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Jaehong Choi

Publications and source records attributed to Jaehong Choi.

9 recordsLinked to original sources

Programmable digital quantum simulation of 2D Fermi-Hubbard dynamics using 72 superconducting qubits

Simulating the time-dynamics of quantum many-body systems was the original use of quantum computers proposed by Feynman, motivated by the critical role of quantum interactions between electrons in the properties of materials and molecules. Accurately simulating such systems remains one of the most promising applications of general-purpose digital quantum computers, in which all the parameters of the model can be programmed and any desired physical quantity output. However, performing such simulations on today's quantum computers at a scale beyond the reach of classical methods requires advances in the efficiency of simulation algorithms and error mitigation techniques. Here we demonstrate programmable digital quantum simulation of the dynamics of the 2D Fermi-Hubbard model -- one of the best-known simplified models of electrons in crystalline solids -- at a scale beyond exact classical state-vector simulation. We implement simulations of this model on lattice sizes up to ${6\times 6}$ using 72 qubits on Google's Willow quantum processor, across a range of physical parameters, including different on-site electron-electron interaction strengths and magnetic flux values, and study phenomena including formation of magnetic polarons (charge carriers surrounded by local magnetic polarisation), dynamical symmetry-breaking in stripe-ordered states, attraction of charge carriers on an entangled background state known as a valence bond solid, and the approach to equilibrium through thermalisation. We validate our results against exact calculations in parameter regimes where these are feasible, and compare them to approximate classical simulations performed using tensor network and operator propagation methods. Our results demonstrate that meaningful programmable digital quantum simulation of many-body interacting electron models is now feasible on state-of-the-art quantum hardware.

quant-ph↗

Multifractal and Glassy Signatures of Non-Ergodic 2D Quantum Dynamics

The fate of ergodicity and localization in disordered, interacting quantum systems in two spatial dimensions remains an outstanding open problem in non-equilibrium physics. Theoretical and numerical approaches are severely constrained by exponential Hilbert space growth. Here, we leverage the high data-acquisition rates of superconducting quantum processors to extensively sample Hilbert space configurations, effectively imaging the state as a wavefunction network (WFN). Tracking the bitstring return probability across varied disorder strengths, we find heavy-tailed distributions and power-law typical decay characteristic of glassy relaxation. Furthermore, the distribution of bitstring probabilities transitions from a Porter-Thomas form at low disorder to an eight-decade power law at stronger disorder. In the reconstructed configuration space, WFN connectivity is compatible with a random geometric network at low disorder and becomes scale-free at stronger disorder. Finally, a multifractal analysis based on the binary intrinsic dimension (BID) reveals a non-ergodic regime where the wavefunction support saturates to a finite fraction of the total Hilbert space. Together, these results rule out a direct ergodic-to-localized transition, pointing instead to an extended multifractal regime. By visualizing wavefunction dynamics directly in configuration space, this work complements traditional real-space studies, showing the potential of quantum processors to resolve long-standing questions in non-equilibrium physics.

quant-ph↗

Active-Learning Inspired $\textit{Ab Initio}$ Theory-Experiment Loop Approach for Management of Material Defects: Application to Superconducting Qubits

Surface oxides are associated with two-level systems (TLSs) that degrade the performance of niobium-based superconducting quantum computing devices. To address this, we introduce a predictive framework for selecting metal capping layers that inhibit niobium oxide formation. Using DFT-calculated oxygen interstitial and vacancy energies as thermodynamic descriptors, we train a logistic regression model on a limited set of experimental outcomes to successfully predict the likelihood of oxide formation beneath different capping materials. This approach identifies Zr, Hf, and Ta as effective diffusion barriers. Our analysis further reveals that the oxide formation energy per oxygen atom serves as an excellent standalone descriptor for predicting barrier performance. By combining this new descriptor with lattice mismatch as a secondary criterion to promote structurally coherent interfaces, we identify Zr, Ta, and Sc as especially promising candidates. This closed-loop strategy integrates first-principles theory, machine learning, and limited experimental data to enable rational design of next-generation materials.

cond-mat.mtrl-sci↗

Low barrier ZrO$_x$-based Josephson junctions

The Josephson junction is a crucial element in superconducting devices, and niobium is a promising candidate for the superconducting material due to its large energy gap relative to aluminum. AlO$_x$ has long been regarded as the highest quality oxide tunnel barrier and is often used in niobium-based junctions. Here we propose ZrO$_x$ as an alternative tunnel barrier material for Nb electrodes. We theoretically estimate that zirconium oxide has excellent oxygen retention properties and experimentally verify that there is no significant oxygen diffusion leading to NbO$_x$ formation in the adjacent Nb electrode. We develop a top-down, subtractive fabrication process for Nb/Zr-ZrO$_x$/Nb Josephson junctions, which enables scalability and large-scale production of superconducting electronics. Using cross sectional scanning transmission electron microscopy, we experimentally find that depending on the Zr thickness, ZrO$_x$ tunnel barriers can be fully crystalline with chemically abrupt interfaces with niobium. Further analysis using electron energy loss spectroscopy reveals that ZrO$_x$ corresponds to tetragonal ZrO$_2$. Room temperature characterization of fabricated junctions using Simmons' model shows that ZrO$_2$ exhibits a low tunnel barrier height, which is promising in merged-element transmon applications. Low temperature transport measurements reveal sub-gap structure, while the low-voltage sub-gap resistance remains in the megaohm range.

