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Why Ni$_3$Al is an itinerant ferromagnet but Ni$_3$Ga is not

A. Aguayo·I. I. Mazin·D. J. Singh
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Abstract

Ni$_3$Al and Ni$_3$Ga are closely related materials on opposite sides of a ferromagnetic quantum critical point. The Stoner factor of Ni is virtually the same in both compounds and the density of states is larger in Ni$_3$Ga. So, according to the Stoner theory, it should be more magnetic, and, in LDA calculations, it is. However, experimentally, it is a paramagnet, while Ni$_3$Al is an itinerant ferromagnet. We show that the critical spin fluctuations are stronger than in Ni$_3$Ga, due to a weaker q-dependence of the susceptibility, and this effect is strong enough to reverse the trend. The approach combines LDA calculations with the Landau theory and the fluctuation-dissipation theorem using the same momentum cut-off for both materials. The calculations provide evidence for strong, beyond LDA, spin fluctuations associated with the critical point in both materials, but stronger in Ni$_3$Ga than in Ni$_3$Al.

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A. Aguayo, I. I. Mazin, D. J. Singh. 2003-11-01. Why Ni$_3$Al is an itinerant ferromagnet but Ni$_3$Ga is not. https://doi.org/10.1103/physrevlett.92.147201

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