Search arXiv⌕ Search

arXiv · 2610.23132

Light-induced local control of magnetic anisotropy and domain pattern in Co/Pt multilayers

Abstract

Control of magnetic anisotropy is essential for the fabrication of next-generation devices in spintronics and magnetic memory. While conventional approaches such as material composition, thermal annealing, and ion bombardment are widely used, achieving spatially resolved, continuous control remains a challenge. Herein, we demonstrate a dual-regime, localized control over both transient magnetic states and permanent intrinsic properties in perpendicularly magnetized Co/Pt multilayers using ultra-short laser pulses. By employing a multi-scale approach combining Kerr microscopy, magnetic force microscopy, and vibrating sample magnetometry, we reveal that low-fluence irradiation enables a reversible, helicity-dependent accumulation of magnetic phases without altering the intrinsic quasistatic properties. Conversely, high-fluence exposure acts as localized thermal annealing that permanently hardens the magnetic system. This structural relaxation leads to a substantial enhancement of the effective perpendicular magnetic anisotropy, driving a twofold increase in the local coercive field and expanding the equilibrium stripe domain width. By offering both reversible spin manipulation and deterministic engineering of 2D magnetic landscapes, this work paves the way towards flexible, lithography-free anisotropy structuring for advanced spintronic applications.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Ivan Soldatov, Aman Singh, Volker Neu, Rudolf Schäfer, Andrei Sherstobitov, Yana Vaynzof, Stanislav Bodnar. 2026-10-16. Light-induced local control of magnetic anisotropy and domain pattern in Co/Pt multilayers. https://arxiv.org/abs/2610.23132

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Landau theory and exchange instabilities in Mn$_5$Si$_3$: A case against strain-induced altermagnetism

Thin-film Mn$_5$Si$_3$ is a prominent altermagnetic candidate owing to its metallicity, demonstrated anisotropic anomalous transport, and proposed $d$-wave exchange splitting that could enable spin-polarized transport. Its postulated altermagnetic structure has zero propagation vector, unlike the bulk collinear antiferromagnetic AFM2 phase, which orders at the $M$ star. We analyze both phases using Landau theory, first-principles paramagnetic-instability calculations, and Monte Carlo simulations. AFM2 appears in Landau theory as a symmetry-protected inversion-even, permutation-odd mode at a single arm of the $M$ star. At $Γ$, the same intracell pattern belongs to the collinear sector of an $E_{2g}$ order parameter; both phases require higher-order terms for their selection. Disordered-local-moment calculations identify the leading exchange instability at $M$, and the resulting classical Heisenberg model orders at the bulk experimental temperature scale into the orthogonal $3M$ phase favored by single-site entropy. Magnetostructural coupling to $E_{2g}$ deformations favors single-$M$ AFM2 ordering. The estimated homogeneous-strain contribution to the relevant quartic coefficient is about a quarter of the competing entropic term near the bulk transition, while internal $E_{2g}$ relaxations are expected to provide additional stabilization. The $Γ$-point $E_{2g}$ mode, whose Landau theory contains the altermagnetic sector, is substantially weaker and further suppressed by epitaxial strain comparable to that reported for Mn$_5$Si$_3$/Si(111) films exhibiting anomalous transport. The same strain reduces the leading magnetic exchange scale. These results explain the bulk $M$-point instability but strongly disfavor relocating the propagation vector from $M$ to $Γ$ in a moderately strained bulklike Mn$_5$Si$_3$ film, leaving the identity of the Hall-active phase unresolved.

cond-mat.mtrl-sci↗

Metastable polar order and phase competition in Carpy-Galy LaTaO4

Carpy-Galy LaTaO$_4$ undergoes a structural sequence linking the antipolar monoclinic $P2_1/c$ ground state and the polar orthorhombic $Cmc2_1$ phase through an incommensurately modulated regime. First-principles calculations identify a metastable polar monoclinic $P2_1$ phase as a commensurate intermediate in the phase-transition landscape. As a common subgroup of $P2_1/c$ and $Cmc2_1$, $P2_1$ provides a symmetry-connected route between the established polymorphs. Mode-resolved energy surfaces for these symmetry-breaking pathways show that coupling between the respective primary order parameters and an isosymmetric relaxation stabilizes the $P2_1$ minimum along both pathways. Consequently, the $P2_1/c\rightarrow P2_1$ transformation has a finite energy barrier, while a restricted soft-mode model retains competing $P2_1$ and $Cmc2_1$ basins over an illustrative range of harmonic stiffness. Lattice-metric and neutron-diffraction comparisons indicate a shared displacement character between the calculated commensurate state and the experimental IC-o modulation, supporting the use of $P2_1$ as a commensurate structural reference for IC-o. Finally, composition-dependent energetics suggest chemical routes for tuning polar-antipolar competition.

cond-mat.mtrl-sci↗

Angular compliance, not amplitude, governs the dielectric response of BaTiO3

Soft-mode theory specifies a frequency, not what a local polar unit does. What real-space motion underlies the dielectric response of BaTiO3 therefore remains unclear. Using electric-field-induced molecular dynamics with a machine-learning force field, we show that the permittivity tracks the field-induced angular redistribution of local Ti-O off-centering, not its magnitude. Temperature and biaxial strain modify the local structure through different microscopic routes, yet both dielectric responses collapse onto a common relation with the same orientational descriptor, providing a real-space counterpart to soft-mode behavior.

cond-mat.mtrl-sci↗