cond-mat.supr-con↗

Microscopic mechanisms of flexoelectricity in oxide membranes

Modern electromechanical actuators and sensors rely on the piezoelectric effect that linearly couples strain and electric polarization. However, this effect is restricted to materials that lack inversion symmetry. In contrast, the flexoelectric effect couples strain gradients to electric polarization, and is a universal property in insulating materials of arbitrary symmetry. Flexoelectricity becomes prominent at the nanoscale from the inverse scaling of strain gradients with material dimensions. Here, we measure the strain-gradient-induced structural distortions in strontium titanate using multislice electron ptychography. This technique enables reliable picometer-scale measurements of the dominant oxygen-titanium distortions, correcting for artifacts that limited conventional imaging methods. This enables us to directly measure the sign of the net ionic contribution to the flexoelectric polarization. Guided by the experimental measurements, first-principles calculations show how the sign and magnitude of the bulk contribution to the flexoelectric coefficient in strontium titanate can be switched by tuning the strain state. Hybridization between the optical soft phonon and acoustic phonon modes drives this transition, yielding a large response and a polarity switch across the resonance. This strain-dependence might explain the sign discrepancy and orders of magnitude variation in the values of previously reported flexoelectric coefficients for strontium titanate. As the strain state of curved membranes can be tuned, our approach also suggests an approach to engineer nanoscale flexoelectric polarization using strain as a control parameter.

cond-mat.mtrl-sci↗

Purcell enhancement and spin spectroscopy of silicon vacancy centers in silicon carbide using an ultra-small mode-volume plasmonic cavity

Silicon vacancy (V$_{Si}$) centers in 4H-silicon carbide have emerged as a strong candidate for quantum networking applications due to their robust electronic and optical properties including a long spin coherence lifetime and bright, stable emission. Here, we report the integration of V$_{Si}$ centers with a plasmonic nanocavity to Purcell enhance the emission, which is critical for scalable quantum networking. Employing a simple fabrication process, we demonstrate plasmonic cavities that support a nanoscale mode volume and exhibit an increase in the spontaneous emission rate with a measured Purcell factor of up to 48. In addition to investigating the optical resonance modes, we demonstrate that an improvement in the optical stability of the spin-preserving resonant optical transitions relative to the radiation-limited value. The results highlight the potential of nanophotonic structures for advancing quantum networking technologies and emphasizes the importance of optimizing emitter-cavity interactions for efficient quantum photonic applications.

quant-ph↗

Tuning exciton emission via ferroelectric polarization at a heterogeneous interface between a monolayer transition metal dichalcogenide and a perovskite oxide membrane

We demonstrate the integration of a thin BaTiO$_3$ (BTO) membrane with monolayer MoSe$_2$ in a dual gate device that enables in-situ manipulation of the BTO ferroelectric polarization with a voltage pulse. While two-dimensional (2D) transition metal dichalcogenides (TMDs) offer remarkable adaptability, their hybrid integration with other families of functional materials beyond the realm of 2D materials has been challenging. Released functional oxide membranes offer a solution for 2D/3D integration via stacking. 2D TMD excitons can serve as a local probe of the ferroelectric polarization in BTO at a heterogeneous interface. Using photoluminescence (PL) of MoSe$_2$ excitons to optically readout the doping level, we find that the relative population of charge carriers in MoSe$_2$ depends sensitively on the ferroelectric polarization. This finding points to a promising avenue for future-generations versatile sensing devices with high sensitivity, fast read-out, and diverse applicability for advanced signal processing.

cond-mat.mtrl-sci↗

Magnetic Vortices in the Abelian Higgs Model with Derivative Interactions

We study the properties of a single magnetic vortex and magnetic vortex lattices in a generalization of the Abelian Higgs model containing the simplest derivative interaction that preserves the $U(1)$ gauge symmetry of the original model. The paper is motivated by the study of finite isospin chiral perturbation theory in a uniform, external : since pions are Goldstone bosons of QCD (due to chiral symmetry breaking by the QCD vacuum), they interact through momentum dependent terms. We introduce a uniform external magnetic field and find the asymptotic properties of single vortex solutions and compare them to the well-known solutions of the standard Abelian Higgs Model. Furthermore, we study the vortex lattice solutions near the upper critical field using the method of successive approximations, which was originally used by Abrikosov in his seminal paper on type-II superconductors. We find the vortex lattice structure, which remains hexagonal as in the standard Abelian Higgs model, and condensation energy of the vortex lattices relative to the normal vacuum (in a uniform magnetic field).

hep-th↗

Vortex solutions in the Abelian Higgs Model with a neutral scalar

We construct an extension of the Abelian Higgs model, which consists of a complex scalar field by including an additional real, electromagnetically neutral scalar field. We couple this real scalar field to the complex scalar field via a quartic coupling and investigate $U(1)$ vortex solutions in this "extended Abelian Higgs Model". Since this model has two additional homogeneous ground states, the $U(1)$ vortices that can form in this model have a richer structure than in the Abelian Higgs Model. We also find the "phase diagram" of the model showing the parameter space in which the real scalar particle condenses in the vortex state while having a zero vacuum expectation value in the homogeneous ground state.

hep-th↗