C. -W. Chuang; R. Ganser; P. Kagerer; M. -J. Huang; J. Buck; M. Hoesch; K. Rossnagel; M. Ünzelmann; F. Reinert

arXiv · 2608.17513

Growth of Altermagnetic α-MnTe Films: Substrate Variation and Surface Modification

M. Dittmar·L. Hirnet·H. Haberkamm·F. Beisler·C. -W. Chuang·R. Ganser·P. Kagerer·M. -J. Huang·J. Buck·M. Hoesch·K. Rossnagel·M. Ünzelmann·F. Reinert

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Abstract

Manganese telluride (MnTe) in its hexagonal α-MnTe crystal structure has evolved as one of the altermagnet workhorse materials. The synthesis of MnTe thin films is highly relevant for both fundamental science and device applications. Here, we report on the epitaxial growth of MnTe thin films and heterostructures. The films are studied by X-ray and electron diffraction as well as soft X-ray angle-resolved photoemission spectroscopy. We demonstrate the ability to grow high-quality α-MnTe on various substrates, ranging from transparent band insulators, over topological insulators, metallic transition metal chalcogenides, to the van der Waals ferromagnet Fe$_3$GeTe$_2$. While insulating substrates are useful for transport experiments or optical spectroscopy, metallic topological surface states may trigger spintronic interface effects, such as spin-orbit torques. Metallic substrates, in general, are highly relevant to avoid charging at the insulating MnTe films in electron spectroscopy or microscopy methods. Lastly, ferromagnetic substrates will be of interest to control magnetization across the interface. In addition, we discuss the formation of superstructures on the MnTe(0001) surfaces, that emerge directly after growth, upon subsequent tellurium evaporation and after thermal treatment. This will be relevant in further studying the surface magnetic and electronic structure in α-MnTe.

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M. Dittmar, L. Hirnet, H. Haberkamm, F. Beisler, C. -W. Chuang, R. Ganser, P. Kagerer, M. -J. Huang, J. Buck, M. Hoesch, K. Rossnagel, M. Ünzelmann, F. Reinert. 2026-08-18. Growth of Altermagnetic α-MnTe Films: Substrate Variation and Surface Modification. https://arxiv.org/abs/2608.17513

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