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arXiv · 2604.13640

Strain-Mediated Lattice Reconstruction Enhances Ferromagnetism in Cr2Ge2Te6/WTe2 van der Waals Heterobilayers

Franz Herling·Mireia Torres-Sala·Dorye L. Esteras·Charlotte Evason·Motomi Aoki·Marcos Rosado·Kapil Gupta·Bernat Mundet·Kai Xu·J. Sebastián Reparaz·Kenji Watanabe·Takashi Taniguchi·Dimitre Dimitrov·Vera Marinova·Ivan A. Verzhbitskiy·Goki Eda·José H. Garcia·Stephan Roche·Juan. F. Sierra·Sergio O. Valenzuela
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Abstract

Van der Waals (vdW) heterostructures enable tailored electronic and magnetic phases by stacking atomically thin layers with pristine interfaces. Here, we investigate fully 2D Cr2Ge2Te6/WTe2 heterostructures and identify a strong enhancement of ferromagnetism in Cr2Ge2Te6 (CGT). Magnetotransport measurements across multiple devices with WTe2 thicknesses ranging from monolayer to bulk reveal a robust anomalous Hall effect together with a more than twofold increase of the Curie temperature and substantially enhanced coercive fields. Interface microscopy confirms chemically abrupt vdW interfaces with no detectable interdiffusion, while control experiments rule out processing- or stray-field-induced artifacts. Our experiments and theoretical calculations demonstrate that interfacial charge transfer renders CGT conductive and that proximity-induced lattice distortions in CGT enhance exchange and magnetocrystalline anisotropy. These results establish strain-mediated lattice reconstruction as a strategy for engineering high-temperature magnetic order in 2D heterostructures and clarify that modifications within the magnetic layer itself can govern proximity effects in vdW stacks.

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Franz Herling, Mireia Torres-Sala, Dorye L. Esteras, Charlotte Evason, Motomi Aoki, Marcos Rosado, Kapil Gupta, Bernat Mundet, Kai Xu, J. Sebastián Reparaz, Kenji Watanabe, Takashi Taniguchi, Dimitre Dimitrov, Vera Marinova, Ivan A. Verzhbitskiy, Goki Eda, José H. Garcia, Stephan Roche, Juan. F. Sierra, Sergio O. Valenzuela. 2026-04-15. Strain-Mediated Lattice Reconstruction Enhances Ferromagnetism in Cr2Ge2Te6/WTe2 van der Waals Heterobilayers. https://doi.org/10.1021/acs.nanolett.6c00201

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