Search arXivSearch

arXiv · 2608.27025

Intrinsic anomalous Hall response in the bilayer kagome ferromagnet Co$_3$Sn

Abstract

Transition-metal kagome magnets provide a rich platform for investigating the interplay between layer stacking, magnetic order, and band topology. Here, we report the molecular beam epitaxy and experimental investigation of high-quality thin films of the kagome metal Co$_3$Sn, which has not been synthesized in bulk form yet. Structural and chemical analyses confirm a hexagonal lattice structure ($P6_3/mmc$) composed of direct A-B stacked Co$_3$Sn kagome bilayers. Magnetometry reveals robust easy-plane ferromagnetism with a Curie temperature exceeding $300\,\text{K}$. Magneto-transport measurements demonstrate metallic behavior (carrier density $n\approx5.01\times10^{22}\,\text{cm}^{-3}$) alongside a temperature-independent anomalous Hall conductivity of $σ_{\rm AHE}\approx90\,Ω^{-1}\cdot{\rm cm}^{-1}$, extending from $2\,\text{K}$ up to room temperature. Results from first-principles density functional theory calculations attribute this anomalous Hall response to intrinsic Berry curvature hotspots near the Fermi level in the spin-split band structure. Our results establish Co$_3$Sn as a room-temperature kagome ferromagnet and highlight the impact of the layer stacking sequence on the material properties of kagome metals from the CoSn family.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Yuqi Qin, Soumya Sankar, Xingkai Cheng, Yifan Jiang, Shiming Lei, Junwei Liu, Berthold Jäck. 2026-08-27. Intrinsic anomalous Hall response in the bilayer kagome ferromagnet Co$_3$Sn. https://arxiv.org/abs/2608.27025

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Incommensurate structural and magnetic modulations in potassium-rich cryptomelane, K$_x$Mn$_8$O$_{16}$ ($x\approx1.45$)

Cryptomelane is a hollandite-like material consisting of K$^+$ cations in an $α$-MnO$_2$ tunnel-like crystallographic motif. Cryptomelane with stoichiometry K$_x$Mn$_8$O$_{16}$ ($x\approx1.45$) has been synthesized and its magnetic properties investigated using variable-temperature magnetic susceptibility, heat capacity, and neutron powder diffraction. Three distinct transitions at $T_1=184$\,K, $T_2=54.5$\,K, and $T_3=24$\,K are observed. At $T_1$ there is a subtle tetragonal$\rightarrow$monoclinic transition associated with emergence of a set of non-magnetic superstructure peaks indexable to a $\vec{k}_\mathrm{struc}\approx0.74\vec{c^*}$ incommensurate modulation parallel to the $α$-MnO$_2$ tunnels. Our findings are consistent with a relation previously reported in titanate hollandites, that $x\approx2|\vec{k}_\mathrm{struc}|$. Magnetic Bragg peaks emerge below $T_2=54.5$\,K, and their positions indicate an incommensurate modulated magnetic structure. The model consistent with the data is a dual-$\vec{k}_\mathrm{mag}$ structure with a ferromagnetic $|\vec{k}_\mathrm{mag}|=0$ component and an incommensurate $\vec{k}_\mathrm{mag}\approx0.37\vec{c^*}$, with the latter most likely to be helical. The period of oscillation of the incommensurate magnetic component is in line with predictions based on a Heisenberg spin Hamiltonian [Mandal \textit{et al}. Phys. Rev. B 90, 104420 (2014)]. Below $T_3=24$\,K, there is a magnetic transition, which gives rise to a different set of magnetic Bragg peaks indicative of a highly complex magnetic structure.

cond-mat.mtrl-sci

An anisotropic functional for two-dimensional material systems

Density function theory is the workhorse of modern electronic structure theory. However, its accuracy in practical calculations is limited by the choice of the exchange-correlation potential. In this respect, two-dimensional materials pose a special challenge, as all these materials and their heterostructures have a crucial similarity. The underlying atomic structures are strongly spatially inhomogeneous, implying that current exchange-correlation functionals, that in almost all cases are isotropic, are ill-prepared for an accurate description. We present an anisotropic screened-exchange potential, that remedies this problem and reproduces the band-gap of 2D materials as well as the piecewise linearity of the total energy with fractional occupation number.

cond-mat.mtrl-sci

Thermally-driven reorientation of the Néel vector in altermagnetic MnTe

Altermagnets are novel magnetic systems that possess a spin-polarized electronic band structure without a net magnetic moment, making them promising for device applications. Hexagonal MnTe, a prototypical altermagnet, arguably exhibits the most properties consistent with theoretical predictions, including an anomalous Hall effect despite a vanishing net magnetization, and altermagnetinduced electronic band splitting. However, fundamental questions remain, including why some effects only appear significantly below the magnetic ordering temperature. Here, we resolve this discrepancy by revealing a reorientation of the Néel vector in single-crystalline MnTe. The Néel vector points 30° from the a-axis at low $T$, before aligning directly with the a-axis around $T\simeq 260$ K. We attribute this to single-ion anisotropy, which depends on temperature-dependent lattice parameters. We obtained these results using muon-spin spectroscopy, magnetization measurements, and X-ray diffraction; we show that the findings are consistent with neutron diffraction. Manipulating this effect, for example through strain, could unlock sensitive electronic detection schemes for external stimuli, paving the way for functional altermagnetic devices.

cond-mat.mtrl-sci