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Study of Field-Induced Magnetic Order in Singlet-Ground-State Magnet CsFeCl$_3$

Mitsuru Toda·Yutaka Fujii·Shinji Kawano·Takao Goto·Meiro Chiba·Shizumasa Ueda·Kenji Nakajima·Kazuhisa Kakurai·Jens Klenke·Ralf Feyerherm·Matthias Meschke·Hans Anton Graf·Michael Steiner
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Abstract

The field-induced magnetic order in the singlet-ground-state system CsFeCl$_3$ has been studied by measuring magnetization and neutron diffraction. The field dependence of intensity for the neutron magnetic reflection has clearly demonstrated that the field-induced ordered phase is described by the order parameter $ $. A condensate growth of magnons is investigated through the temperature dependence of $M_z$ and $M_{\perp}$, and this ordering is discussed in the context of a magnon Bose-Einstein condensation. Development of the coherent state and the static correlation length has been observed in the incommensurate phase in the field region of $5 < H < 6$ T at 1.8 K. At $H > H_{\rm c}$, a satellite peak was found in coexistence with the commensurate peak at the phase boundary around 10 T, which indicates that the tilt of the c-axis would be less than $\sim 0.5^{\circ}$ in the whole experiments.

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Mitsuru Toda, Yutaka Fujii, Shinji Kawano, Takao Goto, Meiro Chiba, Shizumasa Ueda, Kenji Nakajima, Kazuhisa Kakurai, Jens Klenke, Ralf Feyerherm, Matthias Meschke, Hans Anton Graf, Michael Steiner. 2004-07-09. Study of Field-Induced Magnetic Order in Singlet-Ground-State Magnet CsFeCl$_3$. https://doi.org/10.1103/physrevb.71.224426

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